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The dynamics of molecular electron excitation and ionisation is studied in real-time for ultra-short IR laser pulses of intensity I>10^{13} W/cm^{2}. The multi-electron molecule is modeled by a system of two active electrons moving in a…

Optics · Physics 2015-06-26 A. I. Pegarkov

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We show that interference phenomena plays a big role for the electron yield in ionization of atoms by an ultra-short laser pulse. Our theoretical study of single ionization of atoms driven by few-cycles pulses extends the photoelectron…

Quantum Physics · Physics 2009-11-13 Diego Arbo , Emil Persson , Joachim Burgdoerfer

The relative roles of multiple electron scattering and in-molecule free-space propagation in transmission electron microscopy of small molecules are discussed. It is argued that while multiple scattering tends to have only a moderate effect…

Image and Video Processing · Electrical Eng. & Systems 2019-12-02 T. E. Gureyev , H. M. Quiney , A. Kozlov , L. J. Allen

Spatial localization of the electrons of an atom or molecule is studied in models of non-relativistic matter coupled to quantized radiation. We give two definitions of the ionization threshold. One in terms of spectral data of cluster…

Mathematical Physics · Physics 2007-05-23 Marcel Griesemer

An electron transport is studied in the system which consists of scanning tunneling microscopy-single molecule magnet-metal. Due to quantum tunneling of magnetization in single-molecule magnet, linear response conductance exhibits stepwise…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Gwang-Hee Kim , Tae-Suk Kim

We analyze the two-dimensional momentum distribution of electrons ionized by few-cycle laser pulses in the transition regime from multiphoton absorption to tunneling by solving the time-dependent Schr\"odinger equation and by a…

Quantum Physics · Physics 2007-05-23 D. G. Arbó , S. Yoshida , E. Persson , K. I. Dimitriou , J. Burgdörfer

It is shown that the geometry of multi-electron threshold ionization in atoms depends on the initial configuration of bound electrons. The reason for this behavior is found in the stability properties of the classical fixed point of the…

Atomic Physics · Physics 2009-11-13 Agapi Emmanouilidou , Peijie Wang , Jan Michael Rost

We present a scheme to synthesize a three-dimensional laser field that produces a chiral electron momentum distribution upon strong-field ionization of atoms. Our approach employs two orthogonally propagating two-color laser beams. This…

The electric microfield distribution at charged particles is studied for two-component electron-ion plasmas using molecular dynamics simulation and theoretical models. The particles are treated within classical statistical mechanics using…

Plasma Physics · Physics 2009-11-11 H. B. Nersisyan , C. Toepffer , G. Zwicknagel

Scanning tunneling spectroscopy measures how a single electron with definite energy propagates between a sample surface and the tip of a scanning tunneling microscope. In the simplest description, the differential conductance measured is…

Mesoscale and Nanoscale Physics · Physics 2019-05-07 Mikko M. Ervasti , Fabian Schulz , Peter Liljeroth , Ari Harju

We study strong-field double ionization in a three-electron atom by applying a simplified, reduced-dimensionality model with three active electrons. The influence of the spin-induced symmetry of the spatial part of the wavefunction on the…

In a previous contribution, we have set up the framework for the calculation of electronic friction for a slow atom traveling through a metal. We provide in the present work a generalization to the case of polyatomic molecules. This…

Other Condensed Matter · Physics 2014-02-19 A. Salin

We study a general problem of the translational/rotational/vibrational/electronic dynamics of a diatomic molecule exposed to an interaction with an arbitrary external electromagnetic field. The theory developed in this paper is relevant to…

Quantum Physics · Physics 2016-09-28 Milan Sindelka , Nimrod Moiseyev

We consider tunneling to the continuum in a multi-dimensional potential. It is demonstrate that this problem can be treated as two separate problems: a) a bound state and b) a non-resonance scattering problem, by a proper splitting of the…

Nuclear Theory · Physics 2016-11-23 S. A. Gurvitz

We develop a correlated-electron minimal model for the normal state of charged phenanthrene ions in the solid state, within the reduced space of the two lowest antibonding molecular orbitals of phenanthrene. Our model is general and can be…

Strongly Correlated Electrons · Physics 2014-06-25 Tirthankar Dutta , Sumit Mazumdar

The elastic scattering of twisted electrons by diatomic molecules is studied within the framework of the non-relativistic first Born approximation. In this process, the coherent interaction of incident electrons with two molecular centers…

Atomic Physics · Physics 2018-10-17 A. V. Maiorova , S. Fritzsche , R. A. Mueller , A. Surzhykov

A theoretical derivation is given for the formula describing N-electron ionization of atom by a dc field and laser radiation in tunneling regime. Numerical examples are presented for noble gases atoms.

Atomic Physics · Physics 2009-10-31 B. A. Zon

Laser-induced optical potentials for atoms have led to remarkable advances in precision measurement, quantum information, and towards addressing fundamental questions in condensed matter physics. Here, we describe analogous optical…

Materials Science · Physics 2010-11-11 Martin J. A. Schuetz , Michael G. Moore , Carlo Piermarocchi

We consider correlation-assisted tunnel ionization of a small molecule by an intense low-frequency laser pulse. In this mechanism, the departing electron excites the state of the ion via a Coulomb interaction. We show that the angular…

Atomic Physics · Physics 2014-04-25 Emilio Pisanty , Misha Ivanov
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