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X-ray magnetic circular dichroism spectroscopy using an X-ray free electron laser is demonstrated with spectra over the Fe L$_{3,2}$-edges. This new ultrafast time-resolved capability is then applied to a fluence-dependent study of…

We propose a semi-classical model for femtosecond-laser induced demagnetization due to spin-polarized excited electron diffusion in the super-diffusive regime. Our approach treats the finite elapsed time and transport in space between…

Materials Science · Physics 2011-06-14 Marco Battiato , Karel Carva , Peter M. Oppeneer

We report cooperative magnetic orderings in a 6H-perovskite multiferroic system, Ba3HoRu2O9, via comprehensive neutron powder diffraction measurements. This system undergoes long-range antiferromagnetic ordering at TN1 ~ 50 K with a…

Strongly Correlated Electrons · Physics 2020-07-29 T. Basu , V. Caignaert , F. Damay , T. W. Heitmann , B. Raveau , X. Ke

The complex interplay between the 3d and 4f moments in hexagonal ErMnO3 is investigated by magnetization, optical second harmonic generation, and neutron-diffraction measurements. We revise the phase diagram and provide a microscopic model…

Strongly Correlated Electrons · Physics 2012-11-14 D. Meier , H. Ryll , K. Kiefer , B. Klemke , J. -U. Hoffmann , R. Ramesh , M. Fiebig

We study the ultrafast demagnetization dynamics of LnRh$_2$Si$_2$ (Ln $=$ Pr, Nd, Sm, Gd, Tb, Dy, Ho) antiferromagnets (AFM) after excitation by a laser pulse, using a combination of density functional theory and atomistic spin and…

We theoretically investigate laser-induced spin transport in metallic magnetic heterostructures using an effective spin transport description that treats itinerant electrons and thermal magnons on an equal footing. Electron-magnon…

Mesoscale and Nanoscale Physics · Physics 2022-04-27 Maarten Beens , Rembert A. Duine , Bert Koopmans

We report on the ultrafast dynamics of magnetic order in a single crystal of CuO at a temperature of 207 K in response to strong optical excitation using femtosecond resonant x-ray diffraction. In the experiment, a femtosecond laser pulse…

Photo-excitation in complex oxides1 transfers charge across semicovalent bonds, drastically perturbing spin and orbital orders2. Light may then be used in compounds like magnetoresistive manganites to control magnetism on nanometre…

Low-lying relaxation satellites give rise to ultrafast electron dynamics following outer-valence ionization of a molecular system is studied. To demonstrate the impact of such satellites, the evolution of the electronic cloud after sudden…

Chemical Physics · Physics 2015-05-13 Siegfried Lünnemann , Alexander I. Kuleff , Lorenz S. Cederbaum

We review neutron scattering investigations of the crystal structures, magnetic structures, and spin dynamics of the iron-based RFe(As,P)O (R=La, Ce, Pr, Nd), (Ba,Sr,Ca)Fe2As2, and Fe1+x(Te-Se) systems. On cooling from room temperature all…

Superconductivity · Physics 2009-05-20 Jeffrey W. Lynn , Pengcheng Dai

Due to a ferromagnetic in-chain coupling between Co$^{3+}$ ions at trigonal sites, chains Co$_2$O$_6$ are considered as large rigid spin moments. The antiferromagnetic Ising model on the triangular lattice is applied to describe an…

Strongly Correlated Electrons · Physics 2009-11-11 Yuri B. Kudasov

We report on the magnetic properties of HoCo dimers as a model system for the smallest intermetallic transition metal-lanthanide compound. The dimers are adsorbed on ultrathin MgO(100) films grown on Ag(100). New for $4f$ elements, we…

Atomic and Molecular Clusters · Physics 2018-12-26 A. Singha , F. Donati , F. D. Natterer , C. Wäckerlin , S. Stavrić , Z. S. Popović , {Ž}. {Š}ljivan{č}anin , F. Patthey , H. Brune

Neutron diffraction, magnetization and muon spin relaxation measurements, supplemented by density functional theory (DFT) calculations are employed to unravel temperature-driven magnetization reversal (MR) in inverse spinel Co$_2$VO$_4$.…

We have studied the crystal and magnetic structures of the magnetoelectric materials RMn2O5 (R = Tb, Ho, Dy) using neutron diffraction as a function of temperature. All three materials display incommensurate antiferromagnetic ordering below…

Strongly Correlated Electrons · Physics 2009-11-11 G. R. Blake , L. C. Chapon , P. G. Radaelli , S. Park , N. Hur , S-W. Cheong , J. Rodriguez-Carvajal

Antiferromagnetism is relevant to high temperature (high-Tc) superconductivity because copper oxide and iron arsenide high-Tc superconductors arise from electron- or hole-doping of their antiferromagnetic (AF) ordered parent compounds.…

Superconductivity · Physics 2010-02-07 Jun Zhao , D. T. Adroja , Dao-Xin Yao , R. Bewley , Shiliang Li , X. F. Wang , G. Wu , X. H. Chen , Jiangping Hu , Pengcheng Dai

X-ray magnetic circular and linear dichroism (XMCD and XMLD) have been used to investigate the Fe magnetic response during the spin reorientation transition (SRT) in TmFeO3. These experiments are complemented with resonant magnetic…

Static and dynamic magnetic properties of P\={3}1$m$-phase MnSb$_2$O$_6$ have been studied by means of muon spin relaxation ($\mu$SR), high-frequency electron spin resonance (HF-ESR), specific heat, and magnetisation studies in magnetic…

Ultrafast strengthening or quenching of the ferromagnetic order of semiconducting Eu1-xGdxO was achieved by resonant photoexcitation. The modification of the magnetic order is established within 3 ps as revealed by optical second harmonic…

We report the electronic and magnetic behaviour of the frustrated triangular metallic antiferromagnet 2H-AgNiO2 in high magnetic fields (54 T) using thermodynamic and transport measurements. Here localized d electrons are arranged on an…

Current induced magnetization manipulation is a key issue for spintronic application. Therefore, deterministic switching of the magnetization at the picoseconds timescale with a single electronic pulse represents a major step towards the…

Materials Science · Physics 2017-04-13 Y. Xu , M. Deb , G. Malinowski , M. Hehn , W. Zhao , S. Mangin