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Energy barriers for different moves of a single Rh adatom in the vicinity of steps on Rh(111) surface are studied with molecular statics. Interatomic interactions are modeled by the semi-empirical many-body Rosato-Guillope-Legrand…

Materials Science · Physics 2016-08-31 F. Maca , M. Kotrla , O. S. Trushin

In this paper we develop a model to describe the diffusion process in a porous medium. For the observed decrease in current yield, we propose other causes than difference in diffusivity, which we consider unaltered by the porous medium. The…

Chemical Physics · Physics 2012-05-10 P. C. T. DÁjello , G. L. Nunes , J. J. Piacentini , L. Lauck

We study kinetics of electrons, scattered by heavy particles undergoing slow diffusive motion. In a three-dimensional space we claim the existence of the crossover region (on the energy axis), which separates the states with fast diffusion…

Disordered Systems and Neural Networks · Physics 2007-05-23 E. Kogan

We examine the ionic migration of Li in LATP [$\text{Li}_{1+x} \text{Al}_x \text{Ti}_{2-x} {(\text{P} \text{O}_4)}_3$] solid electrolytes from an atomistic viewpoint by means of density functional theory calculations. We vary the Al content…

Materials Science · Physics 2021-08-20 Daniel Pfalzgraf , Daniel Mutter , Daniel F. Urban

We study the phase behaviour of a fluid composed of particles which interact via a pair potential that is repulsive for large inter-particle distances, is attractive at intermediate distances and is strongly repulsive at short distances…

Soft Condensed Matter · Physics 2008-09-17 A. J. Archer , C. Ionescu , D. Pini , L. Reatto

We propose a unified diffusion-mobility relation which quantifies both quantum and classical levels of understanding on electron dynamics in ordered and disordered materials. This attempt overcomes the inability of classical Einstein…

Other Condensed Matter · Physics 2017-05-11 K. Navamani , Swapan K. Pati

We study quantum transport properties of finite periodic quasi-one-dimensional waveguides whose classical dynamics is diffusive. The system we consider is a scattering configuration, composed of a finite periodic chain of $L$ identical…

Statistical Mechanics · Physics 2012-01-18 Jaime Zuñiga Vukusich

We study the long-time self-diffusion of a single conjugated organic para-sexiphenyl (p-6P) molecule physisorbed on the inorganic ZnO $\left(10\overline{1}0\right)$ surface by means of all-atom molecular dynamics computer simulations. We…

Materials Science · Physics 2014-08-20 Karol Palczynski , Joachim Dzubiella

Y-doped BaZrO$_3$ is a promising proton conductor for intermediate temperature solid oxide fuel cells. In this work, a combination of static DFT calculations and DFT based molecular dynamics (DFT-MD) was used to study proton conduction in…

We propose an experimental method to fully characterize the energy exchange of particles during the physical vapor deposition process of thin surface layers. Our approach is based on the careful observation of perturbations of the…

This article is devoted to investigation of cation self-diffusion mechanisms, taking place in UO2, UO2+x, and UO2-x crystals simulated under periodic (PBC) and isolated (IBC) boundary conditions using the method of molecular dynamics in the…

Materials Science · Physics 2015-06-15 A. S. Boyarchenkov , S. I. Potashnikov , K. A. Nekrasov , A. Ya. Kupryazhkin

A model of the collisional kinetics of energetic hydrogen atoms, molecules, and ions in pure H$_2$ discharges is used to predict H$_\alpha$ emission profiles and spatial distributions of emission from the cathode regions of low-pressure,…

Plasma Physics · Physics 2015-05-20 A. V. Phelps

Diffusion is often accompanied by a reaction or sorption which can induce temperature inhomogeneities. Monte Carlo simulations of Lennard-Jones atoms in zeolite NaCaA are reported with a hot zone presumed to be created by a reaction. Our…

Statistical Mechanics · Physics 2019-05-15 A. V. Anil Kumar , S. Yashonath , G. Ananthakrishna

We study the dynamics of the quantum phase distribution associated with the reduced density matrix of a system for a number of situations of practical importance, as the system evolves under the influence of its environment, interacting via…

Quantum Physics · Physics 2009-11-13 Subhashish Banerjee , R. Srikanth

The interaction between an atom and the quantized electromagnetic field depends on the position of the atom. Then the atom experiences a force which is the minus gradient of this interaction. Through the Heisenberg equations of motion and…

Quantum Physics · Physics 2021-11-11 Li Ge

We consider a two dimensional Turing like system with two diffusing species which interact with each other. Considering the species to be charged, we include the effect of an electric field along a given direction which can lead to a drift…

Other Condensed Matter · Physics 2008-12-31 B K Agarwalla , J K Bhattacharjee , P Titum

We demonstrate the phenomenon of directed diffusion in a symmetric periodic potential. This has been realized with cold atoms in a one-dimensional dissipative optical lattice. The stochastic process of optical pumping leads to a diffusive…

The reaction dynamics of H$_2$COO to form linear HCOOH and dioxirane as first steps for OH-elimination is quantitatively investigated. Using a machine learned potential energy surface at the CASPT2/aug-cc-pVTZ level of theory vibrational…

Chemical Physics · Physics 2024-02-16 Kaisheng Song , Meenu Upadhyay , Markus Meuwly

The high-temperature performance of liquid $Li_{17}Pb_{83}$, a key fusion reactor material, is governed by its atomic-scale dynamics. Using ab initio molecular dynamics, we discover that lithium diffusion is not free but confined within…

Materials Science · Physics 2025-11-13 Sensen Lin , Yang Gao , Yongheng Lu , Yongkuan Zhang , Yiqiang Sun

The native point defects are studied in LiGaO2 using hybrid functional calculations. We find that the relative energy of formation of the cation vacancies and the cation antisite defects depends strongly on the chemical potential…

Materials Science · Physics 2020-01-08 Adisak Boonchun , Klichchupong Dabsamut , Walter R. L. Lambrecht