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Divalent atoms provide excellent means for advancing control in Rydberg atom-based quantum simulation and computing, due to the second optically active valence electron available. Particularly promising in this context are circular Rydberg…

We describe a method for controlling many-body states in extended ensembles of Rydberg atoms, forming crystalline structures during laser excitation of a frozen atomic gas. Specifically, we predict the existence of an excitation number…

Atomic Physics · Physics 2015-05-14 T. Pohl , E. Demler , M. D. Lukin

Rydberg atoms, with their giant electronic orbitals, exhibit dipole-dipole interaction reaching the GHz range at a distance of a micron, making them a prominent contender for realizing quantum operations well within their coherence time.…

The formation of rf-dressed Rydberg dark states in thermal Rb vapour is demonstrated. It is shown that such states exhibit enhanced sensitivity to dc electric fields compared to their bare counterparts and enable precise measurement of the…

Anapole states associated with the resonant suppression of electric-dipole scattering exhibit minimized extinction and maximized storage of electromagnetic energy inside a particle. Using numerical simulations, optical extinction…

The Stark effect provides a powerful method to shift the spectra of molecules, atoms and electronic transitions in general, becoming one of the simplest and most straightforward way to tune the frequency of quantum emitters by means of a…

We investigate the electronic structure and properties of Rydberg atoms exposed to a magnetic quadrupole field. It is shown that the spatial as well as generalized time reversal symmetries lead to a two-fold degeneracy of the electronic…

Atomic Physics · Physics 2007-05-23 I. Lesanovsky , J. Schmiedmayer , P. Schmelcher

In an experiment on three-photon laser excitation $5S_{1/2} \to 5P_{3/2} \to 6S_{1/2} \to 37P_{3/2}$ of a single $^{87}$Rb Rydberg atom in an optical dipole trap, we have observed for the first time three-photon Rabi oscillations between…

Open systems that are weakly coupled to a thermal environment and driven by fast, periodically oscillating fields are commonly assumed to approach an equilibrium-like steady state with respect to a truncated Floquet-Magnus Hamiltonian.…

Statistical Mechanics · Physics 2025-02-04 Wilson S. Martins , Federico Carollo , Kay Brandner , Igor Lesanovsky

We present measurements of the resonant microwave absorption by the Rydberg energy levels of surface state electrons on the surface of superfluid liquid helium, in the frequency range 165 - 220 GHz. The resonant frequency was strongly…

Mesoscale and Nanoscale Physics · Physics 2017-12-27 E. Collin , W. Bailey , P. Fozooni , P. G. Frayne , P. Glasson , K. Harrabi , M. J. Lea

We report first ab initio relativistic correlation calculations of potential curves for ten low-lying electronic states, effective electric field on the electron and hyperfine constants for the ^3\Delta_1 state of cation of a heavy…

Atomic Physics · Physics 2013-05-29 A. N. Petrov , N. S. Mosyagin , T. A. Isaev , A. V. Titov

A new synchrotron study for CH$_2$F$_2$ from has been combined with earlier data. The onset of absorption, band I and also band IV, is resolved into broad vibrational peaks, which contrast with the continuous absorption previously claimed.…

High Rydberg states of nitric oxide (NO) with principal quantum numbers between 40 and 100 and lifetimes in excess of 10 $\mu$s have been prepared by resonance enhanced two-color two-photon laser excitation from the X $^2\Pi_{1/2}$ ground…

Chemical Physics · Physics 2020-05-04 A. Deller , S. D Hogan

Rydberg atom-based electrometry enables traceable electric field measurements with high sensitivity over a large frequency range, from gigahertz to terahertz. Such measurements are particularly useful for the calibration of radio frequency…

Quantum Physics · Physics 2017-04-26 Santosh Kumar , Haoquan Fan , Harald Kübler , Akbar J. Jahangiri , James P. Shaffer

Rydberg atoms, which possess exceptionally large electric dipole moments, offer a promising route for electric field sensing as well as metrology traceable to the International System of Units (SI); however, current research predominantly…

Quantum Physics · Physics 2026-04-20 Tianyu Zhou , Haipeng Xie , Xin Wang

We studied magneto-optical resonances caused by excited-state level crossings in a nonzero magnetic field. Experimental measurements were performed on the transitions of the $D_2$ line of rubidium. These measured signals were described by a…

Stark-induced electric dipole amplitudes between states of the same nominal parity can be important in experiments to observe parity nonconservation in atoms. The Stark-induced E1 amplitudes are expressed in terms of an irreducible…

Atomic Physics · Physics 2007-05-23 David DeMille , Mikhail Kozlov

We present a comprehensive study of the diverse properties of heteronuclear Rydberg molecules, placing a special emphasis on those composed of the light alkali atoms, Li, Na, and K. Electron-atom scattering phase shifts, which determine the…

Atomic Physics · Physics 2019-02-13 Matthew T. Eiles

In a recent article Wang et al. (Class. Quantum Grav. 23 (2006) L59), demonstrated that the phase of a particle fluctuates due to interactions with random deviations of a conformal gravitational field. Furthermore they demonstrated that…

General Relativity and Quantum Cosmology · Physics 2009-05-05 Mark S. Everitt , Martin L. Jones , Benjamin T. H. Varcoe

Ultralong-range Rydberg molecules, composed of an excited Rydberg atom and a ground-state atom, are characterized by large bond lengths, dipole moments, sensitivity to external fields, and an unusual binding mechanism based on low-energy…

Atomic Physics · Physics 2025-05-13 Agata Wojciechowska , Michał Tomza , Matthew T. Eiles