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We report on the transfer of coherence from a quantum-well electron-hole condensate to the light it emits. As a function of density, the coherence of the electron-hole pair system evolves from being full for the low density Bose-Einstein…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 A. Olaya-Castro , F. J. Rodriguez , L. Quiroga , C. Tejedor

The creation of superpositions of hole states via single-photon ionization using attosecond extreme-ultraviolet pulses is studied with the time-dependent configuration interaction singles (TDCIS) method. Specifically, the degree of…

Atomic Physics · Physics 2011-02-04 Stefan Pabst , Loren Greenman , Phay J. Ho , David A. Mazziotti , Robin Santra

Transient XUV spectroscopy is growing in popularity for the measurement of solar fuel and photovoltaic materials as it can separately measure electron and hole energies for multiple elements at once. However, interpretation of transient XUV…

Materials Science · Physics 2021-08-06 Hanzhe Liu , Jonathan M. Michelsen , Isabel M. Klein , Scott K. Cushing

We develop photoelectron interferometry based on laser-assisted extreme ultraviolet ionization for flexible and robust control of photoelectron circular dichroism in randomly oriented chiral molecules. A comb of XUV photons ionizes a sample…

We consider the ionisation of atomic hydrogen by a strong infrared field. We extend and study in more depth an existing semi-analytical model. Starting from the time-dependent Schroedinger equation in momentum space and in the velocity…

The concept of using photoelectron interferometry in short laser fields to probe electron dynamics and target structures was introduced more than two decades ago. However, the quality of experimental data has remained insufficient for…

Using a three-dimensional quasiclassical technique we explore the double ionization pathways of a diatomic molecule driven by an intense infrared (800nm) ultrashort laser pulse. For intensities corresponding to the tunneling regime, we find…

Atomic Physics · Physics 2009-02-26 Agapi Emmanouilidou

We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…

We present a source of coherent extreme ultraviolet (XUV) radiation with a flux of 10$^{13}$ photons per second at 26.5 eV. The source is based on high-harmonic generation (HHG) in argon and pumped by a frequency-doubled 100 kHz repetition…

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

Plasma high harmonics generation from an extremely intense short-pulse laser is explored by including the effects of ion motion, electron-ion collisions and radiation reaction force in the plasma dynamics. The laser radiation pressure…

Plasma Physics · Physics 2017-05-17 Suo Tang , Naveen Kumar , Christoph H. Keitel

A proposal for a novel source of isolated attosecond XUV -- soft X-ray pulses with a well controlled carrier-envelope phase difference (CEP) is presented in the framework of nonlinear Thomson-backscattering. Based on the analytic solution…

Atomic Physics · Physics 2019-05-07 Szabolcs Hack , Sándor Varró , Attila Czirják

Strong-field ionization generally produces ions in a superposition of ionic eigenstates. This superposition is generally not fully coherent und must be described in terms of a density matrix. A recent experiment [E. Goulielmakis et al.,…

Atomic Physics · Physics 2015-05-27 Robin Santra , Vladislav S. Yakovlev , Thomas Pfeifer , Zhi-Heng Loh

The dissociative ionization of H2+ interacting with intense, femtosecond extreme-ultraviolet laser pulses is investigated theoretically. This is done by numerical propagation of the time-dependent Schr\"{o}dinger equation for a colinear…

Atomic Physics · Physics 2015-02-25 Lun Yue , Lars Bojer Madsen

The effective transparency of rare-gas clusters, post-interaction with an extreme ultraviolet (XUV) pump pulse, is predicted by using an atomistic hybrid quantum-classical molecular dynamics model. We find there is an intensity range for…

Atomic and Molecular Clusters · Physics 2016-06-21 Rishi Pandit , Kasey Barrington , Thomas Teague , Zachary Hartwick , Nicolas Bigaouette , Lora Ramunno , Edward Ackad

Clusters excited by intense laser pulses are a unique source of warm dense matter, that has been the subject of intensive experimental studies. The majority of those investigations concerns atomic clusters, whereas the evolution of…

Atomic and Molecular Clusters · Physics 2015-06-18 M. Negro , H. Ruf , B. Fabre , F. Dorchies , M. Devetta , D. Staedter , C. Vozzi , Y. Mairesse , S. Stagira

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

Atomic Physics · Physics 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos

We investigate theoretically charge migration following prompt double ionization of a polyatomic molecule (C$_2$H$_4$BrI) and find that for double ionization, correlation-driven charge migration appears to be particularly prominent, i.e.,…

Chemical Physics · Physics 2016-05-24 Maximilian Hollstein , Robin Santra , Daniela Pfannkuche

A heavy hole confined to an InGaAs quantum dot promises the union of a stable spin and optical coherence to form a near perfect, high-bandwidth spin-photon interface. Despite theoretical predictions and encouraging preliminary measurements,…

Quantum Physics · Physics 2018-07-04 L. Huthmacher , R. Stockill , E. Clarke , M. Hugues , C. Le Gall , M. Atatüre

We present an ab initio study of the nonsequential strong-field ionization dynamics of a model two-electron atom with helium character. Single- and double-ionization events are characterized and displayed using detector signals extracted at…

Atomic Physics · Physics 2023-06-14 Daniel Younis , Joseph H. Eberly