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We successfully dope the magnetically silent double perovskite semiconductor Sr2GaSbO6 to induce ferromagnetism and tune its band gap, with Ga3+ partially substituted by the magnetic trivalent cation Mn3+, in a rigid cation ordering with…

Materials Science · Physics 2022-01-24 Lun Jin , Danrui Ni , Xin Gui , Daniel B. Straus , Qiang Zhang , Robert J. Cava

Multiferroic compounds have gained research attention in the field of ferroelectric photovoltaics due to the presence of transition-metal d states from magnetic ions, which tend to reduce the bandgap value. In this work,…

Materials Science · Physics 2023-11-13 L. Imhoff , M. B. Di Marco , C. Lavado , S. Barolin , M. G. Stachiotti

Introducing an isolated intermediate band (IB) into a wide band gap semiconductor can potentially improve the optical absorption of the material beyond the Shockley-Queisser limitation for solar cells. Here, we present a systematic study of…

Materials Science · Physics 2018-05-24 Tingting Wang , Xiaoguang Li , Wenjie Li , Li Huang , Ya Cheng , Jun Cui , Hailin Luo , Guohua Zhong

All inorganic halide perovskites offer promising optoelectronic properties at low cost, but their structural softness and thermal instability limit applications. Density functional theory using the FP-LAPW method (WIEN2k) was used to study…

Materials Science · Physics 2026-04-28 Sikander Azam , Asif Zaman , Qaiser Rafiq , Amin Ur Rahman , Saleem Ayaz Khan

The phenomenon of oxygen incorporation induced superconductivity in iron telluride (Fe1+yTe, with antiferromagnetic (AFM) orders) is intriguing and quite different from the case of FeSe. Until now, the microscopic origin of the induced…

The defect chemistry of perovskite compounds is directly related to the stoichiometry and to the valence states of the transition-metal ions. Defect engineering has become increasingly popular as it offers the possibility to influence the…

Atomic and atom-like defects in the solid-state are widely explored for quantum computers, networks and sensors. Rare earth ions are an attractive class of atomic defects that feature narrow spin and optical transitions that are isolated…

Perovskite-type BiNiO$_3$ is an insulating antiferromagnet in which a charge disproportionation occurs at the Bi site. La substitution for Bi suppresses the charge disproportionation and makes the system metallic. We have measured the…

Strongly Correlated Electrons · Physics 2007-05-23 H. Wadati , M. Takizawa , T. T. Tran , K. Tanaka , T. Mizokawa , A. Fujimori , A. Chikamatsu , H. Kumigashira , M. Oshima , S. Ishiwata , M. Azuma , M. Takano

Electronic structure calculations indicate that the Sr2FeSbO6 double perovskite has a flat-band set just above the Fermi level that includes contributions from ordinary sub-bands with weak kinetic electron hopping plus a flat sub-band that…

Doping is an effective way to tune the property of metal oxides1-5, for achieving functional oxide electronics6-8. Previously we developed a controllable hydrogen doping technology at ambient conditions by use of electron-proton synergistic…

Applied Physics · Physics 2021-03-30 Yuliang Chen , Changlong Hu , Liyan Xie , Xiaoyu Zhou , Bowen Li , Hui Ren , Liang Li , Guobin Zhang , Jun Jiang , Chongwen Zou

In the realm of ferroelectric memories, HfO2-based ferroelectrics stand out because of their exceptional CMOS compatibility and scalability. Nevertheless, their switchable polarization and switching speed are not on par with those of…

In our paper (W\"olfle and Balatsky, Phys. Rev. B 98, 104505 (2018)) we presented a microscopic theory of superconductivity for doped SrTiO$_{3}$ by proposing two pairing mechanisms acting simultaneously with relative strength depending on…

Superconductivity · Physics 2020-01-29 P Wölfle , A V Balatsky

Single crystals of KNbO3 and KNbO3 : Fe have been grown using the flux method at various technological conditions. The investigations of optical absorption of these crystals were carried out. Marked influence of technological conditions and…

Condensed Matter · Physics 2007-05-23 M. Milata , K. Wojcik , K. Zieleniec

In Sr2IrO4 and Sr3Ir2O7, correlations, magnetism and spin-orbit coupling compete on similar energy scales, creating a new context to study metal-insulator transitions (MIT). We use here Angle-Resolved photoemission to investigate the MIT as…

Strongly Correlated Electrons · Physics 2018-12-13 V. Brouet , L. Serrier-Garcia , A. Louat , L. Fruchter , F. Bertran , P. Le Fevre , J. Rault , A Forget , D. Colson

Single-phase perovskite 5 at.% Mn-doped and undoped polycrystalline BaTiO3 thin films have been grown under different oxygen partial pressures by pulsed laser deposition on platinum-coated sapphire substrates. Ferroelectricity is only…

Domain engineering in ferroelectric thin films is crucial for next-generation microelectronic and photonic technologies. Here, a method is demonstrated to precisely control domain configurations in BaTiO$_3$ thin films through low-energy He…

By means of oxide molecular beam epitaxy with shutter-growth mode, we have fabricated a series of electron-doped (Sr1-xLax)2IrO4(001)(x = 0, 0.05, 0.1 and 0.15) single crystalline thin films and then investigated the doping dependence of…

Strongly Correlated Electrons · Physics 2015-04-27 M. Y. Li , Z. T. Liu , H. F. Yang , J. L. Zhao , Q. Yao , C. C. Fan , J. S. Liu , B. Gao , D. W. Shen , X. M. Xie

Recent advances in electrostatic gating provide a novel way to modify the carrier concentration in materials via electrostatic means instead of chemical doping, thus minimizing the impurity scattering. Here, we use first-principles Density…

Materials Science · Physics 2020-05-13 Ezra Day-Roberts , Turan Birol , Rafael M. Fernandes

The efforts in the optimization of the physical and chemical properties related to the photocatalytic efficiency of TiO2 nanoparticles relies mainly on defect engineering strategies, been the structural and the doping the most common ones.…

Materials Science · Physics 2022-03-07 M. P. Ferreira , H. B. de Carvalho

We have analyzed two mechanisms proposed recently for superconductivity in doped SrTiO3 - the plasmon-mediated pairing and the potential of an instantaneous attraction between two electrons that owes its origin to the exchange by…

Superconductivity · Physics 2016-10-10 Lev P. Gor'kov