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We present confocal microscopy studies of novel particle-stabilized emulsions. The novelty arises because the immiscible fluids have an accessible upper critical solution temperature. The emulsions have been created by beginning with…

Soft Condensed Matter · Physics 2009-11-11 P. S. Clegg , E. M. Herzig , A. B. Schofield , T. S. Horozov , B. P. Binks , M. E. Cates , W. C. K. Poon

When a drop laden with solid particles and suspended in a liquid passes through a narrow pore, its interface experiences strong shear and elongation, and the raft of particles may accumulate toward the back of the drop. Using well…

Soft Condensed Matter · Physics 2022-10-19 Franz de Soete , Nicolas Passade-Boupat , Laurence Talini , François Lequeux , Emilie Verneuil

Nano- to micro-sized particles with differently charged surface areas exhibit complex interaction patterns, characterized by both opposite-charge attraction and like-charge repulsion. While several successful models have been proposed in…

Soft Condensed Matter · Physics 2025-01-16 Daniele Notarmuzi , Silvano Ferrari , Emanuele Locatelli , Emanuela Bianchi

We study the behavior of negatively charged colloids with two positively charged polar caps close to a planar patterned surface. The competition between the different anisotropic components of the particle-particle interaction patterns is…

Soft Condensed Matter · Physics 2018-09-25 Emanuele Locatelli , Emanuela Bianchi

The electrostatic interaction between two non-identical, moderately charged colloids situated in close proximity of each other at a fluid interface is studied. By resorting to a well-justified model system, this problem is analytically…

Soft Condensed Matter · Physics 2018-04-30 Arghya Majee , Timo Schmetzer , Markus Bier

We present an approach to electronic polarization in molecular solids treated as a set of quantum systems interacting classically. Individual molecules are dealt with rigorously as quantum-mechanical systems subject to classical external…

Condensed Matter · Physics 2009-11-07 E. V. Tsiper , Z. G. Soos

We use a reactive Monte Carlo simulation method and primitive model of electrolyte to study acid-base equilibrium that controls charge regulation in colloidal systems. The simulations are performed in a semi-grand canonical ensemble in…

Soft Condensed Matter · Physics 2021-12-21 Amin Bakhshandeh , Derek Frydel , Yan Levin

We investigate percolation in binary and ternary mixtures of patchy colloidal particles theoretically and using Monte Carlo simulations. Each particle has three identical patches, with distinct species having different types of patch.…

Soft Condensed Matter · Physics 2016-09-21 Felix Seiferling , Daniel de las Heras , Margarida M. Telo da Gama

When polyelectrolyte-neutral block copolymers are mixed in solutions to oppositely charged species (e.g. surfactant micelles, macromolecules, proteins etc), there is the formation of stable supermicellar aggregates combining both…

Soft Condensed Matter · Physics 2007-05-23 J. -F. Berret , K. Yokota , M. Morvan

Inverse patchy colloids are nano- to micro-scale particles with a surface divided into differently charged regions. This class of colloids combines directional, selective bonding with a relatively simple particle design: owing to the…

Soft Condensed Matter · Physics 2021-01-22 Emanuela Bianchi , Peter D. J. van Oostrum , Christos N. Likos , Gerhard Kahl

We simulate colloids (radius $R \sim 1\mu$m) trapped at the interface between a cholesteric liquid crystal and an immiscible oil, at which the helical order (pitch p) in the bulk conflicts with the orientation induced at the interface,…

Soft Condensed Matter · Physics 2013-11-11 J. S. Lintuvuori , A. C. Pawsey , K. Stratford , M. E. Cates , P. S. Clegg , D. Marenduzzo

Variational methods are used to calculate structural and thermodynamical properties of a titrating polyelectrolyte in a discrete representation. The Coulomb interactions are emulated by harmonic repulsive forces, the force constants being…

chem-ph · Physics 2008-02-03 B. Jönsson , M. Ullner , C. Peterson , O. Sommelius , B. Söderberg

We demonstrate that the formation of bicontinuous emulsions stabilized by interfacial particles (bijels) is more robust when nanoparticles rather than microparticles are used. Emulsification via spinodal demixing in the presence of nearly…

Soft Condensed Matter · Physics 2015-09-30 M. Reeves , A. T. Brown , A. B. Schofield , M. E. Cates , J. H. J. Thijssen

We simulate structural phase behavior of polymer-grafted colloidal particles by molecular Monte Carlo technique. Interparticle potential, which has a finite repulsive square-step outside a rigid core of the colloid, was previously confirmed…

Soft Condensed Matter · Physics 2015-03-19 Yuki Norizoe , Toshihiro Kawakatsu

We present a study on buckling of colloidal particles, including experimental, theoretical and numerical developments. Oil-filled thin shells prepared by emulsion templating show buckling in mixtures of water and ethanol, due to dissolution…

Soft Condensed Matter · Physics 2009-05-14 Catherine Quilliet , Carmen Zoldesi , Christophe Riera , Alfons Van Blaaderen , Arnout Imhof

We study segregation of a binary mixture of similarly charged particles under shear using particle-based simulations. We simulate particle dynamics using a discrete-element model including electrostatic interactions and find that particles…

Computational Physics · Physics 2017-05-12 R. Yoshimatsu , N. A. M. Araújo , T. Shinbrot , H. J. Herrmann

In order to control aggregation phenomena in suspensions of nanoparticles, one often charges the particles electrically, e.g. by triboelectric charging. Stabilization of suspensions against aggregation of particles is an important issue,…

General Physics · Physics 2007-05-23 J. H. Werth , S. M. Dammer , H. A. Knudsen , H. Hinrichsen , D. E. Wolf

Electrostatic interactions play an important role in numerous self-assembly phenomena, including colloidal aggregation. Although colloids typically have a dielectric constant that differs from the surrounding solvent, the effective…

Soft Condensed Matter · Physics 2018-09-17 Kipton Barros , Erik Luijten

We study the kinetics of the liquid-to-crystal transformation and of gel formation in colloidal suspensions of oppositely charged particles. We analyse, by means of both computer simulations and experiments, the evolution of a fluid…

Equilibrium gels of colloidal particles can be realized through the introduction of a second species, a linker that mediates the bonds between the colloids. A gel forming binary mixture whose linkers can self-assemble into linear chains…

Soft Condensed Matter · Physics 2022-11-09 M. Gouveia , C. S. Dias , J. M. Tavares