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We investigate nonlinear optical absorption in diamond crystals containing high densities of nitrogen vacancy (NV) centers using open-aperture Z-scan measurements with 230 fs laser pulses at 1032 nm, within the transparency window of…

We survey the Si K edge structure in various absorbed Galactic low-mass X-ray binaries (LMXBs) to study states of silicon in the inter- and circum-stellar medium. The bulk of these LMXBs lie toward the Galactic bulge region and all have…

Astrophysics of Galaxies · Physics 2016-08-17 Norbert S. Schulz , Lia Corrales , Claude R. Canizares

Although diamond photonics has driven considerable interest and useful applications, as shown in frequency generation devices and single photon emitters, fundamental studies on the third-order optical nonlinearities of diamond are still…

We introduce a real-space approach to understand the relationship between optical absorption and crystal structure. We apply this approach to alternative phases of silicon, with a focus on the Si$_{20}$ crystal phase as a case study. We…

Materials Science · Physics 2018-01-08 Chin Shen Ong , Sinisa Coh , Marvin L. Cohen , Steven G. Louie

In this paper, we analyse the optical absorption in porous silicon . This is the first attempt to explicitly demonstrate that it is not possible to extract the band gap of such low dimensional nanostructures like porous silicon from a Tauc…

Soft Condensed Matter · Physics 2007-05-23 Shouvik Datta , K. L. Narasimhan

To achieve atomic-level characterization of the diamond (001) surface, persistent efforts have been made over the past few decades. The motivation behind the pursuit extends beyond investigating surface defects and adsorbates; it also…

Soft x-rays were applied to induce graphitization of diamond through a non-thermal solid-to-solid phase transition. This process was observed within poly-crystalline diamond with a time-resolved experiment using ultrashort soft x-ray pulses…

We compare energy spectra, electron localization and optical absorption of square and diamond quantum rings and analyze how sample geometry affects those features. We show that low energy levels of diamond rings form two groups delocalized…

Mesoscale and Nanoscale Physics · Physics 2015-09-07 Anna Sitek , Vidar Gudmundsson , Andrei Manolescu

We show an experimental evidence of the domination of absorption over scattering in absorbance spectra of detonation nanodiamonds. We perform the absorbance measurements on the UV-Vis spectrophotometer equipped with integrating sphere and…

Mesoscale and Nanoscale Physics · Physics 2020-03-25 S. V. Koniakhin , M. K. Rabchinskii , N. A. Besedina , L. V. Sharonova , A. V. Shvidchenko , E. D. Eidelman

Enabled by x-ray free-electron lasers, nonlinear optical phenomena can be explored in the x-ray domain nowadays. Among the multitude of newly accessible processes, this theoretical study focuses parametric x-ray optical wavemixing for…

Optics · Physics 2021-04-14 Dietrich Krebs , Nina Rohringer

In this paper the authors analyse near-edge absorption of x rays in noncentrosymmetric crystals. The work is motivated by recent observations of x-ray dichroic effects which stems from parity-nonconserving electron interactions. We provide…

Condensed Matter · Physics 2009-11-07 Paolo Carra , Andres Jerez , Ivan Marri

We present a reciprocal-space pseudopotential scheme for calculating X-ray absorption near-edge structure (XANES) spectra. The scheme incorporates a recursive method to compute absorption cross section as a continued fraction. The continued…

Condensed Matter · Physics 2009-11-07 Mathieu Taillefumier , Delphine Cabaret , Anne-Marie Flank , Francesco Mauri

X-ray absorption spectroscopy is a well established tool for obtaining information about orbital and spin degrees of freedom in transition metal- and rare earth-compounds. For this purpose usually the dipole transitions of the L- (2p to 3d)…

Strongly Correlated Electrons · Physics 2014-02-21 P. Hansmann , M. W. Haverkort , A. Toschi , G. Sangiovanni , F. Rodolakis , J. P. Rueff , M. Marsi , K. Held

The refractive index of a y-cut SiO$_2$ crystal surface is reconstructed from polarization dependent soft X-ray reflectometry measurements in the energy range from 45 eV to 620 eV. Due to the anisotropy of the crystal structure in the (100)…

Materials Science · Physics 2021-06-25 A. Andrle , P. Hönicke , J. Vinson , R. Quintanilha , Q. Saadeh , S. Heidenreich , F. Scholze , V. Soltwisch

In this paper, we report on the optical absorption in porous silicon. We model the absorption process assuming that porous silicon is a pseudo 1D material system having a distribution of band gaps. We show that in order to explain the…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Shouvik Datta , K. L. Narasimhan

Diamond materials are central to an increasing range of advanced technological demonstrations, from high power electronics, to nano-scale quantum bio-imaging with unprecedented sensitivity. However, the full exploitation of diamond for…

We investigate theoretically the resonant inelastic x-ray scattering (RIXS) at the $K$ edge of Si on the basis of an ab initio calculation. We calculate the RIXS spectra with systematically varying transfered-momenta, incident-photon energy…

Materials Science · Physics 2007-05-23 Yunori Nisikawa , Manabu Usuda , Jun-ichi Igarashi

Absolute X-ray reflectivity of chemically vapor deposited (CVD) diamond single crystals was measured in the Laue geometry in the double-crystal non-dispersive setting with an asymmetric Si beam conditioner crystal. The measurements were…

Materials Science · Physics 2018-05-22 S. Stoupin , J. P. C. Ruff , T. Krawczyk , K. D. Finkelstein

Results of Small-Angle Scattering study of diamonds with various types of point and extended defects and different degrees of annealing are presented. It is shown that thermal annealing and/or mechanical deformation cause formation of…

Materials Science · Physics 2012-09-11 A A Shiryaev , P Boesecke

We report measured dipolar asymmetry ratios at the LIII edges of the heavy rare earth metals. The results are compared with a first principles calculation and excellent agreement is found. A simple model of the scattering is developed,…

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