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Magnetic properties of a single vacancy in graphene is a relevant and still much discussed problem. The experimental results point to a clearly detectable magnetic defect state at the Fermi energy, while calculations based on density…

Mesoscale and Nanoscale Physics · Physics 2017-10-31 Ana M. Valencia , Marilia J. Caldas

Magnetic properties of a single vacancy in graphene is a relevant and still unsolved problem. The experimental results point to a clearly detectable magnetic defect state at the Fermi energy, while several calculations based on density…

Mesoscale and Nanoscale Physics · Physics 2017-10-11 A. M. Valencia , M. J. Caldas

Vacancy-induced magnetization of a graphene layer is investigated by means of a first principle DFT method. Calculations of the formation energy and the magnetization by creating the different number of vacancies in a supercell show that a…

Mesoscale and Nanoscale Physics · Physics 2019-05-15 E. Nakhmedov , E. Nadimi , S. Vedaei , O. Alekperov , F. Tatardar , A. I. Najafov , I. I. Abbasov , A. M. Saletskii

The correlation between structural distortion and emergence of magnetism in graphene containing a single vacancy was investigated using first-principles calculations based on density functional theory (DFT). Our results have shown that a…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Wendel S. Paz , Wanderlã L. Scopel , Jair C. C. Freitas

Atomic vacancies have a strong impact in the mechanical, electronic and magnetic properties of graphene-like materials. By artificially generating isolated vacancies on a graphite surface and measuring their local density of states on the…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 M. M. Ugeda , I. Brihuega , F. Guinea , J. M. Gomez-Rodriguez

We present an ab initio DFT study of the magnetic moments that arise in graphite by creating single carbon vacancies in a 3-D graphite network, using a full potential, all electron, spin polarized electronic structure calculations. In…

We study the effect of various configurations of vacancies on the magnetic properties of graphene nanoflake (GNF) with screened realistic long-range electron interaction [T. O. Wehling, et. al., Phys. Rev. Lett. 106, 236805 (2011)] within…

Strongly Correlated Electrons · Physics 2023-12-12 V. S. Protsenko , A. A. Katanin

The observation of intrinsic magnetic order in graphene and graphene-based materials relies on the formation of magnetic moments and a sufficiently strong mutual interaction. Vacancies are arguably considered the primary source of magnetic…

Mesoscale and Nanoscale Physics · Physics 2012-06-29 J. J. Palacios , F. Yndurain

Understanding the coupling of graphene with its local environment is critical to be able to integrate it in tomorrow's electronic devices. Here we show how the presence of a metallic substrate affects the properties of an atomically…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 M. M. Ugeda , D. Fernández-Torre , I. Brihuega , P. Pou , A. J. Martínez-Galera , R. Pérez , J. M. Gómez-Rodríguez

We investigate the interactions between two identical magnetic impurities substituted into a graphene superlattice. Using a first-principles approach, we calculate the electronic and magnetic properties for transition-metal substituted…

We address the electronic structure and magnetic properties of vacancies and voids both in graphene and graphene ribbons. Using a mean field Hubbard model, we study the appearance of magnetic textures associated to removing a single atom…

Mesoscale and Nanoscale Physics · Physics 2008-11-27 J. J. Palacios , J. Fernandez-Rossier , L. Brey

With quantum Monte Carlo methods, we investigate the consequences of placing a magnetic adatom adjacent to a vacancy in a graphene sheet. We find that instead of the adatom properties depending on the energy of the adatom orbital, as in a…

Strongly Correlated Electrons · Physics 2012-03-29 F. M. Hu , J. E. Gubernatis , Hai-Qing Lin , Yan-Chao Li , R. M. Nieminen

Carbon atom vacancies in graphene give rise to a local magnetic moment of $\sigma+\pi$ origin, whose magnitude is yet uncertain and debated. Partial quenching of $\pi$ magnetism has been ubiquitously reported in periodic $first-principles$…

Materials Science · Physics 2023-02-27 Mirko Leccese , Rocco Martinazzo

Using density functional calculations we have investigated the local spin moment formation and lattice deformation in graphene when an isolated vacancy is created. We predict two competing equilibrium structures: a ground state planar…

Materials Science · Physics 2016-05-13 Haricharan Padmanabhan , B. R. K. Nanda

Using the tight-binding model, we investigate the influence of vacancy disorder on electrical transport in graphene Hall bars in the presence of quantizing magnetic fields. Disorder, induced by a random distribution of monovacancies, breaks…

Mesoscale and Nanoscale Physics · Physics 2016-12-21 M. D. Petrović , F. M. Peeters

The electronic structure, bonding and magnetism in graphene containing vacancies are studied using density-functional methods. The single-vacancy graphene ground state is spin polarized and structurally flat. The unpolarized state is non…

Mesoscale and Nanoscale Physics · Physics 2008-07-11 M. W. C. Dharma-wardana , Marek Z. Zgierski

Vacancy-induced magnetism in graphene bilayers is investigated using spin-polarized density functional theory calculations. One of two graphene layers has a monovacancy. Two atomic configurations for bilayers are considered with respect to…

Other Condensed Matter · Physics 2009-11-13 Sangkook Choi , Byoung Wook Jeong , Seungchul Kim , Gunn Kim

The indirect exchange interaction between magnetic impurities localized in a graphene plane is considered theoretically, with the influence of intrinsic spin-orbit interaction taken into account. Such an interaction gives rise to an energy…

Materials Science · Physics 2015-06-25 V. K. Dugaev , V. I. Litvinov , J. Barnas

Motivated by recent studies reporting the formation of localized magnetic moments in doped graphene, we investigate the energetic cost for spin polarizing isolated impurities embedded in this material. When a well-known criterion for the…

Materials Science · Physics 2015-05-14 P. Venezuela , R. B. Muniz , A. T. Costa , D. M. Edwards , S. R. Power , M. S. Ferreira

We employ the Green's function technique to investigate the vacancy-induced quasi-localized magnetic moment formation in mono-layer graphene starting with the Dirac Hamiltonian, which focuses on the {\pi}- orbitals only, involving the…

Mesoscale and Nanoscale Physics · Physics 2012-05-08 Partha Goswami , Ajay Pratap Singh Gahlot
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