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Hyperfine interactions, magnetic interactions between the spins of electrons and nuclei, in graphene and related carbon nanostructures are studied. By using a combination of accurate first principles calculations on graphene fragments and…

Materials Science · Physics 2008-04-09 Oleg V. Yazyev

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

An interacting spin system is an excellent testbed for fundamental quantum physics and applications in quantum sensing and quantum simulation. For these investigations, detailed information of the interactions, e.g., the number of spins and…

Quantum Physics · Physics 2024-11-12 Yuhang Ren , Susumu Takahashi

Precise characterization of a hyperfine interaction is a prerequisite for high fidelity manipulations of electron and nuclear spins belonging to a hybrid qubit register in diamond. Here, we demonstrate a novel scheme for determining a…

Quantum Physics · Physics 2013-09-11 J. H. Shim , B. Nowak , I. Niemeyer , J. Zhang , F. D. Brandao , D. Suter

The interaction of solid-state electronic spins with deformations of their host crystal is an important ingredient in many experiments realizing quantum information processing schemes. Here, we theoretically characterize that interaction…

Mesoscale and Nanoscale Physics · Physics 2018-08-08 Péter Udvarhelyi , Vladyslav O. Shkolnikov , Adam Gali , Guido Burkard , András Pályi

We experimentally demonstrate an approach to scale up quantum devices by harnessing spin defects in the environment of a quantum probe. We follow this approach to identify, locate, and control two electron-nuclear spin defects in the…

Quantum Physics · Physics 2020-03-04 Alexandre Cooper , Won Kyu Calvin Sun , Jean-Christophe Jaskula , Paola Cappellaro

Magnetic Resonance Imaging (MRI) can characterize and discriminate among tissues using their diverse physical and biochemical properties. Unfortunately, submicrometer screening of biological specimens is presently not possible, mainly due…

Mesoscale and Nanoscale Physics · Physics 2010-11-03 C. A. Meriles , L. Jiang , G. Goldstein , J. S. Hodges , J. R. Maze , M. D. Lukin , P. Cappellaro

Nuclear spins with hyperfine coupling to single electron spins are highly valuable quantum bits. In this work we probe and characterise the particularly rich nuclear spin environment around single silicon vacancy color-centers (V2) in…

For decades, searches for exotic spin interactions have used increasingly-precise laboratory measurements to test various theoretical models of particle physics. However, most searches have focused on interaction length scales greater than…

Quantum Physics · Physics 2022-07-04 P. -H. Chu , N. Ristoff , J. Smits , N. Jackson , Y. J. Kim , I. Savukov , V. M. Acosta

Nuclear spins are among the potential candidates prospected for quantum information technology. A recent breakthrough enabled to atomically resolve their interaction with the electron spin, the so-called hyperfine interaction, within…

Mesoscale and Nanoscale Physics · Physics 2021-06-09 Sufyan Shehada , Manuel dos Santos Dias , Filipe Souza Mendes Guimarães , Muayad Abusaa , Samir Lounis

We describe how to prepare an electrically levitated nanodiamond in a superposition of orientations via microwave driving of a single embedded nitrogen-vacancy (NV) center. Suitably aligning the magnetic field with the NV center can serve…

Nanodiamonds containing nitrogen vacancy (NV-) centers show promise for a number of emerging applications including targeted in vivo imaging and generating nuclear spin hyperpolarization for enhanced NMR spectroscopy and imaging. Here, we…

We propose a scheme to achieve nuclear-nuclear indirect interactions mediated by a mechanically driven nitrogen-vacancy (NV) center in diamond. Here we demonstrate two-qubit entangling gates and quantum-state transfer between two carbon…

Quantum Physics · Physics 2022-11-18 Wan-Jun Su , Guang-Zheng Ye , Ya-Dong Wu , Zhen-Biao Yang , Barry C. Sanders

Mapping the positions of single electron spins is a highly desired capability for applications such as nanoscale magnetic resonance imaging and quantum network characterization. Here, we demonstrate a method based on rotating an external…

Mesoscale and Nanoscale Physics · Physics 2022-11-11 Dan Yudilevich , Rainer Stöhr , Andrej Denisenko , Amit Finkler

Precise knowledge of a quantum system's Hamiltonian is a critical pre-requisite for its use in many quantum information technologies. Here, we report a method for the precise characterization of the non-secular part of the excited-state…

Quantum Physics · Physics 2017-06-20 F. Poggiali , P. Cappellaro , N. Fabbri

We present a protocol that detects molecular conformational changes with two nitroxide electron-spin labels and a nitrogen-vacancy (NV) center in diamond. More specifically, we demonstrate that the NV can detect energy shifts induced by the…

Quantum Physics · Physics 2022-12-21 C. Munuera-Javaloy , R. Puebla , B. D'Anjou , M. B. Plenio , J. Casanova

Quantum sensors have attracted broad interest in the quest towards sub-micronscale NMR spectroscopy. Such sensors predominantly operate at low magnetic fields. Instead, however, for high resolution spectroscopy, the high-field regime is…

The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Hai-Jing Wang , Chang S. Shin , Scott J. Seltzer , Claudia E. Avalos , Alexander Pines , Vikram S. Bajaj

Mechanical resonators operating in the high-frequency regime have become a versatile platform for fundamental and applied quantum research. Their exceptional properties, such as low mass and high quality factor, make them also very…

Mesoscale and Nanoscale Physics · Physics 2023-11-29 Diego A. Visani , Letizia Catalini , Christian L. Degen , Alexander Eichler , Javier del Pino

Nuclear spins of dopant atoms in semiconductors are promising candidates as quantum bits, due to the long lifetime of their quantum states. Conventionally, coherent control of nuclear spins is done using ac magnetic fields. Using the…

Mesoscale and Nanoscale Physics · Physics 2018-06-27 Péter Boross , Gábor Széchenyi , András Pályi