Related papers: Observation of mixed singlet-triplet Rb$_2$ Rydber…
Highly excited Rydberg atoms inherit their level structure, symmetries, and scaling behavior from the hydrogen atom. We demonstrate that these fundamental properties enable a thermodynamic limit of a single Rydberg atom subjected to…
Ultracold atoms are increasingly used for high precision experiments that can be utilized to extract accurate scattering properties. This calls for a stronger need to improve on the accuracy of interatomic potentials, and in particular the…
By applying a circularly polarized and slightly blue-detuned microwave field with respect to the first excited rotational state of a dipolar molecule, one can engineer a long-range, shallow potential well in the entrance channel of the two…
A Rydberg and a ground-state atom can form ultralong range diatomic molecules provided the interaction between the ground-state atom and the Rydberg electron is attractive [C. H. Greene, et al., Phys. Rev. Lett. 85, 2458 (2000)]. A…
We perform two-photon photoassociation spectroscopy of the heteronuclear CsYb molecule to measure the binding energies of near-threshold vibrational levels of the $X~^{2}\Sigma_{1/2}^{+}$ molecular ground state. We report results for…
We demonstrate that through localised Rydberg excitation in a three-dimensional cold atom cloud atomic motion can be rendered directed and nearly confined to a plane, without spatial constraints for the motion of individual atoms. This…
Atom-atom interactions within a small volume were investigated through the excitation of ultracold Rb atoms. The application of microwaves enhances these interactions, causing the suppression of Rydberg state excitation. The suppression of…
We investigate the interactions between ultracold alkali metal atoms and closed-shell atoms using electronic structure calculations on the prototype system Rb+Sr. There are molecular bound states that can be tuned across atomic thresholds…
Ultracold metastable RbCs molecules are observed in a double species MOT through photoassociation near the Rb(5S$_{1/2}$)+Cs(6P$_{3/2}$) dissociation limit followed by radiative stabilization. The molecules are formed in their lowest…
We examine spectral signatures of Rydberg atoms driven with near-resonant dual-tone radio-frequency (RF) fields in the regime of strong driving. We experimentally demonstrate and theoretically model a variety of nonlinear and multiphoton…
We study the possibility to use interaction between a polar molecule in the ground electronic and vibrational state and a Rydberg atom to construct two-qubit gates between molecular qubits and to coherently control molecular states. A polar…
Starting from weakly bound Feshbach molecules, we demonstrate a two-photon pathway to the dipolar ground state of bi-alkali molecules that involves only singlet-to-singlet optical transitions. This pathway eliminates the search for a…
Complete sticking at low incidence energies and broad angular scattering distributions at higher energies are often observed in molecular beam experiments on gas-surface systems which feature a deep chemisorption well and lack early…
We consider non-adiabatic coupling in the "trilobite"-like long-range Rydberg molecules created by perturbing degenerate high-$\ell$ Rydberg states with a ground-state atom. Due to the flexibility granted by the high Rydberg level density,…
We report on the observation of interactions between ultracold Rydberg atoms and ions in a Paul trap. The rate of observed inelastic collisions, which manifest themselves as charge transfer between the Rydberg atoms and ions, exceeds that…
We propose a novel type of Rydberg dimer, consisting of a Rydberg-state atom bound to a distant positive ion. The molecule is formed through long-range electric-multipole interaction between the Rydberg atom and the point-like ion. We…
Non-radiative energy transfer between a Rydberg atom and a polar molecule can be controlled by a DC electric field. Here we show how to exploit this control for state-resolved, non-destructive detection and spectroscopy of the molecules…
We investigate the possibility of forming deeply bound ultracold RbCs molecules by a two-color photoassociation experiment. We compare the results with those for Rb_2 in order to understand the characteristic differences between…
Atoms confined in optical tweezer arrays constitute a platform for the implementation of quantum computers and simulators. State-dependent operations are realized by exploiting electrostatic dipolar interactions that emerge, when two atoms…
We theoretically investigate the manipulation of the motional states of trapped ground-state atoms using Rydberg dressing via nonresonant laser fields. The forces resulting from Rydberg-state interaction between dressed neighboring atoms in…