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Detecting the internal state of polar molecules is a substantial challenge when standard techniques such as resonance-enhanced multi photon ionization (REMPI) or laser-induced fluorescense (LIF) do not work. As this is the case for most…

Atomic Physics · Physics 2014-12-01 Rosa Glöckner , Alexander Prehn , Gerhard Rempe , Martin Zeppenfeld

We develop the recently proposed analytical R-matrix (ARM) method to encompass strong field ionisation by circularly polarised fields, for atoms with arbitrary binding potentials. Through ARM, the effect of the potential can now be included…

Atomic Physics · Physics 2013-08-05 Jivesh Kaushal , Olga Smirnova

Numerical attoclock is a theoretical model of attosecond angular streaking driven by a very short, nearly a single oscillation, circularly polarized laser pulse. The reading of such an attoclock is readily obtained from a numerical solution…

Atomic Physics · Physics 2019-07-03 Vladislav V. Serov , Alexander W. Bray , Anatoli S. Kheifets

Electrons carrying orbital angular momentum (OAM) have recently been discovered theoretically and obtained experimentally that opens up possibilities for using them in high-energy physics. We consider such a twisted electron moving in…

High Energy Physics - Phenomenology · Physics 2012-12-12 Dmitry V. Karlovets

We present a quantum optics-based detection method for determining the position and current of an electron beam. As electrons pass through a dilute vapor of rubidium atoms, their magnetic field perturb the atomic spin's quantum state and…

We present an analysis of two experimental approaches to controlling the directionality of molecular rotation with ultrashort laser pulses. The two methods are based on the molecular interaction with either a pair of pulses (a "double kick"…

Optics · Physics 2015-06-11 C. Bloomquist , S. Zhdanovich , A. A. Milner , V. Milner

We present a numerical method for investigating the non-perturbative quantum mechanical interaction of light with atoms in two dimensions, without a basis expansion. This enables us to investigate intense laser-atom interactions with light…

Quantum Physics · Physics 2009-10-30 M. Protopapas , D. G. Lappas , P. L. Knight

We report on non-sequential double ionization of Ar by a laser pulse consisting of two counter rotating circularly polarized fields (390 nm and 780 nm). The double ionization probability depends strongly on the relative intensity of the two…

We study ionization of atoms in strong elliptically-polarized laser fields. We focus on the physical origin of the offset angle in the photoelectron momentum distribution and its possible relation to a specific time. By developing a model…

Atomic Physics · Physics 2022-12-12 Y. G. Peng , J. Y. Che , C. Chen , G. G. Xin , Y. J. Chen

Strong-field ionization by counter-rotating two-color laser fields produces quantum interference between photoelectrons emitted on the leading and trailing edges of the laser field oscillations. We show that in chiral molecules, this…

We explore the laser-induced ionization dynamics of N2 and CO2 molecules subjected to a few-cycle, linearly polarized, 800\,nm laser pulse using effective two-dimensional single active electron time-dependent quantum simulations. We show…

Atomic Physics · Physics 2012-10-02 Michel Peters , Tung Nguyen-Dang , Eric Charron , Arne Keller , Osman Atabek

The Doppler effect of moving atoms can create irreversibility of light. We show that the laser field in electromagnetic induced transparency (EIT) scheme with atomic motion can control the directional propagation of two counter-propagating…

Quantum Physics · Physics 2008-07-23 C. H. Raymond Ooi

We perform ab initio calculations for the hydrogen atom initially in one of the six circular bound states with the principal quantum numbers n = 2, 3 and 4, irradiated by a short circularly polarized laser pulse of 400 nm. The field…

Atomic Physics · Physics 2020-07-01 Jarosław H. Bauer , Zbigniew Walczak

The transition between two distinct mechanisms for the laser-induced field-free orientation of CO molecules is observed via measurements of orientation revival times and subsequent comparison to theoretical calculations. In the first…

Chirality causes symmetry breaks in a large variety of natural phenomena ranging from particle physics to biochemistry. We investigate one of the simplest conceivable chiral systems, a laser-excited, oriented, effective one-electron Li…

Orientation states of two coupled polar molecules controlled by laser pulses are studied theoretically. By varying the period of a series of periodically applied laser pulse, transition from regular to chaotic behavior may occur. Schmidt…

Quantum Physics · Physics 2007-05-23 Ying-Yen Liao , Yueh-Nan Chen , Der-San Chuu

We analize theoretically the dynamics of N electrons localized in a semiconductor quantum ring under a train of phase-locked infrared laser pulses. The pulse sequence is designed to control the total angular momentum of the electrons. The…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Yuriy V Pershin , Carlo Piermarocchi

We present an experiment investigating the rotational Doppler effect using a single trapped ion excited by two copropagating vortex laser beams. The setup isolates the azimuthal gradients of the fields, eliminating longitudinal and…

We consider few-photon ionization of atomic lithium by linearly polarized femtosecond laser pulses, and demonstrate that asymmetries of the electron angular distribution can occur for initially polarized (2p, m=+1) target atoms. The…

We use the $R$-matrix with time-dependence method to study detachment from F$^-$ in circularly-polarized laser fields of infrared wavelength. By decomposing the photoelectron momentum distribution into separate contributions from detached…

Atomic Physics · Physics 2019-11-04 G. S. J. Armstrong , D. D. A. Clarke , A. C. Brown , H. W. van der Hart