Related papers: Quantum-beat Auger spectroscopy
We begin with the theoretical study of spectral energy cascade due to the propagation of high amplitude sound in the absence of thermal sources. To this end, a first-principles-based system of governing equations, correct up to second order…
Quantum interferometry methods exploit quantum resources, such as photonic entanglement, to enhance phase estimation beyond classical limits. Nonlinear optics has served as a workhorse for the generation of entangled photon pairs, ensuring…
Spectroscopy is an important tool for probing the properties of materials, chemicals and biological samples. We design a practical transmitter-receiver system that exploits entanglement to achieve a provable quantum advantage over all…
We investigate quantum phase transitions, quantum criticality, and Berry phase for the ground state of an ensemble of non-interacting two-level atoms embedded in a non-linear optical medium, coupled to a single-mode quantized…
Besides their stunning physical properties which are unmatched in a classical world, squeezed states of electromagnetic radiation bear advanced application potentials in quantum information systems and precision metrology, including…
The modulational instability of broadband optical pulses in a four-state atomic system is investigated. In particular, starting from a recently derived generalized nonlinear Schr\"odinger equation, a wave-kinetic equation is derived. A…
Ultrafast optical pump-probe spectroscopy is a powerful tool to study dynamics in solid materials on femto- and picosecond timescales. In such experiments, a pump pulse induces dynamics inside a sample by impulsive light-matter interaction,…
We study the nonlinear spectra and multi-photon correlation functions for the waveguide output of a two-level system (including realistic dissipation channels) with a time-delayed coherent feedback. We compute these observables by extending…
We experimentally demonstrate a nonlinear detection scheme exploiting time-reversal dynamics that disentangles continuous variable entangled states for feasible readout. Spin-exchange dynamics of Bose-Einstein condensates is used as the…
Control over the joint spectral amplitude of a photon pair has proved highly desirable for many quantum applications, since it contains the spectral quantum correlations, and has crucial effects on the indistinguishability of photons, as…
Quantum machine learning has emerged as a promising tool for pattern recognition, yet many audio-focused approaches still treat spectrograms as generic images and do not explicitly exploit their time-frequency structure. We propose Q-Patch,…
Frequency conversion of non-classical light enables robust encoding of quantum information based upon spectral multiplexing that is particularly well-suited to integrated-optics platforms. Here we present an intrinsically deterministic…
We introduce the concept of a quantum pulse gate (QPG), a method for accessing the intrinsic broadband spectral mode structure of ultrafast quantum states of light. This mode structure can now be harnessed for applications in quantum…
We demonstrate the simultaneous estimation of signal frequency and amplitude by a single quantum sensor in a single experimental shot. Sweeping the qubit splitting linearly across a span of frequencies induces a non-adiabatic Landau-Zener…
We have studied theoretically the basic operation of a quantum feedback loop designed to maintain the desired phase of quantum coherent oscillations in a two-level system. Such feedback can suppress the dephasing of oscillations due to…
A quantum coherent capacitor subject to large amplitude pulse cycles can be made to emit or reabsorb an electron in each half cycle. Quantized currents with pulse cycles in the GHz range have been demonstrated experimentally. We develop a…
A one-dimensional system with two $\delta$-like barriers or wells bi-chromaticaly oscillating at frequencies $\omega$ and $2\omega$ is considered. The alternating signal leads to the direct current across the structure (even in a symmetric…
Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…
We consider the continuous-time version of our recently proposed quantum theory of optical temporal phase and instantaneous frequency [Tsang, Shapiro, and Lloyd, Phys. Rev. A 78, 053820 (2008)]. Using a state-variable approach to…
Optical pump-probe spectroscopy is a powerful tool to directly probe the carrier dynamics in materials down to sub-femtosecond resolution. To perform such measurement, while keeping the pump induced perturbation to the sample as small as…