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Enhanced optical absorption of molecules in the vicinity of metallic nanostructures is key to a number of surface-enhanced spectroscopies and of great general interest to the fields of plasmonics and nano-optics. Yet, experimental access to…

We point out a novel manifestation of many-body correlations in the linear optical response of electrons confined in a quantum well. Namely, we demonstrate that along with conventional absorption peak at frequency close to intersubband…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Dai , M. E. Raikh , T. V. Shahbazyan

We investigate an efficient two-photon up-conversion process in more than one molecule coupled to an optical antenna. In the previous work [Y. Osaka et al., PRL 112, 133601 (2014)], we considered the two-photon up-conversion process in a…

Optics · Physics 2016-05-04 Yoshiki Osaka , Nobuhiko Yokoshi , Hajime Ishihara

Surface lattice resonance supported on plasmonic nanoparticle arrays enhances light-matter interactions for applications such as photoluminescence enhancement. The photoluminescence process is enhanced through confining light beyond the…

Optics · Physics 2024-06-14 Joshua T. Y. Tse , Shunsuke Murai , Katsuhisa Tanaka

We present a theoretical study of the dispersion relation of surface plasmon resonances of mesoscopic metal-dielectric-metal microspheres. By analyzing the solutions to Maxwell's equations, we obtain a simple geometric condition for which…

Optics · Physics 2009-11-11 Keisuke Hasegawa , Charles A. Rohde , Miriam Deutsch

Absorption induced transparency is an optical phenomenon that occurs in metallic arrays of nanoholes when materials featuring narrow lines in their absorption spectra are deposited on top of it. First reported in the visible range, using…

Optics · Physics 2021-09-22 Sergio G Rodrigo

The infrared range optical absorption mechanism of Carbon-Copper composite thin layer coated on the Diamond-Like Carbon (DLC) buffer layer has been investigated. By consideration of weak interactions between copper nanoparticles in their…

In this paper, optical and electronic properties of diamond shaped graphene quantum dots (DQDs) have been studied by employing large-scale electron-correlated calculations. The computations have been performed using the \pi-electron…

Mesoscale and Nanoscale Physics · Physics 2015-11-16 Tista Basak , Himanshu Chakraborty , Alok Shukla

Strong field photoemission and electron recollision provide a viable route to extract electronic and nuclear dynamics from molecular targets with attosecond temporal resolution. However, since an {\em ab-initio} treatment of even the…

Atomic Physics · Physics 2016-11-02 N. Suárez , A. Chacón , M. F. Ciappina , B. Wolter , J. Biegert , M. Lewenstein

We study the impact of an environment on the electromagnetic responses of a molecule in the presence of a dielectric medium. By applying the dipole-dipole coupling between the molecule's and the environment's degrees of freedom, we can…

Quantum Physics · Physics 2022-11-04 Johannes Fiedler , Kristian Berland , Stefan Yoshi Buhmann

Spontaneous emission of quantum emitters can be modified by engineering their optical environment. This allows a resonant nanoantenna to significantly modify the radiative properties of a quantum emitter. In this article, we go beyond the…

The physics of collective optical response of molecular assemblies, pioneered by Dicke in 1954, has long been at the center of theoretical and experimental scrutiny. The influence of the environment on such phenomena is also of great…

We study how the radiative properties of a dense ensemble of atoms can be modified when they are placed near or between metallic or dielectric surfaces. If the average separation between the atoms is comparable or smaller than the…

Quantum Physics · Physics 2018-06-06 Ryan Jones , Jemma A. Needham , Igor Lesanovsky , Francesco Intravaia , Beatriz Olmos

Codeposition of two molecular species [CuPc (donor) and PFP (acceptor)] on noble metal (111) surfaces leads to the self-assembly of an ordered mixed layer with maximized donor-acceptor contact area. The main driving force behind this…

It is well known that plasmons in bulk metals cannot be excited by direct photoabsorption, that is, by coupling of volume plasmons to light. Here we demonstrate that the situation in nanoclusters of the same metals is entirely different. We…

Atomic and Molecular Clusters · Physics 2009-04-21 Chunlei Xia , Chunrong Yin , Vitaly V. Kresin

We investigate the process of photon absorption by atoms or molecules shortly interacting with a laser beam in the dipole approximation. Assuming that the interaction time $\tau$ is much smaller than the lifetime of the corresponding…

We predict and experimentally demonstrate a new type of collective (cooperative) coupling effect where a disordered atomic ensemble absorbs light with a rise-time longer (i. e., at a rate slower) than what is dictated by single-atom…

Quantum Physics · Physics 2025-11-18 D. C. Gold , U. Saglam , S. Carpenter , A. Yadav , M. Beede , T. G. Walker , M. Saffman , D. D. Yavuz

We attempt to provide physical interpretations of light-induced desorption phenomena that have recently been observed for alkali atoms on glass surfaces of alkali vapor cells used in atomic physics experiments. We find that the observed…

Other Condensed Matter · Physics 2007-05-23 Atsushi Hatakeyama , Markus Wilde , Katsuyuki Fukutani

We study the core hole-electron correlation in coherently coupled molecules by energy dispersive near edge X-ray absorption fine-structure spectroscopy. In a transient phase, which exists during the transition between two bulk arrangements,…

Materials Science · Physics 2013-12-03 M. Scholz , F. Holch , C. Sauer , M. Wiessner , A. Schöll , F. Reinert

We study light absorption by a dipolar absorber in a given environment, which can be a nanoantenna or any complex inhomogeneous medium. From first-principle calculations, we derive an upper bound for the absorption, which decouples the…

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