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The dispersive magnetic excitations in Sr2IrO4 have previously been well described within an isospin-1/2 Heisenberg model on a square lattice that revealed parallels with La2CuO4. Here we investigate the inelastic spectra of Sr2Ir0.8Ru0.2O4…

Strongly Correlated Electrons · Physics 2017-01-04 S. Calder , J. W. Kim , A. E. Taylor , M. H. Upton , D. Casa , Guixin Cao , M. D. Lumsden , A. D. Christianson

We put forward a scheme to study the anisotropic magnetic couplings in Sr2IrO4 by mapping fully relativistic constrained noncollinear density functional theory including an on-site Hubbard U correction onto a general spin model Hamiltonian.…

Spin-orbit entangled magnetic dipoles, often referred to as pseudospins, provide a new avenue to explore novel magnetism inconceivable in the weak spin-orbit coupling limit, but the nature of their low-energy interactions remains to be…

The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

We analyze the spin anisotropy of the magnetic susceptibility of Sr$_2$RuO$4$ in presence of spin-orbit coupling and anisotropic strain using quasi-two-dimensional tight-binding parametrization fitted to the ARPES results. Similar to the…

Superconductivity · Physics 2016-12-15 Sergio Cobo , Felix Ahn , Ilya Eremin , Alireza Akbari

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

Strongly Correlated Electrons · Physics 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

Strongly Correlated Electrons · Physics 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

Temperature dependent Raman scattering measurements have been performed to explore unusual coupling between magnetism and crystal structure in doped pyrochlore iridate Y$_2$(Ir$_{1-x}$Ru$_x$)$_2$O$_7$ with $x$ = 0.0, 0.05 and 0.2. The…

Strongly Correlated Electrons · Physics 2019-02-20 Harish Kumar , V. G. Sathe , A. K. Pramanik

The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The…

Strongly Correlated Electrons · Physics 2019-04-23 Kousik Samanta , Danilo Rigitano , Pascoal Jose Giglio Pagliuso , Eduardo Granado

The anisotropy of the magnetic incommensurate fluctuations in Sr2RuO4 has been studied by inelastic neutron scattering with polarized neutrons. We find a sizeable enhancement of the out of plane component by a factor of two for intermediate…

Strongly Correlated Electrons · Physics 2009-11-10 M. Braden , P. Steffens , Y. Sidis , J. Kulda , S. Hayden , N. Kikugawa , Y. Maeno

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

Strongly Correlated Electrons · Physics 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

We study the magnetic excitations in 5d transition-metal oxide Sr$_2$IrO$_4$ on the basis of the Heisenberg model with small anisotropic terms on a square lattice. We calculate the correlation functions by using the Green's functions in the…

Strongly Correlated Electrons · Physics 2015-06-18 Jun-ichi Igarashi , Tatsuya Nagao

We report neutron scattering experiments which reveal a large spin gap in the magnetic excitation spectrum of weakly-monoclinic double perovskite Sr2ScOsO6. The spin gap is demonstrative of appreciable spin-orbit-induced anisotropy, despite…

Strongly Correlated Electrons · Physics 2016-07-06 A. E. Taylor , R. Morrow , R. S. Fishman , S. Calder , A. I. Kolesnikov , M. D. Lumsden , P. M. Woodward , A. D. Christianson

Motivated by recent experiments exploring the spin-orbit-coupled magnetism in $4d$- and $5d$-band transition metal oxides, we study magnetic interactions in Ir- and Rh-based compounds. In these systems, the comparable strength of spin-orbit…

Strongly Correlated Electrons · Physics 2015-06-17 Natalia B. Perkins , Yuriy Sizyuk , Peter Wölfle

We study the low-lying excitations in 5d transition-metal oxide Sr_2IrO_4 on the localized electron picture. We find that Hund's coupling together with the spin-orbit interaction leads to exchange anisotropy which causes the spin wave gap.…

Strongly Correlated Electrons · Physics 2013-09-11 Jun-ichi Igarashi , Tatsuya Nagao

Using Raman spectroscopy to study the correlated 4$d$-electron metal Sr$_2$RhO$_4$, we observe pronounced excitations at 220 meV and 240 meV with $A_\mathrm{1g}$ and $B_\mathrm{1g}$ symmetries, respectively. We identify them as transitions…

Antiferromagnetic spintronics actively introduces new principles of magnetic memory, in which the most fundamental spin-dependent phenomena, i.e. anisotropic magnetoresistance effects, are governed by an antiferromagnet instead of a…

Materials Science · Physics 2018-05-08 Chengliang Lu , Bin Gao , Haowen Wang , Wei Wang , Songliu Yuan , Shuai Dong , Jun-Ming Liu

We used resonant inelastic x-ray scattering to reveal the nature of magnetic interactions in Sr2IrO4, a 5d transition-metal oxide with a spin-orbit entangled ground state and Jeff=1/2 magnetic momemts, referred to as 'isospins'. The magnon…

We present a comprehensive study of magnon excitations in the tetragonal easy-plane anti-ferromagnet Bi$_2$CuO$_4$ using inelastic neutron scattering and spin wave analyses. The nature of low energy magnons, and hence the anisotropy in this…

Strongly Correlated Electrons · Physics 2021-04-14 Bo Yuan , Nicholas P. Butch , Guangyong Xu , Barry Winn , J. P. Clancy , Young-June Kim

We report point-contact measurements of anisotropic magnetoresistance (AMR) in a single crystal of antiferromagnetic (AFM) Mott insulator Sr2IrO4. The point-contact technique is used here as a local probe of magnetotransport properties on…

Mesoscale and Nanoscale Physics · Physics 2014-12-03 Cheng Wang , Heidi Seinige , Gang Cao , Jian-Shi Zhou , John B. Goodenough , Maxim Tsoi
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