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Muon spin rotation (muSR) experiments reveal unconventional spin freezing and dynamics in the two-dimensional (2D) triangular lattice antiferromagnet NiGa2S4. Long-lived disordered Ni-spin freezing (correlation time > 10-6 s at 2 K) sets in…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Nambu , S. Nakatsuji , R. H. Heffner , Lei Shu , O. O. Bernal , K. Ishida

Spin dynamics in the van der Waals antiferromagnet FeGa$_2$S$_4$ with triangular lattices are investigated using magnetometry, neutron scattering, and muon spin relaxation measurements. The characteristic spin relaxation time is thoroughly…

Strongly Correlated Electrons · Physics 2024-10-30 Yifei Tang , Yoshihiko Umemoto , Yo Kawamoto , Masahiro Kawamata , Shinichiro Asai , Yoichi Ikeda , Masaki Fujita , Yusuke Nambu

We report a study of the triangular lattice Heisenberg magnet NiGa2S4 by the positive muon spin rotation and relaxation technique. We unravel three temperature regimes: (i) below T_c = 9.2(2) K a spontaneous static magnetic field at the…

Strongly Correlated Electrons · Physics 2009-11-13 A. Yaouanc , P. Dalmas de Reotier , Y. Chapuis , C. Marin , G. Lapertot , A. Cervellino , A. Amato

Nuclear spin-lattice relaxation times are measured on copper using magnetic resonance force microscopy performed at temperatures down to 42 mK. The low temperature is verified by comparison with the Korringa relation. Measuring spin-lattice…

Motivated by experiments on NiGa2S4, we discuss characteristic (finite temperature) properties of spin S = 1 quantum antiferromagnets on the triangular lattice. Several recent theoretical studies have suggested the possibility of…

Strongly Correlated Electrons · Physics 2009-06-30 E. M. Stoudenmire , Simon Trebst , Leon Balents

The electron spin resonance (ESR) spectroscopy was employed to investigate the spin dynamics in triangular lattice antiferromagnets CuCr$_{1-x}$Mg$_{x}$O$_2$ with $x =$ 0 and 0.02. All spectra can be well fitted by a single Lorentzian…

Strongly Correlated Electrons · Physics 2012-07-16 Renwen Li , Zhe Qu , Wei Tong , Yuheng Zhang

Magnetic susceptibility and muon spin relaxation (muSR) experiments have been carried out on the quasi-2D triangular-lattice spin S = 2 antiferromagnet FeGa2S4. The muSR data indicate a sharp onset of a frozen or nearly-frozen spin state at…

Strongly Correlated Electrons · Physics 2015-06-11 Songrui Zhao , P. Dalmas de R/'eotier , A. Yaouanc , D. E. MacLaughlin , J. M. Mackie , O. O. Bernal , Y. Nambu , T. Higo , S. Nakatsuji

We report the experimental and the analytical results of electron spin resonance (ESR) and magnetization in high magnetic fields up to about 68 T of the quasi two-dimensional triangular lattice antiferromagnet NiGa$_2$S$_4$. From the…

We have performed $^{69,71}$Ga nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) and muon spin rotation/resonance on the quasi two-dimensional antiferromagnet (AFM) NiGa$_2$S$_4$, in order to investigate its spin…

Strongly Correlated Electrons · Physics 2009-11-13 H. Takeya , K. Ishida , K. Kitagawa , Y. Ihara , K. Onuma , Y. Maeno , Y. Nambu , S. Nakatsuji , D. E. MacLaughlin , A. Koda , R. Kadono

NiGa$_2$S$_4$ is a triangular lattice S=1 system with strong two-dimensionality of the lattice, actively discussed as a candidate to host spin-nematic order brought about by strong quadrupole coupling. Using Raman scattering spectroscopy we…

We have studied magnetically frustrated Tb$_2$Sn$_2$O$_7$ by neutron diffraction and high resolution energy-resolved neutron scattering. At 0.1 K, we observe short range magnetic correlations with a typical scale of 4 \AA, close to the near…

Strongly Correlated Electrons · Physics 2009-11-13 I. Mirebeau , H. Mutka , P. Bonville , A. Apetrei , A. Forget

The crystal structure and magnetic correlations in triangular antiferromagnet FeGa$_2$S$_4$ are studied by x-ray diffraction, magnetic susceptibility, neutron diffraction and neutron inelastic scattering. We report significant mixing at the…

Neutron scattering is used to investigate spin correlations in ultra pure single crystals of the S=1 triangular lattice NiGa2S4. Despite a Curie-Weiss temperature of Theta_CW=-80(2) K, static (tau > 1 ns) short range (xi_ab=26(3) \AA)…

Strongly Correlated Electrons · Physics 2015-05-19 C. Stock , S. Jonas , C. Broholm , S. Nakatsuji , Y. Nambu , K. Onuma , Y. Maeno , J. -H. Chung

The anisotropic spin glass transition, in which spin freezing is observed only along the c-axis in pseudobrookite Fe$_2$TiO$_5$, has long been perplexing because the Fe$^{3+}$ moments (d$^5$) are expected to be isotropic. Recently, neutron…

Disordered Systems and Neural Networks · Physics 2023-01-18 Yu Li , P. G. LaBarre , D. M. Pajerowski , A. P. Ramirez , S. Rosenkranz , D. Phelan

Spin correlations and fluctuations in the 3d-transition-metal-based icosahedral quasicrystal Zn-Fe-Sc have been investigated by neutron scattering using polycrystalline samples. Magnetic diffuse scattering has been observed in the elastic…

The correlated spin dynamics and the temperature dependence of the correlation length $\xi(T)$ in two-dimensional quantum ($S=1/2$) Heisenberg antiferromagnets (2DQHAF) on square lattice are discussed in the light of experimental results of…

Strongly Correlated Electrons · Physics 2009-10-31 P. Carretta , T. Ciabattoni , A. Cuccoli , E. Mognaschi , A. Rigamonti , V. Tognetti , P. Verrucchi

Using elastic and inelastic neutron scattering techniques, we show that upon cooling a spatially anisotropic triangular antiferromagnet Ag$_2$MnO$_2$ freezes below $T_f ~\sim 50$ K into short range collinear state. The static spin…

Strongly Correlated Electrons · Physics 2009-07-21 S. Ji , J. -H. Kim , Y. Qiu , M. Matsuda , H. Yoshida , Z. Hiroi , M. A. Green , T. Ziman , S. -H. Lee

Inelastic neutron scattering is used to characterize spin fluctuations in the $d$-electron heavy fermion spinel $\rm LiV_2O_4$. The spin relaxation rate, $\Gamma_Q$, for $Q=0.6$ \AA$^{-1}$ is 1.5(1) meV at low temperatures and increases…

Strongly Correlated Electrons · Physics 2009-11-07 S. -H. Lee , Y. Qiu , C. Broholm , Y. Ueda , J. J. Rush

We present muon spin lattice relaxation measurements in the V15 spin 1/2 molecular nano-magnet. We find that the relaxation rate in low magnetic fields (<5 kG) is temperature independent below ~10 K, implying that the molecular spin is…

Mesoscale and Nanoscale Physics · Physics 2008-08-28 Z. Salman , R. F. Kiefl , K. H. Chow , W. A. MacFarlane , T. Keeler , T. Parolin , S. Tabbara , D. Wang

Spin fluctuations in the triangular-lattice Heisenberg antiferromagnet NaCrO$_2$ are investigated by means of quasi-elastic neutron scattering with high energy resolution and wide energy band. Two components with the following features are…

Strongly Correlated Electrons · Physics 2022-08-17 K. Tomiyasu , Y. P. Mizuta , M. Matsuura , K. Aoyama , H. Kawamura
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