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We investigate a spin-$\frac{1}{2}$ antiferromagnet, CuBr$_2$, which has quasi-one-dimensional structural motifs. The system has previously been observed to exhibit unusual Raman modes possibly due to a locally deformed crystal structure…

Strongly Correlated Electrons · Physics 2024-09-23 Biaoyan Hu , Yingying Peng , Xiaoqiang Liu , Qizhi Li , Qiangqiang Gu , Matthew J. Krogstad , Raymond Osborn , Takashi Honda , Ji Feng , Yuan Li

We calculate the two-magnon Raman scattering spectra in antiferromagnetic phases of several frustrated spin models defined on the honeycomb lattice. These include the N\'{e}el antiferromagnetic phase of a $J_1$-$J_2$-$J_3$ model and the…

Strongly Correlated Electrons · Physics 2021-04-06 Junru Pan , Feng Jin , Jianting Ji , Qingming Zhang , Rong Yu

Raman selection rules for electronic and magnetic excitations in BaFe2As2 were theoretically investigated and applied them to the separate detection of the nodal and anti-nodal gap excitations at the spin density wave (SDW) transition and…

We investigate the magnetic excitations of the hyperhoneycomb Kitaev magnet $\beta$-$\text{Li}_2\text{IrO}_3$ by means of inelastic Raman scattering. The spectra exhibits a coexistence of a broad scattering continuum and two sharp…

Strongly Correlated Electrons · Physics 2022-06-15 Yang Yang , Yiping Wang , Ioannis Rousochatzakis , Alejandro Ruiz , James G. Analytis , Kenneth S. Burch , Natalia B. Perkins

We explore the Mott insulating phases of dual-species bosonic spinor lattice gases, emphasizing the intriguing interplay between synthetic flux and inter-species spin exchange interaction. One of the species is subjected to Raman assisted…

Quantum Gases · Physics 2025-09-30 Rui-Shan Li , Zong-Zhen Pan , Shi-Jie Yang , Yi Zheng

Sr2IrO4 is one of the prime candidates for realizing exotic quantum spin orders owing to the subtle combination of spin-orbit coupling and electron correlation. Sensitive local magnetization measurement can serve as a powerful tool to study…

Materials Science · Physics 2025-03-26 Hyeokjun Heo , Jeongha An , Junyoung Kwon , Kwangrae Kim , Youngoh Son , B. J. Kim , Joonho Jang

Two-magnon Raman scattering intensity is obtained for two-dimensional spin-1/2 antiferromagnets in presence of hopping disorder. A consistent mode assignment scheme is prescribed which essentially establishes a correspondence between the…

Condensed Matter · Physics 2007-05-23 Saurabh Basu

Identifying and characterizing the parent phases of iron-based superconductors is an important step towards understanding the mechanism for their high temperature superconductivity. We present an investigation into the magnetic interactions…

Strongly Correlated Electrons · Physics 2015-06-18 E. E. McCabe , C. Stock , E. E. Rodriguez , A. S. Wills , J. W. Taylor , J. S. O. Evans

We report on Raman scattering measurements of single crystalline La$_{1-x}$Sr$_x$MnO$_3$ ($x$=0, 0.06, 0.09 and 0.125), focusing on the high frequency regime. We observe multi-phonon scattering processes up to fourth-order which show…

High-resolution resonant inelastic X-ray scattering (RIXS) at the oxygen K-edge has been used to study the orbital excitations of Ca2RuO4 and Sr2RuO4. In combination with linear dichroism X-ray absorption spectroscopy, the ruthenium…

Single crystals of the spin-gap system $\rm (VO)_2P_2O_7$ have been investigated by means of Raman scattering. At temperatures below T=75 K~$\approx 2\Delta_{01}({\bf k}=0)$, with $\Delta_{01}$ the singlet-triplet gap, a shoulder appears at…

Superconductivity · Physics 2009-10-31 M. Grove , P. Lemmens , G. Güntherodt , B. C. Sales , F. Büllesfeld , W. Assmus

The Mott insulator YVO$_{3}$ with $T_{N}$ = 118 K is revisited to explore the role of spin, lattice and orbital correlations across the multiple structural and magnetic transitions observed as a function of temperature. Upon cooling, the…

Strongly Correlated Electrons · Physics 2022-07-28 Yu Tao , Douglas L. Abernathy , Tianran Chen , Taner Yildirim , Jiaqiang Yan , Jianshi Zhou , John B. Goodenough , Despina Louca

We report temperature-dependent Raman scattering and X-ray diffraction studies of pyrochlore iridates, (Eu$_{1-x}$Bi$_x$)$_2$Ir$_2$O$_7$, for x=0, 0.02, 0.035, 0.05 and 0.1. The temperature variation in Raman experiments spans from 4 K to…

Strongly Correlated Electrons · Physics 2022-03-14 Anoop Thomas , Prachi Telang , Kshiti Mishra , Martin Cesnek , Jozef Bednarcik , D V S Muthu , Surjeet Singh , A K Sood

Polarized Raman scattering and infrared reflection spectra of hexagonal HoMnO$_3$ single crystals in the temperature range 10-300 K are reported. Group-theoretical analysis is performed and scattering selection rules for the second order…

Strongly Correlated Electrons · Physics 2009-11-10 A. P. Litvinchuk , M. N. Iliev , V. N. Popov , M. M. Gospodinov

The entanglement of electronic spin and orbital degrees of freedom is often the precursor to emergent behaviors in condensed matter systems. With considerable spin-orbit coupling strength, the cobalt atom on a honeycomb lattice offers a…

We report inelastic light scattering studies on Ca(Fe0.97Co0.03)2As2 in a wide spectral range of 120-5200 cm-1 from 5K to 300K, covering the tetragonal to orthorhombic structural transition as well as magnetic transition at Tsm ~ 160K. The…

Superconductivity · Physics 2014-07-11 Pradeep Kumar , D. V. S. Muthu , L. Harnagea , S. Wurmehl , B. Büchner , A. K. Sood

Lattice and spin excitations have been studied by Raman scattering in hexagonal YbMnO3 single crystals. The temperature dependences of the phonon modes show that the E2 mode at 256 cm-1 related to the displacement of Mn and O ions in a-b…

Strongly Correlated Electrons · Physics 2012-11-12 J. Liu , C. Toulouse , P. Rovillain , M. Cazayous , Y. Gallais , M. -A. Measson , S. W. Cheong , N. Lee , A. Sacuto

We report on the lattice and spin dynamics in the monopnictide CrAs using polarized Raman scattering. This system exhibits a first-order magneto-structural phase transition at T_N~ 265 K, below which the magnetic moments of Cr form an…

Materials Science · Physics 2019-10-07 K. Sen , Y. Yao , R. Heid , A. Omoumi , F. Hardy , K. Willa , M. Merz , A. A. Haghighirad , M. Le Tacon

We present two different theories for Raman scattering and Resonant Inelastic X-ray Scattering (RIXS) in the low temperature ferromagnetic phase of YTiO$_3$ and compare this to the available experimental data. For description of the orbital…

Strongly Correlated Electrons · Physics 2010-03-30 L. J. P. Ament , G. Khaliullin

We used a combination of polarized Raman spectroscopy and spin wave calculations to study magnetic excitations in the strong spin-orbit-coupled (SOC) bilayer perovskite antiferromagnet $Sr_3Ir_2O_7$. We observed two broad Raman features at…

Strongly Correlated Electrons · Physics 2020-08-24 Siwen Li , Elizabeth Drueke , Zach Porter , Wencan Jin , Zhengguang Lu , Dmitry Smirnov , Roberto Merlin , Stephen D. Wilson , Kai Sun , Liuyan Zhao
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