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In this work, we provide mechanistic insight into the initial stages of formation of ice across the limit of stability of supercooled water. Such an analysis is particularly important since crystal nucleation is not a relevant mechanism…

Statistical Mechanics · Physics 2026-05-26 Ashutosh Srivastava , Pankaj A. Apte

We study the nature of the glass transition by cooling model atomistic glass formers at constant rate from a temperature above the onset of glassy dynamics to $T=0$. Motivated by the East model, a kinetically constrained lattice model with…

Statistical Mechanics · Physics 2018-04-16 Alexander Hudson , Kranthi K. Mandadapu

We discuss some generic features of the dynamics of glass-forming liquids close to the glass transition singularity of the idealized mode-coupling theory (MCT). The analysis is based on a recent model by one of the authors for the…

Statistical Mechanics · Physics 2015-10-07 Tommaso Rizzo , Thomas Voigtmann

We studied the liquid-glass transition of $SiO_2$ by means of replica theory, utilizing an effective pair potential which was proved to reproduce a few experimental features of silica. We found a finite critical temperature $T_0$, where the…

Condensed Matter · Physics 2009-11-07 B. Coluzzi , P. Verrocchio

The phase diagram of H2O is extremely complex, in particular, it is believed that a second critical point exists deep below the supercooled water (SCW) region where two liquids of different densities coexist. The problem however, is that…

Chemical Physics · Physics 2015-08-26 Fei Yen , Zhenhua Chi , Adam Berlie , Xiaodi Liu , Alexander F. Goncharov

Over the last decade, an increasing body of evidence has emerged, supporting the existence of a metastable liquid-liquid critical point in supercooled water, whereby two distinct liquid phases of different densities coexist. Analysing long…

Soft Condensed Matter · Physics 2024-08-20 Cesare Malosso , Natalia Manko , Maria Grazia Izzo , Stefano Baroni , Ali Hassanali

The behaviour of a model glass forming liquid is analyzed for a range of densities, with a focus on the temperature interval where the liquid begins to display non-Arrhenius temperature dependence of relaxation times. Analyzing the dynamics…

Statistical Mechanics · Physics 2007-05-23 Srikanth Sastry

There has been long-standing debate about the physical state and possible phase transformations of confined liquids. In this report we show that a model confined liquid can behave both as a Newtonian liquid with very little change in its…

Soft Condensed Matter · Physics 2007-05-23 Shivprasad Patil , George Matei , Ahmet Oral , Peter M. Hoffmann

The striking behavior of water has deserved it to be referred to as an "anomalous" liquid. The water anomalies are greatly amplified in metastable (supercooled/stretched) regions. This makes difficult a complete experimental description…

Statistical Mechanics · Physics 2016-08-24 Miguel A. Gonzalez , Chantal Valeriani , Frederic Caupin , Jose L. F. Abascal

The possible superfluid transition of supercooled liquid parahydrogen is investigated by quantum Monte Carlo simulations. The cooling protocol adopted here allows for the investigation of a fluid phase down to a temperature T=0.25 K. No…

Statistical Mechanics · Physics 2018-03-07 Massimo Boninsegni

The shapes of cooperatively rearranging regions in glassy liquids change from being compact at low temperatures to fractal or ``stringy'' as the dynamical crossover temperature from activated to collisional transport is approached from…

Soft Condensed Matter · Physics 2015-06-25 Jacob D. Stevenson , Joerg Schmalian , Peter G. Wolynes

The quasi-2D Pt-based rare earth intermetallic material LaPt$_2$Si$_2$ has attracted attention as it exhibits strong interplay between charge density wave (CDW) and and superconductivity (SC). However, the most of the results reported on…

The stability-limit conjecture (SLC) proposes that the liquid spinodal of water returns to positive pressure in the supercooled region, and that the apparent divergence of water's thermodynamic response functions as temperature decreases…

Statistical Mechanics · Physics 2019-07-24 Pheerawich Chitnelawong , Francesco Sciortino , Peter H. Poole

Recent experimental results suggest that metallic liquids universally exhibit a high-temperature dynamical crossover, which is correlated with the glass transition temperature ($T_{g}$). We demonstrate, using molecular dynamics results for…

Disordered Systems and Neural Networks · Physics 2016-03-24 Ryan Soklaski , Vy Tran , Zohar Nussinov , K. F. Kelton , Li Yang

By means of Monte Carlo simulations, using finite size scaling and conformal transformations, evidences of a topological phase transition in liquid crystals in two dimensions are reported. A paramagnetic phase appears at high temperature…

Other Condensed Matter · Physics 2010-07-13 V. Ricardo Paredes , Ana I. Fariñas-Sánchez , Bertrand Berche

It is generally assumed that solid hydrogen will transform into a metallic alkali-like crystal at sufficiently high pressure. However, some theoretical models have also suggested that compressed hydrogen may form an unusual two-component…

Materials Science · Physics 2009-11-10 Stanimir A. Bonev , Eric Schwegler , Tadashi Ogitsu , Giulia Galli

Surface freezing is a phenomenon in which crystallization is enhanced at a vapor-liquid interface. In some systems, such as $n$-alkanes, this enhancement is dramatic, and results in the formation of a crystalline layer at the free interface…

Soft Condensed Matter · Physics 2017-09-13 Amir Haji Akbari , Pablo G. Debenedetti

Many qualitative observations on the glass transition in classical fluids are well described by the mode coupling theory (MCT) but the extent of the non-ergodicity domain is often over-estimated by this theory. Making it more quantitative…

Statistical Mechanics · Physics 2012-10-04 S. Amokrane , F. Tchangnwa Nya , J. M. Ndjaka

There have been ample studies of the many phases of H2O in both its solid and low pressure liquid states, and the transitions between them. Using molecular dynamics simulations we address the hitherto unexplored deeply supercritical…

Soft Condensed Matter · Physics 2020-09-02 Cillian Cockrell , Oliver Dicks , Vadim Brazhkin , Kostya Trachenko

When liquids are cooled sufficiently rapidly below their melting temperature, they may bypass crystalization and, instead, enter a long-lived metastable supercooled state that has long been the focus of intense research. Although they…

Statistical Mechanics · Physics 2023-12-05 Zohar Nussinov
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