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The motion of electrons and ions in medium-sized rare gas clusters (1000 atoms) exposed to intense laser pulses is studied microscopically by means of classical molecular dynamics using a hierarchical tree code. Pulse parameters for optimum…

Atomic and Molecular Clusters · Physics 2007-05-23 Ulf Saalmann , Jan-Michael Rost

The electron dynamics of rare gas clusters in laser fields is investigated quantum mechanically by means of time-dependent density functional theory. The mechanism of early inner and outer ionization is revealed. The formation of an…

Atomic Physics · Physics 2009-11-10 D. Bauer , A. Macchi

Pulses of extreme ultraviolet (XUV) light, with wavelengths between 10 and 100$\,$nm, can be used to image and excite ultra-fast phenomena such as the motion of atomic electrons. Here we show that the illumination of plasma with…

Plasma Physics · Physics 2018-08-24 T. G. Blackburn , A. A. Gonoskov , M. Marklund

XUV fluorescence spectroscopy provides information on energy absorption and dissipation processes taking place in the interaction of helium clusters with intense femtosecond laser pulses. The present experimental results complement the…

Atomic and Molecular Clusters · Physics 2023-10-23 Malte Sumfleth , Andreas Przystawik , Mahesh Namboodiri , Tim Laarmann

We derive the analytical theory describing the process of sub-femtosecond pulse formation from a quasi-monochromatic seeding extreme ultraviolet (XUV) radiation, which propagates in active medium of a hydrogen-like plasma-based X-ray laser…

We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

Atomic Physics · Physics 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao

Resonant Raman excitation by ultrafast vacuum ultraviolet laser pulses is a powerful means to study electron dynamics in molecules, but experiments must contend with linear background ionization: frequencies high enough to reach resonant…

Chemical Physics · Physics 2015-06-23 S. Miyabe , P. Bucksbaum

A method to generate an intense isolated few-cycle attosecond XUV pulse is demonstrated using particle-in-cell simulations. When a tailored laser pulse with a sharp edge irradiates a foil target, a strong transverse net current can be…

Plasma Physics · Physics 2014-06-13 Zi-Yu Chen , Xiao-Ya Li , Li-Ming Chen , Yu-Tong Li , Wen-Jun Zhu

We present and discuss a new computationally inexpensive method to study, within the single active electron approximation, the interaction of a complex system with an intense ultrashort laser pulse. As a first application, we consider the…

The interaction of strong near-infrared (NIR) laser pulses with wide-bandgap dielectrics produces high harmonics in the extreme ultraviolet (XUV) wavelength range. These observations have opened up the possibility of attosecond metrology in…

We present a theoretical study of the ionization dynamics of a hydrogen atom exposed to attosecond laser pulses in the extreme ultra violet region at very high intensities. The pulses are such that the electron is expected to reach…

Atomic Physics · Physics 2017-04-12 Tor Kjellsson , Sølve Selstø , Eva Lindroth

We report on a compact and spectrally intense extreme-ultraviolet (XUV) source, which is based on high-harmonic generation (HHG) driven by 395 nm pulses. In order to minimize the XUV virtual source size and to maximize the XUV flux, HHG is…

Optics · Physics 2021-07-01 M. Kretschmar , M. J. J. Vrakking , B. Schütte

The ionization dynamics of helium droplets in a wide size range from 220 to 10^6 He atoms irradiated with intense femtosecond extreme ultraviolet (XUV) pulses of 10^9 {\div} 10^{12} W/cm2 power density is investigated in detail by…

In this study the generation of energetic coherent extreme ultraviolet (XUV) radiation with controlled polarization, is reported. The XUV radiation results from the process of high harmonic generation (HHG), in a gas phase atomic medium,…

Atomic Physics · Physics 2021-06-17 E. Vassakis , I. Orfanos , I. Liontos , D. Charalambidis , P. Tzallas , E. Skantzakis

The effect of intense X-ray laser interaction on argon clusters is studied theoretically with a mixed quantum/classical approach. In comparison to a single atom we find that ionization of the cluster is suppressed, which is in striking…

Atomic and Molecular Clusters · Physics 2009-11-07 Ulf Saalmann , Jan M Rost

The interaction of short laser pulses with small rare gas clusters is investigated by using a microscopic, semi-classical model with an explicit treatment of the inner-atomic dynamics. Field and collisional ionisation as well as…

Atomic and Molecular Clusters · Physics 2007-05-23 D. Bauer

Clusters and nanodroplets hold the promise of enhancing high-order nonlinear optical effects due to their high local density. However, only moderate enhancement has been demonstrated to date. Here, we report the observation of energetic…

The interaction of atomic clusters with short, intense pulses of laser light to form extremely hot, dense plasmas has attracted extensive experimental and theoretical interest. The high density of atoms within the cluster greatly enhances…

Atomic Physics · Physics 2009-11-11 Zachary B. Walters , Robin Santra , Chris H. Greene

The quantum-classical hybrid-description of rare-gas clusters interacting with intense light pulses which we have developed is described in detail. Much emphasis is put on the treatment of screening electrons in the cluster which set the…

Atomic and Molecular Clusters · Physics 2011-11-09 Ionut Georgescu , Ulf Saalmann , Jan M. Rost

We present a theoretical study of atomic ionization due to an XUV pulse in the presence of an infrared laser. Within the strong field approximation and considering the periodicity and symmetry of the transition matrix we show that the…

Atomic Physics · Physics 2020-08-26 Renata Della Picca , Ana Alicia Gramajo , Sebastián López , Diego G Arbó