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Localized plasmons formed in ultrathin metallic nanogaps can lead to robust absorption of incident light. Plasmonic metasurfaces based on this effect can efficiently generate energetic charge carriers, also known as hot electrons, owing to…

Optics · Physics 2022-09-28 Larousse Khosravi Khorashad , Christos Argyropoulos

Ultrafast nanophotonics is an emerging research field aimed at the development of nanodevices capable of light modulation with unprecedented speed. A promising approach exploits the optical nonlinearity of nanostructured materials (either…

Nanoplasmonics exploits the coupling between light and collective electron density oscillations (plasmons) to bypass the stringent limits imposed by diffraction. This coupling enables confinement of light to sub-wavelength volumes and is…

The nonlinear optical dynamics of nano-materials comprised of plasmons interacting with quantum emitters is investigated by a self-consistent model based on the coupled Maxwell-Liouville-von Neumann equations. It is shown that ultra-short…

Mesoscale and Nanoscale Physics · Physics 2013-12-04 Maxim Sukharev , Tamar Seideman , Robert J. Gordon , Adi Salomon , Yehiam Prior

The damping of surface plasmons generates hot carriers, which holds promise for photoelectric conversion and photocatalysis. Recent studies have revealed the nonequilibrium characters of the plasmonic hot carriers and their nonadiabatic…

Materials Science · Physics 2025-07-10 Yu Chen , Shengxiang Wu , Shiwu Gao

Exploring nonequilibrium hot carriers from plasmonic metal nanostructures is a dynamic field in optoelectronics, driving photochemical reactions such as solar fuel generation. The hot carrier injection mechanism and the reaction rate are…

Nonlinear metasurfaces are multifunctional photonic elements that generate and control light, enabling multiple proof-of-principle applications, such as in nonlinear holography, beam shaping, and nanoscale sources of entangled photon pairs.…

The combination of isochoric heating of solids by free electron lasers (FEL) and in situ diagnostics by X-ray Thomson scattering (XRTS) allows for measurements of material properties at warm dense matter (WDM) conditions relevant for…

Hybrid plasmonic devices involve a nanostructured metal supporting localized surface plasmons to amplify light-matter interaction, and a non-plasmonic material to functionalize charge excitations. Application-relevant epitaxial…

Heterogeneous catalysis of adsorbates on metallic surfaces mediated by plasmon has potential high photoelectric conversion efficiency and controllable reaction selectivity. Theoretical modeling of dynamical reaction processes provides…

Chemical Physics · Physics 2023-06-05 Xiaoyan Wu , Tammo van der Heide , Thomas Frauenheim , Sergei Tretiak , ChiYung Yam , Yu Zhang

Above-threshold light emission from plasmonic tunnel junctions, when emitted photons have energies significantly higher than the energy scale of the incident electrons, has attracted much recent interest in nano-optics, while the underlying…

Mesoscale and Nanoscale Physics · Physics 2020-12-08 Longji Cui , Yunxuan Zhu , Mahdiyeh Abbasi , Arash Ahmadivand , Burak Gerislioglu , Peter Nordlander , Douglas Natelson

While being extensively studied as an important physical process to alter exciton population in nanostructures at fs time scale, carrier multiplication has not been considered seriously as a major mechanism for phase transition. Real-time…

Materials Science · Physics 2016-09-20 Junhyeok Bang , Y. Y. Sun , X. -Q. Liu , F. Gao , S. B. Zhang

We use a non-equilibrium many-body theory that engages the elements of transient coherence, correlation, and nonlinearity to describe changes in the magnetic and electronic phases of strongly correlated systems induced by femtosecond…

Strongly Correlated Electrons · Physics 2018-04-24 P. C. Lingos , M. D. Kapetanakis , M. Mootz , J. Wang , I. E. Perakis

Hot electrons generated from the decay of localized surface plasmons in metallic nanostructures have the potential to transform photocatalysis, photodetection and other optoelectronic applications. However, the understanding of hot-carrier…

The knowledge of the carrier dynamics in nanostructures is of fundamental importance for the development of (opto)electronic devices. This is true for semiconducting nanostructures as well as for plasmonic nanoparticles (NPs). Indeed,…

Ultrafast plasmonics of novel materials has emerged as a promising field of nanophotonics bringing new concepts for advanced optical applications. Ultrafast electronic photoexcitation of a diamond surface and subsequent surface…

Harnessing non-equilibrium hot carriers from plasmonic metal nanostructures constitutes a vibrant research field. It promises to enable control of activity and selectivity of photochemical reactions, especially for solar fuel generation.…

This work presents numerical and experimental results of plasmonic Metal-Insulator optical nano-cavities. The systems are composed of Silver as metal, polyvinylpyrrolidone or indium tin oxide or zinc oxide as insulator. The proposed…

Plasmonic hot carrier devices extract excited carriers from metal nanostructures before equilibration, and have the potential to surpass semiconductor light absorbers. However their efficiencies have so far remained well below theoretical…

Nanostructured plasmonic metal systems are known to enhance greatly variety of radiative and nonradiative optical processes, both linear and nonlinear, which are due to the interaction of an electron in a molecule or semiconductor with the…

Optics · Physics 2009-11-13 Maxim Durach , Anastasia Rusina , Victor I. Klimov , Mark I. Stockman