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We report on terahertz spectroscopic measurements of quantum spin dynamics on single crystals of a spin-1/2 frustrated spin-ladder antiferromagnet BiCu$_2$PO$_6$ as a function of temperature, polarization, and applied external magnetic…

The magnon and optical phonon spectrum of an incommensurate multiferroic such as BiFeO3 is considered in the framework of a phenomenological Landau theory. The resulting spin wave spectrum is quite distinct from commensurate substances due…

Strongly Correlated Electrons · Physics 2008-01-24 Rogerio de Sousa , Joel E. Moore

Pressure-induced phase transitions of multiferroic BiFeO3 have been investigated using synchrotron radiation X-ray diffraction with diamond anvil cell technique at room temperature. Present experimental data clearly show that rhombohedral…

Materials Science · Physics 2013-08-30 Zhang XiaoLi , Wu Ye , Zhang Qian , Dong JunCai , Wu Xiang , Liu Jing , Wu ZiYu , Chen DongLiang

Elucidating the nature of spin excitations is important to understanding the mechanism of superconductivity in the iron pnictides. Motivated by recent inelastic neutron scattering measurements in the nearly 100% detwinned…

Superconductivity · Physics 2020-03-02 Changle Liu , Xingye Lu , Pengcheng Dai , Rong Yu , Qimiao Si

The magnetic field--driven transition in the spin-Peierls system CuGeO_3 associated with the closing of the spin gap is investigated numerically. The field dependence of the spin dynamical structure factor (seen by inelastic neutron…

Strongly Correlated Electrons · Physics 2009-10-30 D. Poilblanc , J. Riera , C. A. Hayward , C. Berthier , M. Horvatic

Although BiFeO$_3$ is one of the most studied multiferroic materials, recent magnetization and neutron scattering studies have revealed a new magnetic phase in this compound - the transverse conical phase. To study the collective spin…

Materials Science · Physics 2024-02-05 B. Tóth , D. G. Farkas , K. Amelin , T. Rõõm , U. Nagel , L. Udvardi , L. Szunyogh , L. Rózsa , T. Ito , S. Bordács

We present a first-principles study of multiferroic BiFeO3 at high pressures. Our work reveals the main structural (change in Bi's coordination and loss of ferroelectricity), electronic (spin crossover and metallization), and magnetic (loss…

Materials Science · Physics 2009-12-17 O. E. Gonzalez-Vazquez , Jorge Iniguez

We report the magnetic field dependence of the THz absorption and non-reciprocal directional dichroism spectra of BiFeO$_3$ measured on the three principal crystal cuts for fields applied along the three principal directions of each cut.…

Strongly Correlated Electrons · Physics 2021-12-01 D. G. Farkas , D. Szaller , I. Kézsmárki , U. Nagel , T. Rõõm , L. Peedu , J. Viirok , J. S. White , R. Cubitt , T. Ito , R. S. Fishman , S. Bordács

We performed inelastic neutron scattering experiments on single crystal samples of a linear magnetoelectric material Mn$_{3}$Ta$_{2}$O$_{8}$, which exhibits a collinear antiferromagnetic order, to reveal the spin dynamics. Numerous modes…

Strongly Correlated Electrons · Physics 2025-04-08 Hodaka Kikuchi , SHunsuke Hasegawa , Shinichiro Asai , Tao Hong , Kenta Kimura , Tsuyoshi Kimura , Shinichi Itoh , Takatsugu Masuda

With the advancement in synthesizing and analyzing Kitaev materials, the Kitaev-Heisenberg model on the honeycomb lattice has attracted a lot of attention in the last few years. Several variations, which include additional anisotropic…

Strongly Correlated Electrons · Physics 2018-08-15 Darshan G. Joshi

Magnetic, dielectric, and magnetoelectric properties in a spin-state transition system are examined, motivated by the recent discovery of a multiferroic behavior in a cobalt oxide. We construct an effective model Hamiltonian based on the…

Strongly Correlated Electrons · Physics 2018-06-13 Makoto Naka , Eriko Mizoguchi , Joji Nasu , Sumio Ishihara

We have created a nonequilibrium population of antiferromagnetic spin-waves in Cr2O3, and characterized its dynamics, using frequency- and time-resolved nonlinear optical spectroscopy of the exciton-magnon transition. We observe a…

Strongly Correlated Electrons · Physics 2009-10-31 J. S. Dodge , A. B. Schumacher , D. S. Chemla , N. Ingle , M. R. Beasley

We report experimental evidence for pressure instabilities in the model multiferroic BiFeO3 and namely reveal two structural phase transitions around 3 GPa and 10 GPa by using diffraction and far-infrared spectroscopy at a synchrotron…

Materials Science · Physics 2011-07-26 R. Haumont , P. Bouvier , A. Pashkin , K. Rabia , S. Frank , B. Dkhil , W. A. Crichton , C. A. Kuntscher , J. Kreisel

We use general hydrodynamic equations to determine the long-wavelength spin excitations in isotropic antiferromagnets in the presence of a homogeneous magnetization. The latter may be induced, such as in antiferromagnets in an external…

Strongly Correlated Electrons · Physics 2017-06-07 T. R. Kirkpatrick , D. Belitz

Magnetic control of correlated spin systems is central to the development of next-generation spin-based technologies. Rare-earth orthoferrites provide an interesting platform in which exchange coupling between rare-earth 4f and…

We investigate the demagnetization dynamics of the cycloidal and sinusoidal phases of multiferroic TbMnO$_3$ by means of time-resolved resonant soft x-ray diffraction following excitation by an optical pump. Using orthogonal linear x-ray…

The magnetic field induced rearrangement of the cycloidal spin structure in ferroelectric mono-domain single crystals of the room-temperature multiferroic BiFeO$_3$ is studied using small-angle neutron scattering (SANS). The cycloid…

Strongly Correlated Electrons · Physics 2018-04-11 S. Bordács , D. G. Farkas , J. S. White , R. Cubitt , L. DeBeer-Schmitt , T. Ito , I. Kézsmárki

High pressure can provoke spin transitions in transition metal-bearing compounds. These transitions are of high interest not only for fundamental physics and chemistry, but also may have important implications for geochemistry and…

Using configuration-state-constrained electronic structure calculations based on the generalized gradient approximation plus Hubbard U method, we sought the origin of the giant tetragonal ferroelectric distortion in the ambient phase of the…

Strongly Correlated Electrons · Physics 2011-05-25 Ting Jia , Hua Wu , Guoren Zhang , Xiaoli Zhang , Ying Guo , Zhi Zeng , Hai-Qing Lin

The pressure dependence of light-induced effects in single-crystalline BiFeO$_3$ is studied by optical spectroscopy. At low pressures, we observe three light-induced absorption features with energies just below the two crystal field…

Materials Science · Physics 2019-10-31 F. Meggle , J. Ebad-Allah , J. Kreisel , C. A. Kuntscher
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