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The possibility of observing a glass transition in water before crystallisation occurs has been debated vigorously but inconclusively over five decades [1,2]. For two decades a glass transition at 136K [2,3] was accepted but this transition…

Chemical Physics · Physics 2007-05-23 Y. -Z. Yue , C. A. Angell

The question of whether glass continues to relax at low temperature is of fundamental and practical interest. Here, we report a novel atomistic simulation method allowing us to directly access the long-term dynamics of glass relaxation at…

Disordered Systems and Neural Networks · Physics 2015-10-27 Yingtian Yu , Mengyi Wang , Dawei Zhang , Bu Wang , Gaurav Sant , Mathieu Bauchy

The history dependence of the glasses formed from flow-melted steady states by a sudden cessation of the shear rate $\dot\gamma$ is studied in colloidal suspensions, by molecular dynamics simulations, and mode-coupling theory. In an ideal…

The nature of defects in amorphous materials, analogous to vacancies and dislocations in crystals, remains elusive. Here we explore their nature in a three-dimensional microscopic model glass-former which describes granular, colloidal,…

Soft Condensed Matter · Physics 2019-11-13 Camille Scalliet , Ludovic Berthier , Francesco Zamponi

The glass transition is considered as a phase transition in the system of topologically protected excitations in matter structure. The critical behavior of the system is considered both in statics and dynamics cases. It is shown in the…

Statistical Mechanics · Physics 2022-04-20 Mikail Vasin

We review recent theoretical progress on glassy dynamics, with special emphasis on the importance and universality of the ``aging regime'', which is relevant to many experimental situations. The three main subjects which we address are: (i)…

Disordered Systems and Neural Networks · Physics 2008-02-03 Jean-Philippe Bouchaud , Leticia F. Cugliandolo , Jorge Kurchan , Marc Mezard

We report avalanche criticality of thermal relaxation in glassy systems after a rapid quench by molecular simulation. Our analysis of the energy landscape and the scaling reveals that particle rearrangement is critical. The critical…

Soft Condensed Matter · Physics 2024-09-25 Yuki Takaha , Hideyuki Mizuno , Atsushi Ikeda

Glass is an under-cooled liquid that very slowly relaxes towards the equilibrium crystalline state. Its energy balance is ill understood, since it is widely believed that the glassy state cannot be described thermodynamically. However, the…

Statistical Mechanics · Physics 2009-11-07 Theo M. Nieuwenhuizen

We consider the stationary state of a fluid comprised of inelastic hard spheres or disks under the influence of a random, momentum-conserving external force. Starting from the microscopic description of the dynamics, we derive a nonlinear…

Statistical Mechanics · Physics 2013-02-25 W. T. Kranz , M. Sperl , A. Zippelius

Recently, ultrastable glasses have been created through vapor deposition. Subsequently, computer simulation algorithms have been proposed that mimic the vapor deposition process and result in simulated glasses with increased stability. In…

Soft Condensed Matter · Physics 2015-01-15 Hannah Staley , Elijah Flenner , Grzegorz Szamel

Some facets of the way sound waves travel through glasses are still unclear. Recent works have shown that in the low-temperature harmonic limit a crucial role in controlling sound damping is played by local elastic heterogeneity. Sound…

Materials Science · Physics 2020-06-01 Hideyuki Mizuno , Giancarlo Ruocco , Stefano Mossa

The interrelation of dynamic processes active on separated time-scales in glasses and viscous liquids is investigated using a model displaying two time-scale bifurcations both between fast and secondary relaxation and between secondary and…

Disordered Systems and Neural Networks · Physics 2015-03-19 Andrea Crisanti , Luca Leuzzi , Matteo Paoluzzi

Dense liquids gradually transform into non-equilibrium amorphous solids as they pass through the experimental glass transition. Experimentally, ergodicity is lost because measurements are conducted within a finite time window. More than…

Soft Condensed Matter · Physics 2025-07-08 Gerhard Jung , Misaki Ozawa , Giulio Biroli , Ludovic Berthier

A system is glassy when the observation time is much smaller than the equilibration time. A unifying thermodynamic picture of the glassy state is presented. Slow configurational modes are in quasi-equilibrium at an effective temperature. It…

Statistical Mechanics · Physics 2009-10-31 Th. M. Nieuwenhuizen

We review the inherent structure thermodynamical formalism and the formulation of an equation of state for liquids in equilibrium based on the (volume) derivatives of the statistical properties of the potential energy surface. We also show…

Soft Condensed Matter · Physics 2009-11-07 S. Mossa , E. La Nave , P. Tartaglia , F. Sciortino

We use coherent X-rays to probe the aging dynamics of a metallic glass directly on the atomic level. Contrary to the common assumption of a steady slowing down of the dynamics usually observed in macroscopic studies, we show that the…

Materials Science · Physics 2015-10-23 Zach Evenson , Beatrice Ruta , Simon Hechler , Moritz Stolpe , Eloi Pineda , Isabella Gallino , Ralf Busch

Measuring, characterizing and modelling the slow dynamics of glassy soft matter is a great challenge, with an impact that ranges from industrial applications to fundamental issues in modern statistical physics, such as the glass transition…

Soft Condensed Matter · Physics 2009-11-11 Luca Cipelletti , Laurence Ramos

When a liquid is cooled below its melting temperature it usually crystallizes. However, if the quenching rate is fast enough, it is possible that the system remains in a disordered state, progressively losing its fluidity upon further…

Disordered Systems and Neural Networks · Physics 2009-11-10 Tullio Scopigno , Giancarlo Ruocco , Francesco Sette , Giulio Monaco

Glass films created by vapor-depositing molecules onto a substrate can exhibit properties similar to those of ordinary glasses aged for thousands of years. It is believed that enhanced surface mobility is the mechanism that allows vapor…

Soft Condensed Matter · Physics 2017-11-03 Ludovic Berthier , Patrick Charbonneau , Elijah Flenner , Francesco Zamponi

We show that, in nonequilibrium systems with small heat flows, there is a time-scale dependent effective temperature which plays the same role as the thermodynamical temperature, in that it controls the direction of heat flows and acts as a…

Disordered Systems and Neural Networks · Physics 2009-10-28 Leticia F. Cugliandolo , Jorge Kurchan , Luca Peliti