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We demonstrate that the capacitance of ionic-liquid filled supercapacitors is substantially increased by placing a diode-like structure on the separator membrane. We call the structured separator: gate, and demonstrate that the order of a…

Applied Physics · Physics 2019-07-09 Tazima S. Chowdhury , Haim Grebel

We investigate electronic transport through two types of conjugated molecules. Mechanically controlled break-junctions are used to couple thiol endgroups of single molecules to two gold electrodes. Current-voltage characteristics (IVs) of…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Reichert , R. Ochs , D. Beckmann , H. B. Weber , M. Mayor , H. v. Loehneysen

A new type of microfluidic system for biological cell manipulation, a CMOS/microfluidic hybrid, is demonstrated. The hybrid system starts with a custom-designed CMOS (complementary metal-oxide semiconductor) chip fabricated in a…

Quantitative Methods · Quantitative Biology 2007-05-23 Hakho Lee , Yong Liu , Donhee Ham , Robert M. Westervelt

The study of electronic transitions within a molecule connected to the absorption or emission of light is a common task in the process of the design of new materials. The transitions are complex quantum mechanical processes and a detailed…

Human-Computer Interaction · Computer Science 2021-06-03 Talha Bin Masood , Signe Sidwall Thygesen , Mathieu Linares , Alexei I. Abrikosov , Vijay Natarajan , Ingrid Hotz

We present transport measurements of electrons on the surface of liquid helium in a microchannel device in which a constriction may be formed by a split-gate electrode. The surface electron current passing through the microchannel first…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 David Rees , Isao Kuroda , Claire Marrache-Kikuchi , Moritz Hofer , Paul Leiderer , Kimitoshi Kono

Partial atomic charges are a useful and intuitive concept for understanding molecular properties and chemical reaction mechanisms, showing how changes in molecular geometry can affect the flow of electronic charge within a molecule.…

Chemical Physics · Physics 2022-01-14 Ryan J. MacDonell , Serguei Patchkovskii , Michael S. Schuurman

Materials in which electrons occupy interstitial sites as anions are called electrides and exhibit unusual dimensionality-dependent electronic behavior. These properties make electrides attractive for catalysis, transparent conductors, and…

Materials Science · Physics 2026-01-01 Lee A. Burton

We investigate electron transport through a finite two dimensional mesoscopic periodic potential, consisting of an array of lateral quantum dots with electron density controlled by a global top gate. We observe a transition from an…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Neal E. Staley , Nirat Ray , Marc A. Kastner , Micah P. Hanson , Arthur C. Gossard

Improvement of electrochemical technologies is one of the most popular topics in the field of renewable energy. However, this process requires a deep understanding of the electrode electrolyte interface behavior under operando conditions.…

Electrochemical devices often consist of multicomponent electrolyte solutions. Two processes influence the overall dynamics of these devices: the formation of electrical double layers and chemical conversion due to redox reactions. However,…

Chemical Physics · Physics 2022-06-20 Nathan Jarvey , Filipe Henrique , Ankur Gupta

Discovering new electrodes for sodium-ion battery requires clear understanding of the material process during battery operation. Using first-principles calculations, we identify mechanisms of ionic diffusion and electronic transfer in newly…

Materials Science · Physics 2017-09-20 Chol-Jun Yu , Song-Hyok Choe , Gum-Chol Ri , Sung-Chol Kim , Hyok-Su Ryo , Yong-Jin Kim

Electric-field-controlled charge transport is a key concept of modern computers, embodied namely in field effect transistors. The metallic gate voltage controls charge population, thus it is possible to define logical elements which are the…

Mesoscale and Nanoscale Physics · Physics 2020-07-30 Deniz Eksi , Afif Siddiki

We present experiments on a superconductor-normal metal electron refrigerator in a regime where single-electron charging effects are significant. The system functions as a heat transistor, i.e., the heat flux out from the normal metal…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Olli-Pentti Saira , Matthias Meschke , Francesco Giazotto , Alexander M. Savin , Mikko Mottonen , Jukka P. Pekola

Cell-based biosensors constitute a fundamental tool in biotechnology, and their relevance has greatly increased in recent years as a result of a surging demand for reduced animal testing and for high-throughput and cost-effective in vitro…

Electron transfer is at the heart of many fundamental physical, chemical, and biochemical processes essential for life. The exact simulation of these reactions is often hindered by the large number of degrees of freedom and by the essential…

This report builds upon work introducing the concept of independent control over current and potential in electrocatalytic systems, as a means of improving control over their product selectivity. Previous work, describing an approach…

Chemical Physics · Physics 2023-10-31 Peter Agbo

In this work, we propose a strategy to sense quantitatively and specifically cations, out of a single organic electrochemical transistor (OECT) device exposed to an electrolyte. From the systematic study of six different chloride salts over…

Applied Physics · Physics 2018-03-29 Sebastien Pecqueur , David Guerin , Dominique Vuillaume , Fabien Alibart

Conjugated polymer-based organic electrochemical transistors (OECTs) are being studied for applications ranging from biochemical sensing to neural interfaces. While new conjugated polymers are being developed that can interface digital…

Materials Science · Physics 2019-10-01 Connor G. Bischak , Lucas Q. Flagg , David S. Ginger

Manipulation of the charge of the dielectric interface between two bulk liquids not only enables the adjustment of the interfacial tension but also controls the storage capacity of ions in the ionic double layers adjacent to each side of…

Soft Condensed Matter · Physics 2018-03-14 Marise J. E. Westbroek , Niels Boon , René van Roij

An electrochemical potentiostat interface for mobile devices has been designed and implemented. The interface consists of a potentiostat module, a microcontroller module, and a Bluetooth module. The potentiostat module performs…

Instrumentation and Detectors · Physics 2015-09-30 Henry Fu , Henry Chow , Michael Lew , Shruti Menon , Craig Scratchley , M. Ash Parameswaran