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By using highly time-resolved spectroscopy with an alternative {\sigma}+/{\sigma} - laser pulse modulation technique, we are able to measure the fast buildup and decay times of the dynamical nuclear spin polarization (DNSP) at 5 K for a…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 X. M. Dou , B. Q. Sun , D. S. Jiang , H. Q. Ni , Z. C. Niu

Repeated injection of spin polarized carriers in a quantum dot leads to the polarization of nuclear spins, a process known as dynamic nuclear spin polarization (DNP). Here, we report the first observation of p-shell carrier assisted DNP in…

Mesoscale and Nanoscale Physics · Physics 2016-03-23 C. F. Fong , Y. Ota , E. Harbord , S. Iwamoto , Y. Arakawa

We study repeated (noncontinuous) measurements on the electron spin in a quantum dot and find that the measurement technique may lead to a different met$ or mechanism to realize nuclear spin polarization. While it may be used in any case,…

Quantum Physics · Physics 2011-07-28 Lian-Ao Wu

A key to achieving ultra-long electron spin memory in quantum dots (QDs) at 0~$T$ is the polarization of the nuclei, such that the electron spin is stabilized along the nuclear magnetic field. We demonstrate that spin-polarized electrons in…

Other Condensed Matter · Physics 2007-05-23 A. Greilich , R. Oulton , S. Yu. Verbin , R. V. Cherbunin , T. Auer , D. R. Yakovlev , M. Bayer , V. Stavarache , D. Reuter , A. Wieck

Resonant laser scattering along with photon correlation measurements have established the atom-like character of quantum dots. Here, we present measurements which challenge this identification for a wide range of experimental parameters:…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 C. Latta , A. Högele , Y. Zhao , A. N. Vamivakas , P. Maletinsky , M. Kroner , J. Dreiser , I. Carusotto , A. Badolato , D. Schuh , W. Wegscheider , M. Atature , A. Imamoglu

Dynamical polarization of nuclear spin ensembles is of central importance for magnetic resonance studies, precision sensing and for applications in quantum information theory. Here we propose a scheme to generate long-lived singlet pairs in…

Quantum Physics · Physics 2017-04-06 Johannes N. Greiner , D. D. Bhaktavatsala Rao , Jörg Wrachtrup

Multielectron semiconductor quantum dots (QDs) provide a novel platform to study the role of Coulomb correlations in finite quantum systems and their impact on many-body energy spectra. An example is the formation of interaction-driven,…

Electron spin dephasing in a singly charged semiconductor quantum dot can partially be suppressed by periodic laser pulsing. We propose a semi-classical approach describing the decoherence of the electron spin polarization governed by the…

Mesoscale and Nanoscale Physics · Physics 2017-11-15 Natalie Jäschke , Andreas Fischer , E. Evers , V. V. Belykh , Alex Greilich , Manfred Bayer , Frithjof B. Anders

We review our investigation of the spin dynamics for two electrons confined to a double quantum dot under the influence of the hyperfine interaction between the electron spins and the surrounding nuclei. Further we propose a scheme to…

Mesoscale and Nanoscale Physics · Physics 2015-06-25 D. Klauser , W. A. Coish , Daniel Loss

The hyperpolarization of nuclear spins can enable powerful imaging and sensing techniques provided the hyperpolarization is sufficiently long-lived. Recent experiments on nanodiamond $^{13}$C nuclear spins demonstrate that relaxation times…

Mesoscale and Nanoscale Physics · Physics 2024-02-20 Gargee Sharma , Torsten Gaebel , Ewa Rej , David J. Reilly , Sophia E. Economou , Edwin Barnes

We investigate the dynamic nuclear polarization from the hyperfine interaction between nonequilibrium electronic spins and nuclear spins coupled to them in semiconductor nanostructures. We derive the time and position dependence of the…

Materials Science · Physics 2007-05-23 Ionel Tifrea , Michael E. Flatte

Dynamic nuclear polarisation (DNP) refers to a class of techniques used to increase the signal in nuclear magnetic resonance measurements by transferring spin polarisation from ensembles of highly polarised electrons to target nuclear…

Quantum Physics · Physics 2020-12-24 L. T. Hall , D. A. Broadway , A. Stacey , D. A. Simpson , J-P. Tetienne , L. C. L. Hollenberg

Dynamical nuclear polarisation (DNP) is an important technique that uses polarisation transfer from electron to nuclear spins to achieve nuclear hyperpolarisation. As the electron spin of the nitrogen vacancy (NV) centres in diamond can be…

Non-equilibrium dynamics of many-body systems is important in many branches of science, such as condensed matter, quantum chemistry, and ultracold atoms. Here we report the experimental observation of a phase transition of the quantum…

Quantum Physics · Physics 2015-09-24 Gonzalo A. Alvarez , Dieter Suter , Robin Kaiser

We have demonstrated experimentally the manipulation of exciton and nuclear spins in a single self-assembled In$_{0.75}$Al$_{0.25}$As/Al$_{0.3}$Ga$_{0.7}$As quantum dot. The oscillation of exciton and nuclear spin polarizations were clearly…

Other Condensed Matter · Physics 2007-05-23 H. Sasakura , S. Adachi , S. Muto , S. Hirose , H. Z. Song , M. Takatsu

For applications of solid state quantum computing and quantum simulations, high fidelity initialisation of thermally mixed electronic and nuclear spin qubits is essential. Whereas electronic spins can readily be initialised optically to…

Quantum Physics · Physics 2024-04-12 O. T. Whaites , T. S. Monteiro

Hyperfine coupling of electron spins to nuclear spins is studied for a GaAs-based double quantum dot in the spin blockade regime where the electron conduction is mostly blocked by Pauli effect unless the electron spin state in the double…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Keiji Ono , Seigo Tarucha

Dynamic Nuclear Polarization (DNP) has revolutionized the field of solid-state NMR spectroscopy by significantly enhancing the sensitivity of nuclear magnetic resonance experiments. Conventionally, cross effect DNP relies on biradicals to…

Chemical Physics · Physics 2023-09-28 Amaria Javed , Asif Equbal

We review recent theoretical and experimental advances toward understanding the effects of nuclear spins in confined nanostructures. These systems, which include quantum dots, defect centers, and molecular magnets, are particularly…

Mesoscale and Nanoscale Physics · Physics 2009-09-15 W. A. Coish , J. Baugh

In III-V semiconductor nano-structures the electron and nuclear spin dynamics are strongly coupled. Both spin systems can be controlled optically. The nuclear spin dynamics is widely studied, but little is known about the initialization…

Mesoscale and Nanoscale Physics · Physics 2018-04-05 M. Manca , G. Wang , T. Kuroda , S. Shree , A. Balocchi , P. Renucci , X. Marie , M. V. Durnev , M. M. Glazov , K. Sakoda , T. Mano , T. Amand , B. Urbaszek
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