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Reverse Monte Carlo modeling of liquid water, based on one neutron and one X-ray diffraction data set, applying also the most popular interatomic potential for water, SPC/E, has been performed. The strictly rigid geometry of SPC/E water…

Soft Condensed Matter · Physics 2017-02-16 Ildikó Pethes , László Pusztai

There are various routes for deriving partial radial distribution functions of disordered systems from experimental diffraction (and/or EXAFS) data. Due to limitations and errors of experimental data, as well as to imperfections of the…

Disordered Systems and Neural Networks · Physics 2012-07-16 Z. Steinczinger , L. Pusztai

In order to reveal the atomic level structure of liquid carbon tetrabromide, a new synchrotron x-ray diffraction measurement, over a wide momentum transfer (Q-)range, has been performed. These x-ray data have been interpreted together with…

Materials Science · Physics 2014-07-02 László Temleitner

(short version) Accurate determination of the coherent static structure factor of disordered materials containing proton nuclei is prohibitively difficult by neutron diffraction, due to the large incoherent cross section of $^1$H. This…

Soft Condensed Matter · Physics 2021-01-28 László Temleitner , Anne Stunault , Gabriel Cuello , László Pusztai

Synchrotron X-ray diffraction measurements have been conducted on liquid phosphorus trichloride, tribromide and triiodide. Molecular Dynamics simulations for these molecular liquids were performed with a dual purpose: (1) to establish…

Disordered Systems and Neural Networks · Physics 2014-02-06 Szilvia Pothoczki , László Temleitner , László Pusztai

The past decade or so has witnessed a large number of articles about water structure. The most incisive experiments involve radiation with a wavelength compatible with the observed inter-molecular separations found in water, of order $\sim…

Disordered Systems and Neural Networks · Physics 2014-11-06 Alan K. Soper

The design of moderators and cold sources of neutrons is a key point in research-reactor physics, requiring extensive knowledge of the scattering properties of very important light molecular liquids such as methane, hydrogen and their…

Other Condensed Matter · Physics 2021-04-13 Eleonora Guarini

Methanol-water liquid mixtures have been investigated by high-energy synchrotron X-ray and neutron diffraction at low temperatures. We are thus able to report the first complete sets of both X-ray and neutron weighted total scattering…

Simulation (molecular dynamics and Car-Parrinello [Phys. Rev. Lett. 55, 2471 (1985)]) and diffraction (x-ray and neutron) studies on nitromethane are compared aiming at the determination of the liquid structure. Beyond that, the…

Soft Condensed Matter · Physics 2017-02-07 Tünde Megyes , Szabolcs Bálint , Tamás Grósz , Tamás Radnai , Imre Bakó , László Almásy

Intermolecular correlations in liquid acetonitrile (CH3CN) have been revisited by calculating orientational correlation functions. In the present approach, hydrogen atoms are included, so that a concept applicable for molecules of (nearly)…

Chemical Physics · Physics 2019-06-12 Szilvia Pothoczki , László Pusztai

Two different Reverse Monte Carlo strategies, 'RMC++' and 'RMCPOW', have been compared for determining the microscopic structure of some liquid and amorphous solid systems on the basis of neutron diffraction measurements. The first, '$g(r)$…

Soft Condensed Matter · Physics 2015-01-27 V. Sánchez-Gil , E. G. Noya , L. Temleitner , L. Pusztai

We simulate liquid water between hydrophobic walls separated by 0.5 nm, to study how the diffusion constant D_\parallel parallel to the walls depends on the microscopic structure of water. At low temperature T, water diffusion can be…

Soft Condensed Matter · Physics 2015-05-30 Francisco de los Santos , Giancarlo Franzese

Despite a recent flurry of experimental and simulation studies, an accurate estimate of the interaction strength of water molecules with hexagonal boron nitride is lacking. Here we report quantum Monte Carlo results for the adsorption of a…

Monte Carlo computer simulations in the canonical and grand canonical statistical ensemble were used to explore the properties of the central force (CF1) water model. The intramolecular structure of the H$_2$O molecule is well reproduced by…

Soft Condensed Matter · Physics 2021-10-12 V. Ravnik , B. Hribar-Lee , O. Pizio , M. Luksic

Isotopic substitution, which can be realized both in experiment and computer simulations, is a direct approach to assess the role of nuclear quantum effects on the structure and dynamics of matter. Yet, the impact of nuclear quantum effects…

Chemical Physics · Physics 2024-12-03 Nore Stolte , János Daru , Harald Forbert , Jörg Behler , Dominik Marx

A Monte Carlo model was used to study the scattering error of an absorption meter with a divergent light beam and a limited acceptance angle of the receiver. Reflections at both ends of the tube were taken into account. Calculations of the…

Atmospheric and Oceanic Physics · Physics 2009-11-06 Jacek Piskozub , Piotr J. Flatau , J. V. R. Zaneveld

A recent paper by Zeidler et al. (PRL 107, 144501 (2011)) describes a neutron scattering experiment on water in which oxygen isotope substitution is successfully achieved for the first time. Differences between scattering patterns with…

Chemical Physics · Physics 2015-06-03 A. K. Soper , C. J. Benmore

We present an inelastic neutron scattering study of liquid and solid hydrogen carried out using the wide Angular Range Chopper Spectrometer at Oak Ridge National Laboratory. From the observed dynamic structure factor, we obtained empirical…

Other Condensed Matter · Physics 2023-03-29 T. R. Prisk , R. T. Azuah , D. L. Abernathy , G. E. Granroth , T. E. Sherline , P. E. Sokol , J. Hu , M. Boninsegni

In this article, we report a fully ab initio variational Monte Carlo study of the linear, and periodic chain of Hydrogen atoms, a prototype system providing the simplest example of strong electronic correlation in low dimensions. In…

Strongly Correlated Electrons · Physics 2015-05-30 Lorenzo Stella , Claudio Attaccalite , Sandro Sorella , Angel Rubio

Neutron oscillation into mirror neutron, a sterile state exactly degenerate in mass with the neutron, could be a very rapid process, even faster than the neutron decay itself. It can be observed by comparing the neutron lose rates in an…

Computational Physics · Physics 2018-09-05 Riccardo Biondi
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