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We analyze the role of coherent, non-perturbative system-bath interactions in a photosynthetic heat engine. Using the reaction-coordinate formalism to describe the vibrational phonon-environment in the engine, we analyze the efficiency…

Chemical Physics · Physics 2018-09-19 Melina Wertnik , Alex Chin , Franco Nori , Neill Lambert

In this paper, we apply the polaron master equation, which offers the possibilities to interpolate between weak and strong system-bath coupling, to study how system-bath couplings affect charge transfer processes in Photosystem II reaction…

Chemical Physics · Physics 2017-08-02 M Qin , H Z Shen , X L Zhao , X X Yi

We investigate quantum heat transfer and thermal management in the nonequilibrium qubit-phonon hybrid system by applying the quantum master equation embedded with phononic coherent state. We obtain the steady state heat flow by tuning the…

Quantum Physics · Physics 2020-03-13 Chen Wang , Lu-Qin Wang , Jie Ren

A generic and intuitive model for coherent energy transport in multiple minima systems coupled to a quantum mechanical bath is shown. Using a simple spin-boson system, we illustrate how a generic donor-acceptor system can be brought into…

Biological Physics · Physics 2014-06-24 Tristan Farrow , Vlatko Vedral

Fluctuations in the energy gap and coupling constants in and between chromophores can play important role in the absorption and energy transfer across a collection of two level systems. In a noisy environment, fluctuations can control…

Chemical Physics · Physics 2024-04-17 Rajesh Dutta , Biman Bagchi

We analytically derive transfer probabilities and efficiencies for an artificial light-harvesting photosynthetic system, which consists of a ring coupled to a central acceptor. For an incident photon pair, we find near-perfect single…

Chemical Physics · Physics 2025-04-22 Stephon Alexander , Roger Andrews , Oliver Fox , Sarben Sarkar

We investigate the role of quantum coherence in the efficiency of excitation transfer in a ring-hub arrangement of interacting two-level systems, mimicking a light-harvesting antenna connected to a reaction center as it is found in natural…

Quantum Physics · Physics 2009-11-13 Alexandra Olaya-Castro , Chiu Fan Lee , Francesca Fassioli Olsen , Neil F. Johnson

We study the light absorption and energy transferring in a donor-acceptor system with a bionic structure. In the optimal case with uniform couplings, it is found that the quantum dynamics of this seemingly complicated system is reduced as a…

Biological Physics · Physics 2012-04-13 H. Dong , D. Z. Xu , C. P. Sun

We investigate multichromophoric energy transfer allowing for bath-induced fluctuations at different sites to be correlated. As a prototype system we consider a light-harvesting antenna surrounding a reaction center. We show that the…

Quantum Physics · Physics 2010-07-16 Francesca Fassioli , Ahsan Nazir , Alexandra Olaya-Castro

We investigate the quantum thermal transistor effect in nonequilibrium three-level systems by applying the polaron transformed Redfield equation combined with full counting statistics. The steady state heat currents are obtained via this…

Quantum Physics · Physics 2020-08-26 Chen Wang , Dazhi Xu

We present a theory that efficiently describes the quantum dynamics of an electronic excitation that is coupled to a continuous, highly structured phonon environment. Based on a stochastic approach to non-Markovian open quantum systems, we…

Quantum Physics · Physics 2009-11-05 Jan Roden , Alexander Eisfeld , Wolfgang Wolff , Walter T. Strunz

We present a theoretical study showing that an optically driven excitonic two-level system in a solid state environment acts as a heat pump by means of repeated phonon emission or absorption events. We derive a master equation for the…

Quantum Physics · Physics 2010-08-11 Erik M. Gauger , Joachim Wabnig

The question of how quantum coherence facilitates energy transfer has been intensively debated in the scientific community. Since natural and artificial light-harvesting units operate under the stationary condition, we address this question…

Chemical Physics · Physics 2020-07-22 Pei-Yun Yang , Jianshu Cao

To study the full counting statistics of quantum heat transfer in a driven nonequilibrium spin-boson model, we develop a generalized nonequilibrium polaron-transformed Redfield equation with an auxiliary counting field. This enables us to…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 Chen Wang , Jie Ren , Jianshu Cao

We derive an efficiency bound for continuous quantum heat engines absorbing heat from squeezed thermal reservoirs. Our approach relies on a full-counting statistics description of nonequilibrium transport and it is not limited to the…

Statistical Mechanics · Physics 2018-02-05 Bijay Kumar Agarwalla , Jian-Hua Jiang , Dvira Segal

In this work we consider a current carrying two level quantum dot(QD) that is coupled to a single mode phonon bath. Using self-consistent Hartree-Fock approximation, we obtain the I-V curve of QD. By considering the linear response of our…

Mesoscale and Nanoscale Physics · Physics 2018-06-20 Amir Eskandari-asl

Quantum heat transfer is analyzed in nonequilibrium two-qubits systems by applying the nonequilibrium polaron-transformed Redfield equation combined with full counting statistics. Steady state heat currents with weak and strong qubit-bath…

Quantum Physics · Physics 2019-03-13 Huan Liu , Chen Wang , Lu-Qing Wang , Jie Ren

The entanglement dynamics of a laser-pumped two-level quantum dot pair is investigated in the steady-state. The closely spaced two-level emitters, embedded in a semiconductor substrate, interact with both the environmental vacuum modes of…

Quantum Physics · Physics 2018-05-09 Elena Cecoi , Viorel Ciornea , Aurelian Isar , Mihai A. Macovei

Recent evidence suggests that quantum effects may have functional importance in biological light-harvesting systems. Along with delocalized electronic excitations, it is now suspected that quantum coherent interactions with certain…

Chemical Physics · Physics 2015-10-22 Nathan Killoran , Susana F. Huelga , Martin B. Plenio

We investigate the effects of a low frequency (acoustic) phonon bath on the dynamics of a quantum dot modelled as a cascade three-level system. We show that the phonon bath appears to the upper transition of the cascade system as a…

Quantum Physics · Physics 2014-08-27 Hui Huang , Gao-xiang Li , Wen-ju Gu , Zbigniew Ficek
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