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This paper discusses the important role of controllability played on the complexity of optimizing quantum mechanical control systems. The study is based on a topology analysis of the corresponding quantum control landscape, which is…

Quantum Physics · Physics 2013-04-01 Re-Bing Wu , Michael A. Hsieh , Herschel Rabitz

A controlled quantum system possesses a search landscape defined by the target physical objective as a function of the controls. This paper focuses on the landscape for the transition probability Pif between the states of a finite level…

Chemical Physics · Physics 2015-05-27 Vincent Beltrani , Jason Dominy , Tak-San Ho , Herschel Rabitz

A common goal of quantum control is to maximize a physical observable through the application of a tailored field. The observable value as a function of the field constitutes a quantum control landscape. Previous works have shown, under…

Quantum Physics · Physics 2014-03-20 Arun Nanduri , Ashley Donovan , Tak-San Ho , Herschel Rabitz

We report some improvements to the gradient ascent pulse engineering (GRAPE) algorithm for optimal control of quantum systems. These include more accurate gradients, convergence acceleration using the BFGS quasi-Newton algorithm as well as…

Quantum Physics · Physics 2014-07-16 P. de Fouquieres , S. G. Schirmer , S. J. Glaser , Ilya Kuprov

Optimization is ubiquitous in quantum information science and technology, however, the corresponding optimization landscape can encounter false traps, i.e., local but not global optima, likely to prevent used optimizers from finding optimal…

Quantum Physics · Physics 2026-03-06 Xiaozhen Ge , Shuming Cheng , Guofeng Zhang , Re-Bing Wu

Quantum optimal control experiments and simulations have successfully manipulated the dynamics of systems ranging from atoms to biomolecules. Surprisingly, these collective works indicate that the effort (i.e., the number of algorithmic…

Quantum Physics · Physics 2013-05-29 Katharine W. Moore , Herschel Rabitz

The reliable and precise generation of quantum unitary transformations is essential to the realization of a number of fundamental objectives, such as quantum control and quantum information processing. Prior work has explored the optimal…

Quantum Physics · Physics 2010-07-21 Michael Hsieh , Rebing Wu , Herschel Rabitz , Daniel Lidar

Although quantum control typically relies on greedy (local) optimization, traps (irregular critical points) in the control landscape can make optimization hard by foiling local search strategies. We demonstrate the failure of greedy…

Quantum Physics · Physics 2014-09-17 Ehsan Zahedinejad , Sophie Schirmer , Barry C. Sanders

A common goal in the sciences is optimization of an objective function by selecting control variables such that a desired outcome is achieved. This scenario can be expressed in terms of a control landscape of an objective considered as a…

Quantum Physics · Physics 2017-02-08 Benjamin Russell , Herschel Rabitz

We explore the use of policy gradient methods in reinforcement learning for quantum control via energy landscape shaping of XX-Heisenberg spin chains in a model agnostic fashion. Their performance is compared to finding controllers using…

Quantum Physics · Physics 2022-07-19 I. Khalid , C. A. Weidner , E. A. Jonckheere , S. G. Schirmer , F. C. Langbein

$\Lambda$, $V$, $\Xi$ (ladder), and other three-level quantum systems with one forbidden transition ($\Lambda$-type systems) play an important role in quantum physics. Various applications require manipulation by such systems using as…

Quantum Physics · Physics 2025-02-25 Boris Volkov , Anastasia Myachkova , Alexander Pechen

The control of quantum system dynamics is generally performed by seeking a suitable applied field. The physical objective as a functional of the field forms the quantum control landscape, whose topology, under certain conditions, has been…

Quantum Physics · Physics 2014-11-11 Arun Nanduri , Ofer M. Shir , Ashley Donovan , Tak-San Ho , Herschel Rabitz

The problems of optimizing the value of an arbitrary observable of the two-level system at both a fixed time and the shortest possible time is theoretically explored. Complete identification and classification along with comprehensive…

Quantum Physics · Physics 2016-12-02 Dmitry V. Zhdanov , Tamar Seideman

Existing algorithms for the optimal control of quantum observables are based on locally optimal steps in the space of control fields, or as in the case of genetic algorithms, operate on the basis of heuristics that do not explicitly take…

Quantum Physics · Physics 2007-08-27 Raj Chakrabarti , Rebing Wu , Herschel Rabitz

In the quest to achieve scalable quantum information processing technologies, gradient-based optimal control algorithms (e.g., GRAPE) are broadly used for implementing high-precision quantum gates, but their performance is often hindered by…

Quantum Physics · Physics 2019-01-31 Re-Bing Wu , Bing Chu , David Owens , Herschel Rabitz

Optimal control of molecular dynamics is commonly expressed from a quantum mechanical perspective. However, in most contexts the preponderance of molecular dynamics studies utilize classical mechanical models. This paper treats laser-driven…

Chemical Physics · Physics 2015-03-19 Carlee Joe-Wong , Tak-San Ho , Ruixing Long , Herschel Rabitz , Rebing Wu

We establish three tractable, jointly sufficient conditions for the control landscapes of non-linear control systems to be trap free comparable to those now well known in quantum control. In particular, our results encompass end-point…

Optimization and Control · Mathematics 2018-08-01 Benjamin Russell , Shanon Vuglar , Herschel Rabitz

Robust and high-precision quantum control is extremely important but challenging for the functionization of scalable quantum computation. In this paper, we show that this hard problem can be translated to a supervised machine learning task…

Quantum Physics · Physics 2019-04-24 Re-Bing Wu , Haijin Ding , Daoyi Dong , Xiaoting Wang

Variational Quantum Algorithms have emerged as a leading paradigm for near-term quantum computation. In such algorithms, a parameterized quantum circuit is controlled via a classical optimization method that seeks to minimize a…

Quantum Physics · Physics 2021-10-19 Javier Rivera-Dean , Patrick Huembeli , Antonio Acín , Joseph Bowles

The ability to control quantum systems is necessary for many applications of quantum technologies ranging from gate generation in quantum computation to NMR and laser control of chemical reactions. In many practical situations, the…

Quantum Physics · Physics 2024-03-21 Alexander Pechen