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Strong optical forces with minimal spontaneous emission are desired for molecular deceleration and atom interferometry applications. We report experimental benchmarking of such a stimulated optical force driven by ultrafast laser pulses. We…

Atomic Physics · Physics 2019-07-23 Xueping Long , Scarlett S. Yu , Andrew M. Jayich , Wesley C. Campbell

An all-optical method of ultrafast spin rotation is put forward to precisely manipulate the polarization of relativistic charged particle beams of leptons or ions. In particular, laser-driven dense ultrashort beams are manipulated via…

We show that a combination of a half-cycle pulse and a short nonresonant laser pulse produces a strongly enhanced postpulse orientation. Robust transients that display both efficient and long-lived orientation are obtained. The mechanism is…

Quantum Physics · Physics 2007-05-23 D. Daems , S. Guérin , D. Sugny , H. R. Jauslin

Polariton formalism is applied for studying the propagation of a probe field of light in a cloud of cold atoms influenced by two control laser beams of larger intensity. The laser beams couple resonantly three hyperfine atomic ground states…

Quantum Physics · Physics 2011-02-22 J. Ruseckas , A. Mekys , G. Juzeliunas

Molecular hydrogen ions are of metrological relevance due to the possibility of precise theoretical evaluation of their spectrum and of external-field-induced shifts. We report the results of the calculations of the rate of laser-induced…

Atomic Physics · Physics 2018-03-21 Vladimir I. Korobov , Petar Danev , Dimitar Bakalov , Stephan Schiller

Ultrashort laser pulses provide the fastest known way to switch magnetic order. Such excitation commonly creates nanometer-scale domains, even after homogeneous illumination when the position of nucleated domains is not externally defined.…

We demonstrate how dynamic Stark control (DSC) can be achieved on molecular photodissociation in the dipole limit, using single-cycle (FWHM) laser pulses in the terahertz (THz) regime. As the laser-molecule interaction follows the…

Chemical Physics · Physics 2020-03-25 A. Tóth , A. Csehi , G. J. Halász , Á. Vibók

The treatment of the previous paper is extended to molecular wires. Specifically, the effect of electron-vibrational interactions on the electronic transport induced by femtosecond $\omega+2\omega$ laser fields along unbiased molecular…

Quantum Physics · Physics 2009-11-13 Ignacio Franco , Moshe Shapiro , Paul Brumer

We numerically investigate the dynamics of multiply charged hydrogenic ions in near-optical linearly polarized laser fields with intensities of order 10^16 to 10^17 W/cm^2. Depending on the charge state Z of the ion the relation of strength…

Quantum Physics · Physics 2009-11-06 S. X. Hu , C. H. Keitel

For photo-dissociation of a single hydrogen molecule (H2) with combined XUV and IR laser pulses, we demonstrate optical control of the emission direction of the photoelectron with respect to the outgoing neutral fragment (the H-atom).…

The control of solute fluxes through either microscopic phoresis or hydrodynamic advection is a fundamental way to transport molecules, which are ubiquitously present in nature and technology. We study the transport of large solute such as…

Soft Condensed Matter · Physics 2021-09-29 Tatsuya Fukuyama , Sho Nakama , Yusuke T. Maeda

We observe momentum transfer in the ponderomotive potential of near-infrared (NIR) laser pulses in time- and angle-resolved photoemission spectroscopy (tr-ARPES) experiments with ultrashort extreme ultraviolet probe pulses. Acceleration of…

Mesoscale and Nanoscale Physics · Physics 2025-07-08 Xinwei Zheng , Martin Weinelt , Christian Strüber

Non-monotonous changes in velocity autocorrelations across the transformation from molecular to atomic fluid in hydrogen under pressure are studied by ab initio molecular dynamics simulations at the temperature 2500 K. We report diffusion…

Soft Condensed Matter · Physics 2020-05-27 G. Ruocco , T. Bryk , C. Pierleoni , A. P. Seitsonen

We introduce a new scheme for controlling the sense of molecular rotation. By varying the polarization and the delay between two ultrashort laser pulses, we induce unidirectional molecular rotation, thereby forcing the molecules to rotate…

Quantum Physics · Physics 2015-05-13 Sharly Fleischer , Yuri Khodorkovsky , Yehiam Prior , Ilya Sh. Averbukh

A theoretical comparison of the electronic excitation and ionisation behaviour of molecular hydrogen oriented either parallel or perpendicular to a linear polarised laser pulse is performed. The investigation is based on a non-perturbative…

Quantum Physics · Physics 2009-11-13 Yulian V. Vanne , Alejandro Saenz

Excited state hydrogen transfer (ESHT) is responsible to various photochemical processes of aromatics including photoprotection of nuclear basis. Its mechanism is explained by the internal conversion from aromatic $\pi$$\pi$* to…

Atomic and Molecular Clusters · Physics 2017-12-06 Mitsuhiko Miyazaki , Ryuhei Ohara , Claude Dedonder , Christophe Jouvet , Masaaki Fujii

The absorption of traveling photons resonant with electric dipole transitions of an atomic gas naturally leads to electric dipole spin wave excitations. For a number of applications, it would be highly desirable to shape and coherently…

Atomic Physics · Physics 2021-01-04 Yizun He , Lingjing Ji , Yuzhuo Wang , Liyang Qiu , Jian Zhao , Yudi Ma , Xing Huang , Saijun Wu , Darrick E. Chang

We study the manipulation of slow light with an orbital angular momentum propagating in a cloud of cold atoms. Atoms are affected by four copropagating control laser beams in a double tripod configuration of the atomic energy levels…

Quantum Physics · Physics 2013-06-10 J. Ruseckas , V. Kudriasov , I. A. Yu , G. Juzeliunas

The control of ultrafast molecular rotational motion has benefited from the development of innovative techniques in strong-field laser physics. Here, we theoretically demonstrate a novel type of coherent control by inducing rotation of an…

Chemical Physics · Physics 2018-08-27 Alec Owens , Andrey Yachmenev , Jochen Küpper