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Related papers: Calculation of P,T-odd interaction constant of PbF…

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The scalar-pseudoscalar interaction constant of PbF in its ground state electronic configuration is calculated using the Z-vector method in the relativistic coupled-cluster framework. The precise calculated value is very important to set…

Atomic Physics · Physics 2017-06-29 Sudip Sasmal , Kaushik Talukdar , Malaya K. Nayak , Nayana Vaval , Sourav Pal

Ab initio calculation of the hyperfine, P-odd, and P,T-odd constants for the YbF molecule was performed with the help of the recently developed technique, which allows to take into account correlations and polarization in the outercore…

Atomic Physics · Physics 2015-06-26 N. S. Mosyagin , M. G. Kozlov , A. V. Titov

We report ab initio correlated relativistic calculations of the effective electric field W_d acting on the electron in two excited electronic states of PbO, required for extracting the electric dipole moment of the electron from an ongoing…

Atomic Physics · Physics 2009-11-10 T. A. Isaev , A. N. Petrov , N. S. Mosyagin , A. V. Titov , E. Eliav , U. Kaldor

We report the first results of ab initio relativistic correlation calculation of the effective electric field on the electron, E_eff, in the ground state of the HI$^+$ cation. This value is required for interpretation of the suggested…

Atomic Physics · Physics 2013-05-29 T. A. Isaev , N. S. Mosyagin , A. N. Petrov , A. V. Titov

We report ab initio relativistic correlation calculations of potential curves and spectroscopic constants for four lowest-lying electronic states of the lead monofluoride. We also calculated parameters of the spin-rotational Hamiltonian for…

Atomic Physics · Physics 2013-05-29 K. I. Baklanov , A. N. Petrov , A. V. Titov , M. G. Kozlov

The molecular dipole moment and magnetic hyperfine structure constant demand an accurate wavefunction far from the nucleus and in near nuclear region, respectively. We, therefore, employ the so-called Z-vector method in the domain of…

Chemical Physics · Physics 2015-03-31 Sudip Sasmal , Himadri Pathak , Malaya K. Nayak , Nayana Vaval , Sourav Pal

A method and codes for two-step correlation calculation of heavy-atom molecules have been developed, employing the generalized relativistic effective core potential and relativistic coupled cluster (RCC) methods at the first step, followed…

Chemical Physics · Physics 2009-11-07 A. N. Petrov , N. S. Mosyagin , T. A. Isaev , A. V. Titov , V. F. Ezhov , E. Eliav , U. Kaldor

We report results of ab initio calculation of the spin-rotational Hamiltonian parameters including P- and P,T-odd terms for the BaF molecule. The ground state wave function of BaF molecule is found with the help of the Relativistic…

Atomic Physics · Physics 2009-10-30 M. Kozlov , A. Titov , N. Mosyagin , P. Souchko

We have employed both Z-vector method and the expectation value approach in the relativistic coupled-cluster framework to calculate the scalar-pseudoscalar (S-PS) P, T -odd interaction constant (W_s) and the effective electric field (Eeff)…

Atomic Physics · Physics 2016-06-15 Sudip Sasmal , Himadri Pathak , Malaya K. Nayak , Nayana Vaval , Sourav Pal

BaF is one of the potential candidates for the experimental search of the electric dipole moment of the electron (eEDM). The NL-eEDM collaboration is building a new experimental set up to measure the eEDM using the BaF molecule [The NL-eEDM…

Chemical Physics · Physics 2020-06-24 Kaushik Talukdar , Malaya K. Nayak , Nayana Vaval , Sourav Pal

Heavy polar diatomic molecules are currently among the most promising probes of fundamental physics. Constraining the electric dipole moment of the electron (eEDM), in order to explore physics beyond the Standard Model, requires a synergy…

Atomic Physics · Physics 2018-04-18 M Abe , V S Prasannaa , B P Das

The relativistic coupled-clusters method combined with the generalized relativistic effective core potential approach and nonvariational one-center restoration technique is applied to evaluation of parameters of spin-rotational effective…

Atomic Physics · Physics 2014-12-22 L. V. Skripnikov , A. D. Kudashov , A. N. Petrov , A. V. Titov

The combined all-electron and two-step approach is applied to calculate the molecular parameters which are required to interpret the ongoing experiment to search for the effects of manifestation of the T,P-odd fundamental interactions in…

Atomic Physics · Physics 2017-07-14 L. V. Skripnikov

We employ the $Z$-vector method in the four-component relativistic coupled-cluster framework to calculate the parity (${\mathcal{P}}$) and time-reversal (${\mathcal{T}}$) symmetry violating scalar-pseudoscalar (S-PS) nucleus-electron…

Atomic Physics · Physics 2019-03-27 Kaushik Talukdar , Malaya K. Nayak , Nayana Vaval , Sourav Pal

A quasi-relativistic two-component approach for an efficient calculation of $\mathcal{P,T}$-odd interactions caused by a permanent electric dipole moment of the electron (eEDM) is presented. The approach uses a (two-component) complex…

Chemical Physics · Physics 2023-12-19 Konstantin Gaul , Robert Berger

Electric dipole moments of diamagnetic atoms of experimental interest are calculated using the relativistic Hartree-Fock and random-phase approximation methods, the many-body perturbation theory and configuration interaction technique. We…

Atomic Physics · Physics 2009-10-12 V. A. Dzuba , V. V. Flambaum , S. G. Porsev

Recently the Eu$_{0.5}$Ba$_{0.5}$TiO$_{3}$ solid was suggested as a promising candidate for experimental search of the electron electric dipole moment. To interpret the results of this experiment one should calculate the effective electric…

Atomic Physics · Physics 2015-01-13 L V Skripnikov , A V Titov , A N Petrov , N S Mosyagin , O P Sushkov

An accurate determination of the effective electric field (Eeff) in YbF is important, as it can be combined with the results of future experiments to give an improved new limit for the electric dipole moment of the electron. We report a…

Atomic Physics · Physics 2015-06-19 M. Abe , G. Gopakumar , M. Hada , B. P. Das , H. Tatewaki , D. Mukherjee

A recently implemented relativistic four-component configuration interaction approach to study ${\cal{P}}$- and ${\cal{T}}$-odd interaction constants in atoms and molecules is employed to determine the electron electric dipole moment…

Atomic Physics · Physics 2014-04-02 Timo Fleig , Malaya K. Nayak

The magnetic dipole and electric quadrupole hyperfine constants of Aluminium ($^{27}Al$) atom are computed using the relativistic coupled cluster (CC) and unitary coupled cluster (UCC) methods. Effects of electron correlations are…

Atomic Physics · Physics 2007-05-23 Chiranjib Sur , Rajat K. Chaudhuri , B. P. Das , D. Mukherjee
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