Related papers: Mid-Infrared Optical Frequency Combs based on Diff…
Historically, there has been a trade-off in spectroscopic measurements between high spectral resolution, broadband coverage, and acquisition time. Optical frequency combs, initially envisioned for precision spectroscopy of the hydrogen atom…
Optical frequency combs provide equidistant frequency markers in the infrared, visible and ultra-violet and can link an unknown optical frequency to a radio or microwave frequency reference. Since their inception frequency combs have…
We characterize a new mid-infrared frequency comb generator based on difference frequency generation around 3.2 microns. High power per comb mode (>10-7 W/mode) is obtained over a broad spectral span (>700 nm). The source is used for direct…
Dual-comb spectroscopy has demonstrated remarkable capabilities for rapid and sensitive measurements; however, significant challenges still exist in generating high-power, mutually coherent mid-infrared combs. Here we demonstrate that a…
We report on a mid-infrared frequency comb source of unprecedented tunability covering the entire 3-10 {\mu}m molecular fingerprint region. The system is based on difference frequency generation in a GaSe crystal pumped by a 151 MHz…
Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct…
Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…
An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…
Mid-infrared (mid-IR) frequency combs have broad applications in molecular spectroscopy and chemical/biological sensing. Recently developed microresonator-based combs in this wavelength regime could enable portable and robust devices using…
Mid-infrared (mid-IR) spectroscopy offers unparalleled sensitivity for the detection of trace gases, solids and liquids, which is based on the existence of strong telltale vibrational bands in this part of the spectrum. It was shown more…
Long-wavelength mid-infrared frequency combs with high power and flexible tunability are highly desired for molecular spectroscopy, including investigation of large molecules such as C60. We present a high power, phase-stabilized frequency…
The potential of frequency comb spectroscopy has aroused great interest in generating mid-infrared frequency combs in the integrated photonic setting. However, despite remarkable progress in microresonators and quantum cascade lasers, the…
Dual-comb spectroscopy is emerging as one of the most appealing applications of mid-infrared frequency combs for high-resolution molecular spectroscopy, as it leverages on the unique coherence properties of frequency combs combined with the…
Dual-comb spectroscopy is a powerful technique to measure optical spectra in a wide spectral range with high-frequency resolution. The development of compact systems operating in the long-wave infrared wavelength range is of high interest…
A mid-Infrared frequency comb is produced via an optical parametric oscillator (OPO) pumped by an amplified 100 MHz Yb:fiber mode-locked laser. We use this source to make measurements of the concentration of the atmospherically-relevant…
High resolution and fast detection of molecular vibrational absorption is important for organic synthesis, pharmaceutical process and environmental monitoring, and is enabled by mid-infrared (mid-IR) laser frequency combs via dual-comb…
Mid-wave infrared (MIR, 3--5 $\mu$m) optical frequency combs (OFC) are of critical importance for spectroscopy of fundamental molecular absorption features in space and terrestrial applications. Although in this band OFCs can be obtained…
A compact and robust coherent laser light source that provides spectral coverage from the ultraviolet to infrared is desirable for numerous applications, including heterodyne super resolution imaging[1], broadband infrared microscopy[2],…
Powerful and efficient optical frequency combs in the mid-infrared (MIR) spectral region are highly desirable for a broad range of applications. Despite extensive efforts utilizing various techniques, MIR frequency comb sources are still…
Four wave mixing (FWM) is an important way to generate supercontinuum and frequency combs in the mid-infrared band. Here, we obtain simultaneous synthetic FWM in the visible and mid-infrared bands by cascading quadratic nonlinear processes…