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We explore the effects of correlation on the ground-state energies and on photoionization dynamics in atomic Be and Ne. We apply the time-dependent restricted-active-space self-consistent-field method for several excitation schemes and…

Atomic Physics · Physics 2019-03-27 Juan J. Omiste , Lars Bojer Madsen

Methods for estimating the correlation energy of molecules and other electronic systems are discussed based on the assumption that the correlation energy can be partitioned between atomic regions. In one method, the electron density is…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

Most treatments of electron-electron correlations in dense plasmas either ignore them entirely (random phase approximation) or neglect the role of ions (jellium approximation). In this work, we go beyond both these approximations to derive…

Plasma Physics · Physics 2020-02-05 Nathaniel R. Shaffer , Charles E. Starrett

This study investigates the interplay between relativistic effects and electron correlation effects on the first ionization energies of heavy atoms (Au through Rn, Z = 79-86). We perform two complementary analyses: (1) comparing…

Atomic Physics · Physics 2026-02-06 Mohamed Kahil , Fatima Fakih , Nabil Joudieh , Nidal Chamoun

We demonstrate the control of electron-electron correlation in frustrated double ionization (FDI) of the two-electron triatomic molecule D$_{3}^{+}$ when driven by two orthogonally polarized two-color laser fields. We employ a…

Atomic Physics · Physics 2017-09-13 A. Chen , M. F. Kling , A. Emmanouilidou

Electron-electron interactions and correlations form the basis of difficulties encountered in the theoretical solution of problems dealing with multi-electron systems. Accurate treatment of the electron-electron problem is likely to unravel…

Quantum Physics · Physics 2022-03-24 E. O. Jobunga

Molecules show a much increased multiple ionization rate in a strong laser field as compared to atoms of similar ionization energy. A widely accepted model attributes this to the action of the joint fields of the adjacent ionic core and the…

Atomic Physics · Physics 2013-05-16 J. Wu , M. Meckel , L. Ph. H. Schmidt , M. Kunitski , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

We investigate the orientation dependence of Enhanced Ionization (EI) during strong-field-driven nuclear motion in acetylene (C$_2$H$_2$). Here, we both initiate and probe molecular dynamics in acetylene with intense 6-fs cross-polarized…

Atomic Physics · Physics 2024-11-08 S. A. Mohideen , A. J. Howard , C. Cheng , I. Gabalski , A. M. Ghrist , E. Weckwerth , P. H. Bucksbaum

A systematic QED treatment of electron correlation is presented for ions along the lithium isoelectronic sequence. We start with the zeroth-order approximation that accounts for a part of the electron-electron interaction by a local model…

Atomic Physics · Physics 2009-11-13 V. A. Yerokhin , A. N. Artemyev , V. M. Shabaev

We develop an analytical model of correlated two-electron ionization in strong infrared laser fields. The model includes all relevant interactions between the electrons, the laser field, and the ionic core nonperturbatively. We focus on the…

Atomic Physics · Physics 2009-02-14 Denys I. Bondar , Wing-Ki Liu , Misha Yu. Ivanov

In dense stars the nuclear reaction rates are influenced by screening effects arising from both ions and electrons. In this paper we calculate the enhancement factors due to electron polarization in the high-density, degenerate and…

Astrophysics · Physics 2009-10-30 Mikael Sahrling , Gilles Chabrier

We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort XUV pulses with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio…

Electron-electron correlation forms the basis of difficulties encountered in many-body problems. Accurate treatment of the correlation problem is likely to unravel some nice physical properties of matter embedded in this correlation. In an…

Quantum Physics · Physics 2022-03-24 Eric Ouma Jobunga

We examine the effects of electron-electron interactions on transport between edge states in a multilayer integer quantum Hall system. The edge states of such a system, coupled by interlayer tunneling, form a two-dimensional, chiral metal…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. W. Tomlinson , J. -S. Caux , J. T. Chalker

The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation,…

Entanglement engineering plays a central role in quantum-enhanced technologies, with potential physical platforms that outperform their classical counterparts. However, free electrons remain largely unexplored despite their great capacity…

Quantum Physics · Physics 2020-11-12 Shahaf Asban , Javier García de Abajo

The paper presents results and discussion of electron dynamics in molecules in which intense ultrafast pulse drives multiphoton ionization, high harmonic generation, and charge resonance due to the Rabbi flopping in the regime of Charge…

Atomic Physics · Physics 2025-08-15 L. Bauerle , A. Jaron

With a semiclassical quasi-static model we achieve an insight into the complex dynamics of two correlated electrons under the combined influence of a two-center Coulomb potential and an intense laser field. The model calculation is able to…

Atomic and Molecular Clusters · Physics 2009-11-13 J. Liu , D. F. Ye , J. Chen , X. liu

We analyze the electronic correlation contribution to the time delay in the photo-ionization of the excited ortho- and para-Helium states. A simple estimation, based on the ionization probability amplitudes, shows that the different form of…

Atomic Physics · Physics 2024-03-21 Pedro Sancho

The electric double layer (EDL) that forms at the interface between metals and ionic solutions is at the heart of various energy technologies. Recent experimental data have challenged our traditional understanding of the EDL charging…

Statistical Mechanics · Physics 2026-03-05 Nils Bruch , Michael Eikerling , Tobias Binninger