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Temperature dependent EPR studies were performed on a single crystal of CuSiO3.This recently discovered compound is isostructural with the spin-Peierls compound CuGeO3. The EPR signals show different characteristics than those of CuGeO3 and…

Strongly Correlated Electrons · Physics 2007-05-23 J. Sichelschmidt , A. Loidl , M. Baenitz , H. H. Otto , C. Geibel , F. Steglich

We have performed a powder neutron diffraction study on CsO$_2$, where the unpaired electron with $s=1/2$ in the $\pi^*$ orbital of the O$_2^-$ ion is responsible for the magnetism. The magnetic reflections 0 $\frac{1}{2}$ 0 and 0…

Strongly Correlated Electrons · Physics 2023-09-07 Takehito Nakano , Shun Kontani , Masatoshi Hiraishi , Kaito Mita , Mizuki Miyajima , Takashi Kambe

We discuss universal features on the electron spin resonance (ESR) of a temperature-induced Tomonaga-Luttinger liquid phase in a wide class of weakly coupled $S=1/2$ antiferromagnetic spin chains such as spin ladders, spin tubes and…

Strongly Correlated Electrons · Physics 2015-02-12 Shunsuke C. Furuya , Masahiro Sato

Magnetic excitations of the exchange-dipole quasi 1D XXZ antiferromagnet are studied in the ordered phase. We observe a transformation of the electron spin resonance (ESR) spectrum when crossing the N\'{e}el temperature near 0.2 K. The…

Strongly Correlated Electrons · Physics 2025-09-18 T. A. Soldatov , A. I. Smirnov

Alkali superoxide CsO2 is one of candidates for the spin-1/2 one-dimensional (1D) antiferromagnet, which may be sequentially caused by an ordering of the pi-orbital of O2- molecule below TS ~ 70 K. Here, we report on the magnetism in powder…

We present the magnetic phase diagram of a spin-1/2 chain antiferromagnet Sr$_2$CuO$_3$ studied by ultrasound phase-sensitive detection technique. We observe an enhanced effect of external magnetic field on the ordering temperature of the…

Strongly Correlated Electrons · Physics 2020-05-20 E. G. Sergeicheva , S. S. Sosin , D. I. Gorbunov , S. Zherlitsyn , G. Gu , I. Zaliznyak

Alkali superoxides differ from conventional transition metal magnets, exhibit magnetism from partially occupied oxygen molecular $\pi^*$-orbitals. Among them, CsO$_2$ stands out for its potential to exhibit novel quantum collective…

Strongly Correlated Electrons · Physics 2024-11-12 Ryota Ono , Ravi Kaushik , Sergey Artyukhin , Martin Jansen , Igor Solovyev , Russell A. Ewings

We report Electron Paramagnetic Resonance measurements on single crystalline and powder samples of Nd_0.5Ca_0.5MnO_3 across the charge-ordering transition at T_co=240 K down to the antiferromagnetic ordering transition at T_N = 140 K. The…

Strongly Correlated Electrons · Physics 2021-05-26 Janhavi P. Joshi , Rajeev Gupta , A. K. Sood , S. V. Bhat , A. R. Raju , C. N. R. Rao

Elastic and inelastic neutron scattering were used to study the ordered phase of the quasi-one-dimensional spin-1/2 antiferromagnet ${\rm BaCu_{2}Si_{2}O_{7}}$. The previously proposed model for the low-temperature magnetic structure was…

Strongly Correlated Electrons · Physics 2016-08-15 M. Kenzelmann , A. Zheludev , S. Raymond , E. Ressouche , T. Masuda , P. Böni , K. Kakurai , I. Tsukada , K. Uchinokura , R. Coldea

Cu(C$_8$H$_6$N$_2$)Cl$_2$, a strong-rung spin-1/2 Heisenberg ladder compound, is probed by means of electron spin resonance (ESR) spectroscopy in the field-induced gapless phase above $H_{c1}$. The temperature dependence of the ESR…

Strongly Correlated Electrons · Physics 2016-04-19 A. N. Ponomaryov , M. Ozerov , L. Zviagina , J. Wosnitza , K. Yu. Povarov , F. Xiao , A. Zheludev , C. Landee , E. Čižmár , A. A. Zvyagin , S. A. Zvyagin

Akali superoxides AO2 (A=Na, K, Rb, Cs), due to an open p shell of the oxygen ion O2^- with degenerate pi orbitals, have spin and orbital degrees of freedom. The complex magnetic, orbital, and structural phase transitions observed…

Strongly Correlated Electrons · Physics 2024-06-11 Kohei Shibata , Makoto Naka , Harald O. Jeschke , Junya Otsuki

The ESR (Electron Spin Resonance) spectrum of the XXZ spin chain with finite length shows a double-peak structure at high temperatures around the EPR (Electron Paramagnetic Resonance) resonance frequency. This fact has been pointed out by…

Statistical Mechanics · Physics 2017-01-11 Hiroki Ikeuchi , Hans De Raedt , Sylvain Bertaina , Seiji Miyashita

The angular and temperature dependences of single crystal ESR spectra at X-band frequency of quasi 1D spin 1/2 antiferromagnetic zigzag chain system {\beta}-TeVO4 are reported. Two resonance components in the ESR spectrum have been…

Strongly Correlated Electrons · Physics 2013-11-25 Yu. Savina , A. Bludov , V. Pashchenko , S. Gnatchenko , A. Stepanov , P. Lemmens

We present results of an electron paramagnetic resonance (EPR) study of Nd$_{1-x}$Sr$_x$MnO$_3$ with x = 0.5 across the paramagnetic to ferromagnetic, insulator to metal transition at 260 K (T$_c$) and the antiferromagnetic, charge ordering…

Strongly Correlated Electrons · Physics 2007-05-23 Janhavi P. Joshi , A. K. Sood , S. V. Bhat , A. R. Raju , C. N. R. Rao

The work is related with the finding out of magnetic phases in strongly anisotropic high-temperature superconductor Bi1,7Pb0,3Sr2Ca2Cu3O10-d in the temperature region where the superconductor is in the normal state. It was studied the…

Spin-1/2 Heisenberg antiferromagnetic frustrated spin chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is…

High-frequency ($f$ = 190 GHz) electron paramagnetic resonance (EPR) at magnetic fields up to 12 T as well as Q-band ($f$ = 34.1 GHz) EPR were performed on single crystals of the molecular wheel CsFe$_8$. In this molecule, eight Fe(III)…

Mesoscale and Nanoscale Physics · Physics 2010-09-14 Jan Dreiser , Oliver Waldmann , Graham Carver , Christopher Dobe , Hans-Ulrich Güdel , Høgni Weihe , Anne-Laure Barra

The magnetic response of antiferromagnetic CsO2, coming from the p-orbital S=1/2 spins of anionic O2- molecules, is followed by 133Cs nuclear magnetic resonance across the structural phase transition occuring at Ts1=61 K on cooling. Above…

Strongly Correlated Electrons · Physics 2018-04-16 M. Klanjsek , D. Arcon , A. Sans , P. Adler , M. Jansen , C. Felser

We have investigated the electron spin resonance (ESR) on single crystals of BaCu$\_2$Ge$\_2$O$\_7$ at temperatures between 300 and 2 K and in a large frequency band, 9.6 -134 GHz, in order to test the predictions of a recent theory,…

Strongly Correlated Electrons · Physics 2007-05-23 Sylvain Bertaina , V. A. Pashchenko , Anatoli Stepanov , T. Masuda , K. Uchinokura

We report the first electron paramagnetic resonance studies of single crystals and powders of Pr_{0.6}Ca_{0.4}MnO_{3} in the 300-4.2 K range, covering the charge ordering transition at ~ 240 K and antiferromagnetic transition (T_N) at ~ 170…

Strongly Correlated Electrons · Physics 2009-10-31 Rajeev Gupta , Janhavi P. Joshi , S. V. Bhat , A. K. Sood , C. N. R. Rao
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