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For molecules and solids containing heavy elements, accurate electronic structure calculations require accounting not only for electronic correlations but also for relativistic effects. In molecules, relativity can lead to severe changes in…

Chemical Physics · Physics 2025-10-17 Gaurav Harsha , Vibin Abraham , Dominika Zgid

An approximate relativistic two-component Hamiltonian for use in molecular electronic structure calculations is derived in the form of a sum of fixed atom-centered kinetic and spin-orbit operators added to the non-relativistic Hamiltonian.…

Chemical Physics · Physics 2019-02-13 Dimitri N. Laikov

The recursion and path-integral methods are applied to analytically study the electronic structure of a neutral $C_{60}$ molecule. We employ a tight-binding Hamiltonian which considers both the $s$ and $p$ valence electrons of carbon. From…

Materials Science · Physics 2009-10-22 Yeong-Lieh Lin , Franco Nori

The energy levels of hydrogen and helium atoms in strong magnetic fields are calculated in this study. The current work contains estimates of the binding energies of the first few low-lying states of these systems that are improvements upon…

Astrophysics · Physics 2012-02-08 Anand Thirumalai , Jeremy S. Heyl

The classical and quantum mechanics of isolated, nonlinear resonances in integrable systems with N>=2 degrees of freedom is discussed in terms of geometry in the space of action variables. Energy surfaces and frequencies are calculated and…

Chaotic Dynamics · Physics 2015-06-26 Jan Wiersig

In the present paper, first the mathematical basic properties of the exceptional points are discussed. Then, their role in the description of real physical quantum systems is considered. Most interesting value is the phase rigidity of the…

Quantum Physics · Physics 2010-11-03 Ingrid Rotter

Accurate treatment of amide resonance is important in electronic structure calculation of protein, for Resonance-Assisted Hydrogen Bonding in the hydrogen bonded chains of backbone amides of protein secondary structures such as beta sheets…

Chemical Physics · Physics 2016-10-03 John N. Sharley

Partial autoionization rates of doubly excited one-dimensional helium in the collinear Zee and eZe configuration are obtained by means of the complex rotation method. The approach presented here relies on a projection of back-rotated…

The complex-valued quantum mechanics considers quantum motion on the complex plane instead of on the real axis, and studies the variations of a particle complex position, momentum and energy along a complex trajectory. On the basis of…

Quantum Physics · Physics 2021-03-23 C. D. Yang , S. Y. Han

The main motivation for this work is the exploration of rotational-vibrational states corresponding to electronic excitations in a pre-Born-Oppenheimer quantum theory of molecules. These states are often embedded in the continuum of the…

Chemical Physics · Physics 2018-10-15 Edit Mátyus

Electron-phonon coupling (EPC) plays an important role in many fundamental physical phenomena, but the high computational cost of the EPC matrix hinders the theoretical research on them. In this paper, an analytical formula is derived to…

Computational Physics · Physics 2023-02-02 Yang Zhong , Zhiguo Tao , Weibin Chu , Xingao Gong , Hongjun Xiang

Quantum physics is generally concerned with real eigenvalues due to the unitarity of time evolution. With the introduction of $\mathcal{PT}$ symmetry, a widely accepted consensus is that, even if the Hamiltonian of the system is not…

Quantum Physics · Physics 2023-09-19 Tong Liu , Youguo Wang

We present an approach to accelerate real-space electronic structure methods several fold, without loss of accuracy, by reducing the dimension of the discrete eigenproblem that must be solved. To accomplish this, we construct an efficient,…

Computational Physics · Physics 2018-05-01 Qimen Xu , Phanish Suryanarayana , John E. Pask

Multiresolution analysis of electronic structure affords the opportunity to capture the full physics of atomic cores in a systematically improvable manner. Applying new techniques, we demonstrate for the first time that multiresolution…

Condensed Matter · Physics 2009-11-07 Torkel D. Engeness , T. A. Arias

The case of quantum-mechanical system (including electronic molecules) is considered where Hamiltonian allows a separation, in particular by the Faddeev method, of a weakly coupled channel. Width (i.e. the imaginary part) of the resonance…

Nuclear Theory · Physics 2008-02-03 V. B. Belyaev , A. K. Motovilov

In Parts I and II of this series of papers, three new methods for the computation of eigenvalues of singular pencils were developed: rank-completing perturbations, rank-projections, and augmentation. It was observed that a straightforward…

Numerical Analysis · Mathematics 2024-06-12 Michiel E. Hochstenbach , Christian Mehl , Bor Plestenjak

Hadronic resonances are unique probes that allow the properties of heavy-ion collisions to be studied. Topics that can be studied include modification of spectral shapes, in-medium energy loss of parsons, vector-meson spin alignment,…

Nuclear Experiment · Physics 2018-03-14 A. G. Knospe

We present a comprehensive investigation of electron capture (EC) ratios spanning a broad range of atomic numbers. The study employs a self-consistent computational method that incorporates electron screening, electron correlations, overlap…

Nuclear Theory · Physics 2023-07-26 V. A. Sevestrean , O. Niţescu , S. Ghinescu , S. Stoica

The projection of the eigenfunctions obtained in standard plane-wave first-principle electronic-structure calculations into atomic-orbital basis sets is proposed as a formal and practical link between the methods based on plane waves and…

Condensed Matter · Physics 2009-10-28 Daniel Sanchez-Portal , Emilio Artacho , Jose M. Soler

In this chapter we focus first on the theoretical methods and relevant computational approaches to calculate the electronic structure of atoms, molecules, and clusters containing heavy elements for which relativistic effects become…

Chemical Physics · Physics 2021-10-05 Simone Taioli , Stefano Simonucci