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The hyperfine structure of the interstitial muonium (Mu) center in rutile (TiO$_2$, weakly $n$-type) has been identified by means of muon spin rotation technique. The angle-resolved hyperfine parameter has a tetragonal anisotropy within the…

Materials Science · Physics 2015-08-19 K. Shimomura , R. Kadono , A. Koda , K. Nishiyama , M. Mihara

The electronic structure and the location of muonium centers (Mu) in single-crystalline ZnO were determined for the first time. Two species of Mu centers with extremely small hyperfine parameters have been observed below 40 K. Both Mu…

Materials Science · Physics 2009-11-07 K. Shimomura , K. Nishiyama , R. Kadono

The local electronic structure of muons (Mu) as dilute pseudo-hydrogen in single-crystalline $\beta$-Ga$_2$O$_3$ has been studied by the muon spin rotation/relaxation ($\mu$SR). High-precision measurements over a long time range of $\sim$25…

Materials Science · Physics 2023-02-01 M. Hiraishi , H. Okabe , A. Koda , R. Kadono , T. Ohsawa , N. Ohashi , K. Ide , T. Kamiya , H. Hosono

The electronic and magnetic states of $\beta$-MnO$_{2}$ in terms of hydrogen impurities have been investigated by muon spin rotation ($\mu$SR) technique combined with density-functional theory (DFT) calculations for muon as pseudo-hydrogen.…

Materials Science · Physics 2024-01-05 H. Okabe , M. Hiraishi , A. Koda , S. Takeshita , K. M. Kojima , I. Yamauchi , T. Ohsawa , N. Ohashi , H. Sato , R. Kadono

The hyperfine features and thermal stability of a muonium (Mu)-related paramagnetic center were investigated in the SrTiO$_3$ perovskite titanate via muon spin rotation spectroscopy. The hyperfine coupling tensor of the paramagnetic center…

Materials Science · Physics 2019-11-11 T. U. Ito , W. Higemoto , A. Koda , K. Shimomura

The electronic structure of interstitial hydrogen in a compound semiconductor FeS$_2$ (naturally $n$-type) is inferred from a muon study. An implanted muon (Mu, a pseudo-hydrogen) forms electronically different defect centers discerned by…

Materials Science · Physics 2018-09-05 H. Okabe , M. Hiraishi , S. Takeshita , A. Koda , K. M. Kojima , R. Kadono

A paramagnetic muonium (Mu) state with an extremely small hyperfine parameter was observed for the first time in single-crystalline GaN below 25 K. It has a highly anisotropic hyperfine structure with axial symmetry along the [0001]…

Materials Science · Physics 2009-11-10 K. Shimomura , R. Kadono , K. Ohishi , M. Mizuta , M. Saito , K. H. Chow , B. Hitti , R. L. Lichti

We present a direct spectroscopic observation of a shallow hydrogen-like muonium state in SrTiO$_3$ which confirms the theoretical prediction that interstitial hydrogen may act as a shallow donor in this material. The formation of this…

Materials Science · Physics 2014-10-14 Z. Salman , T. Prokscha , A. Amato , E. Morenzoni , R. Scheuermann , K. Sedlak , A. Suter

We report on the local electronic structure of interstitial muon (Mu) as pseudo-hydrogen in In-Ga-Zn oxide (IGZO) semiconductor studied by muon spin rotation/relaxation ($\mu$SR) experiment. In polycrystalline (c-) IGZO, it is inferred that…

Materials Science · Physics 2019-09-19 K. M. Kojima , M. Hiraishi , H. Okabe , A. Koda , 2 R. Kadono , K. Ide , S. Matsuishi , H. Kumomi , T. Kamiya , H. Hosono

We study the electronic and magnetic structure of carbon and nitrogen impurities and interstitials in rutile TiO${_2}$. To this end we perform \textit{ab-initio} calculations of a 48-atom supercell employing the VASP code. In order to…

Materials Science · Physics 2015-01-22 Jacqueline Atanelov , Christoph Gruber , Peter Mohn

With muon spin rotation ($ \mu $SR) we studied the transition between the orthorhombic antiferromagnetic (o-AF) and the tetragonal antiferromagnetic (t-AF) states of a weakly underdoped Ba$ _{1-x} $K$ _{x} $Fe$ _{2} $As$ _{2} $ single…

Superconductivity · Physics 2015-09-15 B. P. P. Mallett , Yu. G. Pashkevich , A. Gusev , Th. Wolf , C. Bernhard

It is inferred from the chemical shift of muon spin rotation ($\mu$SR) spectra that muons implanted in pristine (fully oxidized) mayenite, [Ca$_{12}$Al$_{14}$O$_{32}]^{2+}$[$\square_5$O$^{2-}$] (C12A7, with $\square$ referring to the vacant…

Materials Science · Physics 2016-03-15 M. Hiraishi , K. M. Kojima , M. Miyazaki , I. Yamauchi , H. Okabe , A. Koda , R. Kadono , S. Matsuishi , H. Hosono

The binary ruthenate, RuO$_2$, has been the subject of intense interest due to its itinerant antiferromagnetism and strain-induced superconductivity. The strain mechanism and its effect on the microscopic electronic states leading to the…

The study on the electronic state of muon as pseudo-hydrogen (represented by the elemental symbol Mu) has long been appreciated as one of the few methods to experimentally access the electronic state of dilute hydrogen (H) in semiconductors…

Materials Science · Physics 2022-09-16 M. Hiraishi , H. Okabe , A. Koda , R. Kadono , H. Hosono

Magnesium hydride has great potential as a solid hydrogen (H) storage material because of its high H storage capacity of 7.6 wt%. However, its slow hydrogenation and dehydrogenation kinetics and the high temperature of 300 $^\circ$C…

Materials Science · Physics 2023-04-25 R. Kadono , M. Hiraishi , H. Okabe , A. Koda , T. U. Ito

The hyperfine splitting of the ground and low-energy $3/2^+(7.8 \pm 0.5$ eV) levels in the $^{229}$Th nucleus in muonic atom ($\mu^-_{1S_{1/2}}{}^{229}$Th$)^*$ has been calculated considering the distribution of the nuclear magnetization in…

Nuclear Theory · Physics 2016-07-20 E. V. Tkalya

Using low-energy muons, we map the charge carrier concentration as a function of depth and electric field across the \SiOSi interface up to a depth of \SI{100}{\nano\meter} in Si-based MOS capacitors. The results show that the formation of…

Other Condensed Matter · Physics 2024-05-29 Maria M. Martins , Piyush Kumar , Marianne E. Bathen , Zaher Salman , Ulrike Grossner , Thomas Prokscha

Recently, rutile RuO$_2$ has raised interest for its itinerant antiferromagnetism, crystal Hall effect, and strain-induced superconductivity. Understanding and manipulating these properties demands resolving the electronic structure and the…

The magnetic structure of the antiferromagnetic square cupola compound Ba(TiO)Cu$_4$(PO$_4$)$_4$ with the tetragonal structure is studied with 31P nuclear magnetic resonance techniques. The magnetic hyperfine shift K shows a clear splitting…

Strongly Correlated Electrons · Physics 2020-02-19 Riho Rästa , Ivo Heinmaa , Kenta Kimura , Tsuyoshi Kimura , Raivo Stern

Recently, rutile RuO$_2$ has attracted renewed interest due to expectations of prominent altermagnetic spin-splitting. However, accumulating experimental evidence suggests that in its bulk and thick-film forms, RuO$_2$ does not display any…

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