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Controlling the coherence between light and matter has enabled the radiation of electromagnetic waves with spectral purity and stability that defines the Syst\`eme International (SI) second. While transitions between hyperfine levels in…

We studied dielectric properties of nano-sized liquid water samples confined in polymerized silicates MCM-41 characterized by the porous sizes \sim 3-10nm. We report the direct measurements of the dielectric constant by the dielectric…

Soft Condensed Matter · Physics 2015-05-27 P. O. Fedichev , L. I. Menshikov , G. S. Bordonskiy , A. O. Orlov

Terahertz time-domain spectroscopy (THz-TDS) is a non-invasive, non-contact and label-free technique for biological and chemical sensing as THz-spectra is less energetic and lies in the characteristic vibration frequency regime of proteins…

Optics · Physics 2020-07-01 Subham Adak , Laxmi Narayan Tripathi

We use near infrared spectroscopy to obtain concentration dependent glucose absorption spectra in their aqueous solutions in the near-infrared range (3800 - 7500 cm^{-1}). We introduce a new method to obtain reliable glucose absorption…

Materials Science · Physics 2013-10-03 Youngeui Jung , Jungseek Hwang

The terahertz (THz) response of solvated electrons in liquid water is studied in nonlinear ultrafast pump-probe experiments. Free electrons with concentrations from c_e = 4 to 140 \times 10-6 moles/liter are generated by high-field THz or…

Spintronic terahertz emitters promise terahertz sources with an unmatched broad frequency bandwidth that are easy to fabricate and operate, and therefore easy to scale at low cost. However, current experiments and proofs of concept rely on…

Microwave reflectometry is a non-intrusive plasma diagnostic tool which is widely applied in many fusion devices. In 2014, the microwave reflectometry on Experimental Advanced Superconducting Tokamak (EAST) had been upgraded to measure…

Instrumentation and Detectors · Physics 2016-11-17 Fei Wen , Tao Zhang , Shoubiao Zhang , Defeng Kong , Yuming Wang , Xiang Han , Hao Qu , Xiang Gao

Ultrashort time-domain spectroscopy and field-resolved spectroscopy of molecular fingerprints are gold standards for detecting samples' constituents and internal dynamics. However, they are hindered by the Nyquist criterion, leading to…

The application of tunable diode laser absorption spectroscopy (TDLAS) to flames with non-homogeneous temperature and concentration fields is an area where only few studies exist. Experimental work explores the performance of tomographic…

Optics · Physics 2014-11-26 Avishek Guha , Ingmar Schoegl

The microscopic origins of terahertz (THz) vibrational modes in biological systems are an active and open area of current research. Recent experiments [Physical Review X 8, 031061 (2018)] have revealed the presence of a pronounced mode at…

Biological Physics · Physics 2022-10-28 Khatereh Azizi , Matteo Gori , Uriel Morzan , Ali Hassanali , Philip Kurian

The ability to perform broadband optical spectroscopy with sub-diffraction-limit resolution is highly sought-after for a wide range of critical applications. However, sophisticated tip-enhanced techniques are currently required to achieve…

The reliable operation of micro and nanomechanical devices necessitates a thorough knowledge of the water film thickness present on the surfaces of these devices with an accuracy in the nm range. In this work, the thickness of an ultra-thin…

Materials Science · Physics 2007-05-23 A. Opitz , M. Scherge , S. I. -U. Ahmed , J. A. Schaefer

Time-resolved near-infrared absorption spectroscopy of single non-repeatable transient events is performed at high spectral resolution with a dual-comb interferometer using a continuous-wave laser followed by a single electro-optic…

Terahertz (THz) metamaterials have been developed for THz sensing, detection, imaging, and many other functions due to their unusual absorbers. However, the unusual absorption spectra change with different incident angles. Thus, we designed…

Optics · Physics 2022-02-28 Zhigang Li Wenjing Jiang , Jianyu Fu , Qing Zhao

We demonstrate cantilever-enhanced photoacoustic spectroscopy in the mid-infrared using a supercontinuum source. The approach is broadband, compact, and allows for higher photoacoustic signal intensity and enhanced signal-to-noise ratio as…

Instrumentation and Detectors · Physics 2018-11-14 Tommi Mikkonen , Caroline Amiot , Antti Aalto , Kim Patokoski , Goëry Genty , Juha Toivonen

We report the development of new terahertz techniques for rapidly measuring the complex Faraday angle in systems with broken time-reversal symmetry using the cyclotron resonance of a GaAs two-dimensional electron gas in a magnetic field as…

Materials Science · Physics 2015-06-03 D. K. George , A. V. Stier , C. T. Ellis , B. D. McCombe , J. Černe , A. G. Markelz

In this paper, we study the sensitivity-tunable Terahertz (THz) liquid/gas biosensor in a coupling prism-three-dimensional Dirac semimetal (3D DSM) multilayer structure. The high sensitivity of the biosensor originates from the sharp…

We present a system for molecular spectroscopy using a broadband mid-infrared laser with near infrared detection. Difference frequency generation of a Yb:fiber femtosecond laser produced a mid-infrared (MIR) source tunable from 2100-3700…

Optics · Physics 2015-05-30 Todd A. Johnson , Scott A. Diddams

Ultrafast, time-resolved spectroscopies enable the direct observation of non-equilibrium processes in condensed-phase systems and have revealed key insights into energy transport, hydrogen-bond dynamics, and vibrational coupling. While ab…

Chemical Physics · Physics 2025-09-01 Kit Joll , Philipp Schienbein

White light spectral interferometry is applied to measure the refractive index in absorbing liquids in the spectral range from 400 to 1000 nm. We analyze the influence of absorption on the visibility of interferometric fringes and,…