Related papers: New terahertz dielectric spectroscopy for the stud…
Because it is sensitive to fluctuations occurring over femtoseconds to picoseconds, gigahertz-to-terahertz dielectric relaxation spectroscopy can provide a valuable window into water's most rapid intermolecular motions. In response, we have…
Terahertz spectroscopy is a promising tool for analyzing the picosecond dynamics of biomolecules, which is influenced by surrounding water molecules. However, water causes extreme losses to terahertz signals, preventing sensitive…
Absorption spectra of liquid water at 300 K are calculated from both classical and density functional theory molecular dynamics simulation data, which together span from 1 MHz to hundreds of THz, agreeing well with experimental data…
Liquid water is one of the most studied substances, yet many of its properties are difficult to rationalize. The uniqueness of water is rooted in the dynamic network of hydrogen-bonded molecules with relaxation time constants of about one…
Ultrasensitive terahertz sensing of highly absorptive aqueous solutions remains challenging due to strong absorption of water in the terahertz regime. Here, we experimentally demonstrate a cost-effective metamaterial-based sensor integrated…
We report the first coherent excitation of intramolecular vibrational modes via the nonlinear interaction of a TeraHertz (THz) light field with molecular liquids. A terahertz-terahertz-Raman pulse sequence prepares the coherences with a…
We present a metamaterial-based terahertz (THz) sensor for thickness measurements of subwavelength-thin materials and refractometry of liquids and liquid mixtures. The sensor operates in reflection geometry and exploits the frequency shift…
The model glass-former glycerol and its aqueous mixtures were investigated with terahertz-time domain spectroscopy (THz-TDS) in the frequency range of 0.3--3.0\,THz at temperatures from 80--305\,K. It was shown that the infrared absorption…
We experimentally show the spectrally averaged nonlinear refractive index and absorption coefficient for liquid water, water vapor, {\alpha}-pinene, and Si using a full-phase analysis in the terahertz regime through a standard time-domain…
Terahertz spectrometers with a wide instantaneous frequency coverage for passive remote sensing are enormously attractive for many terahertz applications, such as astronomy, atmospheric science and security. Here we demonstrate a wide-band…
We report on the nonlinear spectroscopy of water vapor at THz frequencies. Atmospheric water vapor has a rich spectrum with several strong resonances at frequencies below 3 THz, falling within the range of operation of most existing THz…
We present the design of a continuous-wave, highly sensitive optical spectrometer for millimeter-wave frequencies between 50 and 1000 GHz. The spectrometer uses photomixing of near-infrared light to generate radiation in a wide frequency…
A novel THz near-field spectrometer is presented which allows to perform biological and medical studies with high spectral resolution combined with a spatial resolution down to l/100. In the setup an aperture much smaller than the used…
Terahertz (THz) waves have been significantly developed in the last fifteen years because of their great potential for applications in industrial and scientific communities1,2. The unique properties of THz waves as transparency for numerous…
Sub-terahertz (sub-THz) and terahertz (THz) radiation offer unique opportunities for non-invasive diagnostics and imaging due to their sensitivity to water content and molecular dynamics in biological tissues. In this work, a comprehensive…
Why does a microwave oven work? How does biological tissue absorb electromagnetic radiation? Astonishingly, we do not have a definite answer to these simple questions because the microscopic processes governing the absorption of…
We demonstrate the capabilities of a novel frequency-domain terahertz spectrometer based on a comb-locked frequency synthesizer, which provides absolute frequency calibration. The inherent stability and repeatability of the scans allow for…
In the present work, we examine the relevance and proper interpretation of broadband-dielectric and THz-spectroscopy data for the investigation of various types of biological matter. We provide an overview of the rich variety of different…
We propose using THz frequency selective surfaces interrogated with THz subwavelength optical fibers as sensors for monitoring of the optical properties of thick films that are brought in contact with such surfaces. Changes in the test film…
We present a rapid-scan, time-domain terahertz spectrometer employing femtosecond Er:fiber technology and an acousto-optic delay with attosecond precision, enabling scanning of terahertz transients over a 12.4 ps time window at a waveform…