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We have first succeefully synthesized the sodium cobalt oxyhydrate superconductors using KMnO4 as a de-intercalating and oxidizing agent. It is a novel route to form the superconductive phase of NaxCoO2.yH2O without resorting to the…

Superconductivity · Physics 2009-11-10 C. -J. Liu , C. -Y. Liao , L. -C. Huang , C. -H. Su , S. Neeleshwar , Y. -Y. Chen

We investigate mixed-valence oxide Co$_3$O$_4$ using Co $2p3d$ resonant inelastic X-ray scattering (RIXS). By setting resonant edges at Co$^{2+}$ and Co$^{3+}$ ions, the $dd$ excitations on the two Co sites are probed selectively, providing…

Ultra-high temperature ceramics (UHTCs) are promising materials for use in next-generation aerospace structures but have primarily been used as monolithic materials or coatings due to processing limitations. Here, new functionality (e.g.,…

Materials Science · Physics 2024-12-30 Catherine Ott , Vaibhav Verma , Adam Peters , Ian McCue

We obtain the electronic states and structures of two-dimensional cobalt oxides, Na$_{x}$CoO$_{2}$ (x=0, 0.35, 0.5 and 0.75) by utilizing the full-potential linear muffin-tin orbitals (FP-LMTO) methods, from which some essential electronic…

Strongly Correlated Electrons · Physics 2009-11-10 Liang-Jian Zou , J. -L. Wang , Z. Zeng

The emergence of transition metal dichalcogenides (TMD) as crystalline atomically thin semiconductors has created a tremendous amount of scientific and technological interest. Many novel device concepts have been proposed and realized…

Mesoscale and Nanoscale Physics · Physics 2020-10-19 Woojoo Lee , Yi Lin , Li-Shuan Lu , Wei-Chen Chueh , Mengke Liu , Xiaoqin Li , Wen-Hao Chang , Robert A. Kaindl , Chih-Kang Shih

CaxCu3Ti4O12 polycrystalline powders with variation in calcium content were prepared via the oxalate precursor route. The structural, morphological and dielectric properties of the ceramics fabricated using these powders were studied using…

Materials Science · Physics 2013-01-18 P. Thomas , K. Dwarakanath , K. B. R. Varma

Sr1-xMnxTiO3 (where x = 0.03, 0.05, 0.07 and 0.09) was synthesized via different routes that include solid-state, oxalate precipitation and freeze drying. In oxalate precipitation technique, compositions corresponding to 3 and 5 mol %…

Materials Science · Physics 2012-05-08 K. R. S. Preethi Meher , C. Bogicevic , Pierre-Eymeric Janolin , K. B. R. Varma

Ba2CoWO6 (BCoW) has been synthesized in polycrystalline form by solid state reaction at 1200C. Structural characterization of the compound was done through X-ray diffraction (XRD) followed by Rietveld analysis of the XRD pattern. The…

We report the synthesis, and structural and physical properties of CaFe4As3 single crystals. Needle-like single crystals of CaFe4As3 were grown out of Sn flux and the compound adopts an orthorhombic structure as determined by X-ray…

Superconductivity · Physics 2015-05-27 A. B. Karki , G. T. McCandless , S. Stadler , Y. M. Xiong , J. Li , Julia Y. Chan , R. Jin

Spin-state ordering - a periodic pattern of ions with different spin-state configurations along a crystal lattice - is a rare phenomenon, and its possible interrelation with other electronic degrees of freedom remains little explored. Here…

Strongly Correlated Electrons · Physics 2024-03-27 E. Granado , C. W. Galdino , B. D. Moreno , G. King , D. C. Freitas

In the R1/2D1/2MnO3 manganites (R: rare earth, D: divalent cation), the structural phase transition at Tco is commonly interpreted as a concomitant charge and orbital ordering (CO/OO) process driven by a cooperative Jahn-Teller effect and…

Strongly Correlated Electrons · Physics 2007-05-23 A. Daoud-Aladine , J. Rodriguez-Carvajal , L. Pinsard-Gaudart , M. T. Fernandez-Diaz , A. Revcolevschi

We report the decomposition of La2-xSrxCuO4 into La2O3 and Cu nanoparticles in ultra-high vacuum, observed by in-situ heating experiments in a transmission electron microscope (TEM). The analysis of electron diffraction data reveals that…

Inorganic oxyfluorides have significant importance in the development of new functionalities for energy production and storage, photonics, catalysis, etc. In order to explore a simple preparation route that avoids the use of toxic HF or F2…

Materials Science · Physics 2018-03-21 Daigorou Hirai , Osamu Sawai , Teppei Nunoura , Zenji Hiroi

The powder of barium titanate (BaTiO3) synthesized by solid state was characterised by spherical grains of the average size about 500 nm. The double mechanical activation and calcination of raw materials was necessary to receive the…

Materials Science · Physics 2015-08-27 Mojtaba Biglar , Magdalena Gromada , Feliks Stachowicz , Tomasz Trzepiecinski

The electronic structure of crystalline CdTe, CdO, $\alpha$-TeO$_2$, CdTeO$_3$ and Cd$_3$TeO$_6$ is studied by means of first principles calculations. The band structure, total and partial density of states, and charge densities are…

Materials Science · Physics 2009-11-10 Eduardo Ariel Menendez Proupin , Gonzalo Gutierrez , Ernesto Palmero , J. L. Peña

This study reports first synthesis of MXene-derived co-existing phases. New family of two-dimensional materials such as Ti3C2 namely MXene, having transition metal forming hexagonal structure with carbon atoms have attracted tremendous…

Mesoscale and Nanoscale Physics · Physics 2019-07-31 Mehroz Iqbal , Jameela Fatheema , Malika Rani , Ren-Kui Zheng , Saleem Ayaz Khan , Syed Rizwan

Silicon telluride (Si2Te3) is a two-dimensional semiconductor with unique structural properties due to the size contrast between Si and Te atoms. A recent experiment shows that the material turns metallic under hydrostatic pressure, while…

Materials Science · Physics 2021-01-11 Romakanta Bhattarai , Xiao Shen

We report the synthesis and superconducting properties of a metastable form of the known superconductor NaxCoO2*yH2O (x ~ 1/3, y ~ 4x). Instead of using the conventional bromine-acetonitrile mixture for sodium deintercalation, we use an…

Materials Science · Physics 2009-11-11 P. W. Barnes , M. Avdeev , J. D. Jorgensen , D. G. Hinks , H. Claus , S. Short

Substitutions of the zirconium and tin ions along with the indium-niobium and iron-niobium complexes for titanium in the barium modified NBT solid solutions impact the formation of phases in the process of the solid state synthesis and the…

Materials Science · Physics 2015-08-11 V. M. Ishchuk , L. G. Gusakova , N. G. Kisel , D. V. Kuzenko , N. A. Spiridonov , V. L. Sobolev

The dielectric properties of tantalum doped BaTi0.85Zr0.15O3 were investigated. The conventional solid state reaction method was used to make the ceramic samples. The composition was close to the pinch point of the three structure phase…

Materials Science · Physics 2007-05-23 Jun Xu , Mitsuru Itoh