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Evolutionary algorithms and the particle swarm optimization method have been used to predict stable and metastable high hydrides of iron between 150-300 GPa that have not been discussed in previous studies. Cmca FeH5, Pmma FeH6 and P2/c…

Superconductivity · Physics 2018-10-31 Niloofar Zarifi , Tiange Bi , Hanyu Liu , Eva Zurek

Hydrogen-rich hydrides attract great attention due to recent theoretical (1) and then experimental discovery of record high-temperature superconductivity in H3S (Tc = 203 K at 155 GPa (2)). Here we search for stable uranium hydrides at…

Hydrogen-rich ternary hydrides are promising candidates for high-Tc superconductivity at megabar pressures, yet their chemical space is vast and largely unexplored. Combining evolutionary structure searches with first-principles…

Following the idea that hydrogen-rich compounds might be high-T$_c$ superconductors at high pressures, and the very recent breakthrough in predicting and synthesizing hydrogen sulfide with record-high T$_c$ = 203 K, ab initio evolutionary…

Superconductivity · Physics 2017-04-19 M. M. Davari Esfahani , A. R. Oganov , H. Niu , J. Zhang

We predicted a new ternary hydride Li$_2$SiH$_6$ at high pressures. A systematic structure search in Li$_2$SiH$_6$ compound reveals novel stable phases with intriguing electronic and phonon properties. It is found that Li$_2$SiH$_6$ is…

Materials Science · Physics 2022-09-13 Sixuan Wu , Bin Li , Zhi Chen , Yu Hou , Yan Bai , Xiaofeng Hao , Yeqian Yang , Shengli Liu , Jie Cheng , Zhixiang Shi

We present a comprehensive first--principles study of the structural stability and superconducting behavior of Li$_2$PdH$_2$ under high pressure. Using random structure searching and phonon calculations, we identify a pressure--induced…

Superconductivity · Physics 2025-08-08 Zahra Alizadeh , Yue-Wen Fang , Ion Errea , M. R. Mohammadizadeh

Gas hydrates are systems of prime importance. In particular, hydrogen hydrates are potential materials of icy satellites and comets, and may be used for hydrogen storage. We explore the H2O-H2 system at pressures in the range 0-100 GPa with…

Materials Science · Physics 2014-04-01 Guang-Rui Qian , Andriy O. Lyakhov , Qiang Zhu , Artem R. Oganov , Xiao Dong

High pressure structures, phase diagram and superconductivity of polonium hydrides have been systematically investigated through the first-principles calculations based on the density functional theory. With the increasing pressure, several…

Using first-principles variable-composition evolutionary methodology, we explored the high-pressure structures of beryllium hydrides between 0 and 400 GPa. We found that BeH$_2$ remains the only stable compound in this pressure range. The…

Materials Science · Physics 2014-07-15 Shuyin Yu , Qingfeng Zeng , Artem R. Oganov , Chaohao Hu , Gilles Frapper , Litong Zhang

The discovery of the high temperature superconducting state in compounds of hydrogen, carbon and sulfur with the critical temperature (Tc) of 288 K at high pressure is an important milestone towards room-temperature superconductors. Here,…

Superconductivity · Physics 2021-07-23 Mingyang Du , Zihan Zhang , Tian Cui , Defang Duan1

In this work, global search for crystal structures of ternary Mg-Sc-H hydrides (Mg$_x$Sc$_y$H$_z$) under high pressure ($100 \le P \le 200$ GPa) were performed using the evolutionary algorithm and first-principles calculations. Based on…

We have performed ab initio calculations for new high-pressure phase of Ca-VI between 158-180 GPa. The study includes elastic parameters of mono- and poly-crystalline aggregates, electronic band structure, lattice dynamics and…

Superconductivity · Physics 2015-05-19 M. Aftabuzzaman , A. K. M. A. Islam

The search for high-temperature superconductors in hydrides under high pressure has always been a research hotspot. Hydrogen-based superconductors offer an avenue to achieve the long-sought goal of superconductivity at room temperature. We…

Superconductivity · Physics 2023-05-22 Ming Xu , Defang Duan , Wendi Zhao , Decheng An , Hao Song , Tian Cui

Recently a big number of works devoted to search for new hydrides with record high-temperature superconductivity and at the same time the successful synthesis of potential high-TC superconducting FeH5 was reported. We present a systematic…

Superconductivity · Physics 2018-02-20 Alexander G. Kvashnin , Ivan A. Kruglov , Dmitrii V. Semenok , Artem R. Oganov

The discoveries of high-temperature superconductivity in H3S and LaH10 have excited the search for superconductivity in compressed hydrides. In contrast to rapidly expanding theoretical studies, high-pressure experiments on hydride…

Superconductivity · Physics 2021-09-15 Wuhao Chen , Dmitrii V. Semenok , Xiaoli Huang , Haiyun Shu , Xin Li , Defang Duan , Tian Cui , Artem R. Oganov

The dependence of the superconducting transition temperature T_{c} on nearly hydrostatic pressure has been determined to 67 GPa in an ac susceptibility measurement for a Li sample embedded in helium pressure medium. With increasing…

Superconductivity · Physics 2009-11-10 Shanti Deemyad , James S. Schilling

Gas hydrates are considered fundamental building blocks of giant icy planets like Neptune and similar exoplanets. The existence of these materials in the interiors of giant icy planets, which are subject to high pressures and temperatures,…

Evolutionary structure searches are used to predict stable phases with unique stoichiometries in the hydrogen-rich region of the magnesium/hydrogen phase diagram under pressure. MgH$_4$, MgH$_{12}$ and MgH$_{16}$ are found to be…

Materials Science · Physics 2015-06-12 David C. Lonie , James Hooper , Bahadir Altintas , Eva Zurek

Observation of high-temperature superconductivity in sulfur hydrides at megabar pressures has generated an irresistible wave on searching for new superconductors in other compressed hydrogen-rich compounds. An immediate effort is towards…

Superconductivity · Physics 2016-02-10 Xin Zhong , Hui Wang , Jurong Zhang , Hanyu Liu , Shoutao Zhang , Hai-Feng Song , Guochun Yang , Lijun Zhang , Yanming Ma

Hydrogen-rich materials are the most promising candidates for high-temperature conventional superconductors under ambient pressure. Multinary hydrides have abundant structural configurations and are more promising to find high-temperature…

Superconductivity · Physics 2025-08-18 Bo-Wen Yao , Zhenfeng Ouyang , Xiao-Qi Han , Chang-Jiang Wu , Peng-Jie Guo , Ze-Feng Gao , Zhong-Yi Lu
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