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Spin engineering of advanced pulse sequences has had a transformative impact on the development of nuclear magnetic resonance (NMR) spectroscopy, to an extending degree also electron paramagnetic resonance (EPR), and the hybrid between the…

Chemical Physics · Physics 2025-01-31 Jose P. Carvalho , Anders Bodholt Nielsen , Eniko Baligacs , Nino Wili , Niels Chr. Nielsen

Hyper-polarization of nuclear spins is crucial for advancing nuclear magnetic resonance (NMR) and quantum information technologies, as nuclear spins typically exhibit extremely low polarization at room temperature due to their small…

Quantum Physics · Physics 2025-05-20 Haiyang Li , Hao Liao , Ping Wang

The magnetic interactions between the spin of an unpaired electron and the surrounding nuclear spins can be exploited to gain structural information, to reduce nuclear relaxation times as well as to create nuclear hyperpolarization via…

We studied spatial distribution of dynamic nuclear polarization (DNP) in a Hall-bar device in a breakdown regime of the quantum Hall effect (QHE). We detected nuclear magnetic resonance (NMR) signals from the polarized nuclear spins by…

Mesoscale and Nanoscale Physics · Physics 2011-01-25 Minoru Kawamura , Kimitoshi Kono , Yoshiaki Hashimoto , Shingo Katsumoto , Tomoki Machida

Nuclear spin polarization can be pumped into spin-blocked quantum dots by multiple Landau- Zener passages through singlet-triplet anticrossings. By numerical simulations of realistic systems including approximately $10^7$ nuclear spins…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Arne Brataas , Emmanuel I. Rashba

The optically induced polarization of localized electron spins in an ensemble of quantum dots (QDs) dephases due to the interaction with the surrounding nuclear spins. Despite this dephasing, the spins in the QDs can be controlled to…

Mesoscale and Nanoscale Physics · Physics 2022-04-08 P. Schering , G. S. Uhrig

Dynamical magnetic and nuclear polarization in complex spin systems is discussed on the example of transfer of spin from exciton to the central spin of magnetic impurity in a quantum dot in the presence of a finite number of nuclear spins.…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Ramin M. Abolfath , Anna Trojnar , Bahman Roostaei , Thomas Brabec , Pawel Hawrylak

The Overhauser effect (OE) and the Solid effect (SE) are two Dynamic Nuclear Polarization techniques. These two-spin techniques are widely used to create nonequilibrium nuclear spin states having polarization far beyond its equilibrium…

Quantum Physics · Physics 2026-02-03 Sarfraj Fency , Rangeet Bhattacharyya

We propose a nuclear-spin-polarization protocol in a general evolution-and-measurement framework. The protocol works in a spin-star configuration, where the central spin is coupled to the surrounding bath (nuclear) spins by flip-flop…

Quantum Physics · Physics 2022-12-07 Zhu-yao Jin , Jia-shun Yan , Jun Jing

We observe multiple stable states of nuclear polarization in a double quantum dot under conditions of electron spin resonance. The stable states can be understood within an elaborated theoretical rate equation model for the polarization in…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 J. Danon , I. T. Vink , F. H. L. Koppens , K. C. Nowack , L. M. K. Vandersypen , Yu. V. Nazarov

The nuclear spins in nanostructured semiconductors play a central role in quantum applications. The nuclear spins represent a useful resource for generating local magnetic fields but nuclear spin noise represents a major source of dephasing…

Optical nuclear electric resonance (ONER), a recently proposed protocol for nuclear spin manipulation in atomic systems via short laser pulses with MHz repetition rate, exploits the coupling between the nuclear quadrupole moment of a…

Quantum Physics · Physics 2025-01-30 Johannes K. Krondorfer , Matthias Diez , Andreas W. Hauser

We present a general method to realize resonant coupling between spins even though their energies are of different scales. Applying the method to the electron and nuclear spin systems such as a nitrogen-vacancy (NV) center with its nearby…

Quantum Physics · Physics 2023-11-20 Sichen Xu , Chanying Xie , Zhen-Yu Wang

Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

Amplification of a single spin state using nuclear magnetic resonance (NMR) techniques in a rotating frame is considered. The main aim is to investigate the efficient of various schemes for quantum detection. Results of numerical simulation…

Quantum Physics · Physics 2007-08-31 Gregory B. Furman , Victor M. Meerovich , Vladimir L. Sokolovsky

Experiments in coherent spectroscopy correspond to control of quantum mechanical ensembles guiding them from initial to final target states. The control inputs (pulse sequences) that accomplish these transformations should be designed to…

Quantum Physics · Physics 2009-11-07 Navin Khaneja , Timo Reiss , Burkhard Luy , Steffen J. Glaser

We demonstrate dynamical nuclear spin polarization in the absence of an external magnetic field, by resonant circularly polarized optical excitation of a single electron or hole charged quantum dot. Optical pumping of the electron spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 C. W. Lai , P. Maletinsky , A. Badolato , A. Imamoglu

We analyze the polarization of nuclear spins in a quantum dot induced by a single-electron spin that is electrically driven to perform coherent Rabi oscillations. We derive the associated nuclear-spin polarization rate and analyze its…

Mesoscale and Nanoscale Physics · Physics 2023-10-25 Peter Stano , Takashi Nakajima , Akito Noiri , Seigo Tarucha , Daniel Loss

Experiments suggest that nuclear spins play a significant role in the quantum Hall effect (QHE) near integer and fractional QHE spin transitions, but many of these phenomena still remain to be understood. Here we study theoretically the…

Mesoscale and Nanoscale Physics · Physics 2026-02-03 Haotian Zhou , Yuli Lyanda-Geller

In this work, we extend the quantum optimal control theory of molecules subject to ultrashort laser pulses to the case of solvated systems, explicitly including the solvent dielectric properties in the system Hamiltonian. A reliable…

Chemical Physics · Physics 2019-12-23 Marta Rosa , Gabriel Gil , Stefano Corni , Roberto Cammi
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