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Related papers: Topological Constraints in Directed Polymer Melts

200 papers

Conformation-dependent design of polymer sequences can be considered as a tool to control macromolecular self-assembly. We consider the monomer unit sequences created via the modification of polymers in a homogeneous melt in accordance with…

Soft Condensed Matter · Physics 2021-07-07 Elena N. Govorun , Ruslan M. Shupanov , Sophia A. Pavlenko , Alexei R. Khokhlov

We study structural properties of a ring polymeric melt confined in a film in comparison to a linear counterpart using molecular dynamics simulations. Local structure orderings of ring and linear polymers in the vicinity of the surface are…

Soft Condensed Matter · Physics 2015-10-21 Eunsang Lee , YounJoon Jung

The size of rings (also called cyclic polymers) in bidisperse blends of chemically identical rings is analyzed by computer simulations. Data of entangled ring blends and blends of interpenetrating rings are compared and it is shown that the…

Soft Condensed Matter · Physics 2021-03-31 Michael Lang

In this article we study a \emph{non-directed} polymer model in dimension $d\ge 2$: we consider a simple symmetric random walk on $\mathbb{Z}^d$ which interacts with a random environment, represented by i.i.d. random variables…

Probability · Mathematics 2022-09-26 Quentin Berger , Niccolò Torri , Ran Wei

The impact of polymer-polymer interactions of various types on the thermodynamics, structure, and accommodation of topological constraints is addressed for systems comprising many directed polymers in two spatial dimensions. The approach is…

Soft Condensed Matter · Physics 2013-07-04 D. Zeb Rocklin , Paul M. Goldbart

We consider the point-to-point continuum directed random polymer ($\mathsf{CDRP}$) model that arises as a scaling limit from $1+1$ dimensional directed polymers in the intermediate disorder regime. We show that the annealed law of a…

Probability · Mathematics 2024-12-25 Sayan Das , Weitao Zhu

It is nontrivial whether the average size of a ring polymer should become smaller or larger under a topological constraint. Making use of some knot invariants, we evaluate numerically the mean square radius of gyration for ring polymers…

Statistical Mechanics · Physics 2016-08-31 Miyuki K. Shimamura , Tetsuo Deguchi

In this paper, we consider directed polymers in random environment with long range jumps in discrete space and time. We extend to this case some techniques, results and classifications known in the usual short range case. However, some…

Probability · Mathematics 2007-05-23 Francis Comets

The static and dynamic properties of ring polymers in concentrated solutions remains one of the last deep unsolved questions in Polymer Physics. At the same time, the nature of the glass transition in polymeric systems is also not well…

Soft Condensed Matter · Physics 2016-10-25 Davide Michieletto , Matthew S. Turner

We introduce a new disorder regime for directed polymers in dimension $1+1$ that sits between the weak and strong disorder regimes. We call it the intermediate disorder regime. It is accessed by scaling the inverse temperature parameter…

Probability · Mathematics 2014-03-28 Tom Alberts , Konstantin Khanin , Jeremy Quastel

Ring polymers remain a major challenge to our current understanding of polymer dynamics. Experimental results are difficult to interpret because of the uncertainty in the purity and dispersity of the sample. Using both equilibrium and…

Soft Condensed Matter · Physics 2015-06-03 Jonathan D. Halverson , Gary S. Grest , Alexander Y. Grosberg , Kurt Kremer

Advances in controlled polymerization have enabled the synthesis of mechanically interlocked polymers like molecular knots and linear[n]catenane. These aesthetic macromolecules with unique topological constraints in the form of mechanical…

Soft Condensed Matter · Physics 2026-03-30 Prabeen Kumar Pattnayak , Aloke Kumar , Gaurav Tomar

We report simulation results on melts of entangled linear polymers confined in a free-standing thin film. We study how the geometric constraints imposed by the confinement alter the entanglement state of the system compared to the…

Soft Condensed Matter · Physics 2019-03-06 Nicolás A. García , Jean-Louis Barrat

We review pro and contra of the hypothesis that generic polymer properties of topological constraints are behind many aspects of chromatin folding in eukaryotic cells. For that purpose, we review, first, recent theoretical and computational…

Biomolecules · Quantitative Biology 2015-06-18 Jonathan D. Halverson , Jan Smrek , Kurt Kremer , Alexander Y. Grosberg

We consider $(1+1)$-dimensional directed polymers in a random potential and provide sufficient conditions guaranteeing joint localization. Joint localization means that for typical realizations of the environment, and for polymers started…

Probability · Mathematics 2022-11-14 Yuri Bakhtin , Douglas Dow

By means of sophisticated Monte Carlo methods, we investigate the conformational phase diagram of a simple model for flexible polymers with explicit thickness. The thickness constraint, which is introduced geometrically via the global…

Soft Condensed Matter · Physics 2009-02-06 Thomas Vogel , Thomas Neuhaus , Michael Bachmann , Wolfhard Janke

We have developed a new multiscale simulation technique to investigate history-dependent flow behavior of entangled polymer melt, using a smoothed particle hydrodynamics simulation with microscopic simulators that account for the dynamics…

Soft Condensed Matter · Physics 2011-11-01 Takahiro Murashima , Takashi Taniguchi

The predictions of the polymer mode coupling theory for the finite size corrections to the transport coefficients of entangled polymeric systems are tested in comparisons with various experimental data. It is found that quantitative…

Condensed Matter · Physics 2009-10-30 Matthias Fuchs , Kenneth S. Schweizer

Through extensive Monte Carlo simulations, we systematically study the effect of chain stiffness on the packing ability of linear polymers composed of hard spheres in extremely confined monolayers, corresponding effectively to 2D films.…

The effect of topology on the collapse transition and instantaneous shape of an energy polydisperse polymer (a model heteropolymer) is studied by means of computer simulations. In particular, we consider three different chain topology,…

Soft Condensed Matter · Physics 2022-11-24 Thoudam Vilip Singh , Lenin S. Shagolsem