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Motivated by ferrimagnetic oligonuclear and chain compounds synthesized by Caneschi et al., both of which consist of alternating manganese(II) ions and nitronyl-nitroxide radicals, we calculate the nuclear spin-lattice relaxation rate 1/T_1…

Strongly Correlated Electrons · Physics 2009-11-10 Hiromitsu Hori , Shoji Yamamoto

Using X-band pulsed electron spin resonance, we report the intrinsic spin-lattice ($T_1$) and phase coherence ($T_2$) relaxation times in molecular nanomagnets for the first time. In Cr$_7M$ heterometallic wheels, with $M$ = Ni and Mn,…

The spin-lattice relaxation rate $T_{1}^{-1}$ and NMR spectra of $^1$H in single crystal molecular magnets of Fe8 have been measured down to 15 mK. The relaxation rate $T_1^{-1}$ shows a strong temperature dependence down to 400 mK. The…

Condensed Matter · Physics 2009-11-07 Miki Ueda , Satoru Maegawa , Susumu Kitagawa

The nuclear spin-lattice relaxation rate ($1/T_{1}$) has been measured in the single crystals of hole doped two-leg ladder compounds Sr$_{14-x}$Ca$_{x}$Cu$_{24}$O$_{41}$ and in the undoped parent material La$_6$Ca$_8$Cu$_{24}$O$_{41}$.…

Strongly Correlated Electrons · Physics 2009-10-31 S. Fujiyama , M. Takigawa , N. Motoyama , H. Eisaki , S. Uchida

The site-selective nuclear spin-lattice relaxation rate T1^{-1} is theoretically studied inside a vortex core in a chiral p-wave superconductor within the framework of the quasiclassical theory of superconductivity. It is found that T1^{-1}…

Superconductivity · Physics 2009-11-07 Nobuhiko Hayashi , Yusuke Kato

Perturbations of all sorts destabilise the rotation of a small body and leave it in a non-principal spin state. In such a state, the body experiences alternating stresses generated by the inertial forces. This yields nutation relaxation,…

Earth and Planetary Astrophysics · Physics 2017-11-15 Julien Frouard , Michael Efroimsky

Understanding the effect of vibrations on the relaxation process of individual spins is crucial for implementing nano systems for quantum information and quantum metrology applications. In this work, we present a theoretical microscopic…

Mesoscale and Nanoscale Physics · Physics 2018-03-28 A. Norambuena , E. Muñoz , H. T. Dinani , A. Jarmola , P. Maletinsky , D. Budker , J. R. Maze

This paper employs the general time-space fractional diffusion equation to derive correlation time function for analyzing nuclear magnetic resonance (NMR) relaxation. Both the anomalous rotational and translational diffusion are treated.…

Chemical Physics · Physics 2018-12-31 Guoxing Lin

We investigate the interplay between the lattice, charge, and spin dynamics in charge ordered high $T_c$ cuprate La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ ($T_{c} =4$~K) based on the inverse Laplace transform (ILT) analysis of the $^{139}$La…

Strongly Correlated Electrons · Physics 2022-03-09 P. M. Singer , A. Arsenault , T. Imai , M. Fujita

Traditional theories of the NMR autocorrelation function for intramolecular dipole pairs assume single-exponential decay, yet the calculated autocorrelation of realistic systems display a rich, multi-exponential behavior resulting in…

Finite-temperature local spin dynamics within the random spin-1/2 antiferromagnetic Heisenberg chain is studied numerically. The aim is to explain measured NMR spin-lattice relaxation times in BaCu_{2}(Si_{0.5}Ge_{0.5})_{2}O_{7}, which is…

Strongly Correlated Electrons · Physics 2013-10-04 J. Herbrych , J. Kokalj , P. Prelovšek

We investigate the magnetization dynamics of a conducting magnetic nanoparticle weakly coupled to source and drain electrodes, under the assumption that all relaxation comes from exchange of electrons with the electrodes. The magnetization…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Xavier Waintal , Piet W. Brouwer

Finite-temperature spin dynamics in planar t-J model is studied using the method based on the Lanczos diagonalization of small systems. Dynamical spin structure factor at moderate dopings shows the coexistence of free-fermion-like and…

Condensed Matter · Physics 2009-10-22 J. Jaklic , P. Prelovsek

The negatively charged boron vacancy $V_B^-$ defect in hexagonal boron nitride (hBN) has recently emerged as a promising spin qubit for sensing due to its high-temperature spin control and versatile integration into van der Waals…

Quantum Physics · Physics 2025-11-24 Chanaprom Cholsuk , Tobias Vogl , Viktor Ivády

A comprehensive theoretical description is given for the spin relaxation and diffusion in solids. The formulation is made in a general statistical-mechanical way. The method of the nonequilibrium statistical operator (NSO) developed by D.…

Statistical Mechanics · Physics 2009-11-11 A. L. Kuzemsky

Nuclear spin-lattice relaxation in one-dimensional Heisenberg ferrimagnets is studied by means of a modified spin-wave theory. Calculating beyond the first-order mechanism, where a nuclear spin directly interacts with spin waves through the…

Strongly Correlated Electrons · Physics 2015-06-25 Shoji Yamamoto , Hiromitsu Hori

The methods of Nuclear Magnetic Resonance belong to the best developed and often used tools for studying random motion of particles in different systems, including soft biological tissues. In the long-time limit the current mathematical…

Statistical Mechanics · Physics 2018-03-06 Vladimir Lisy , Jana Tothova

We present simulation results on the equilibrium relaxation of Brownian planar rotors based on a uniformly frustrated XY model on a square lattice. The rotational relaxation exhibits typical dynamic features of fragile supercooled liquids…

Statistical Mechanics · Physics 2009-10-31 Sung Jong Lee , Bongsoo Kim

Molecular and lattice vibrations are able to couple to the spin of electrons and lead to their relaxation and decoherence. Ab initio simulations have played a fundamental role in shaping our understanding of this process but further…

Materials Science · Physics 2024-10-14 Valerio Briganti , Alessandro Lunghi

Nuclear Magnetic Resonance (NMR) is a tool of choice to characterize molecular motions. In biological macromolecules, pico- to nano-second motions, in particular, can be probed by nuclear spin relaxation rates which depend on the time…

Chemical Physics · Physics 2022-10-12 Nicolas Bolik-Coulon , Fabien Ferrage