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We consider the excitation dynamics of the two-photon \sts transition in a beam of atomic hydrogen by 243 nm laser radiation. Specifically, we study the impact of ionization damping on the transition line shape, caused by the possibility of…

We present analytical expressions of momentum-resolved core-level photoemission time delay in a molecular frame of a heteronuclear diatomic molecule upon photoionization by a linearly polarized soft x-rays attosecond pulse. For this…

Chemical Physics · Physics 2022-05-31 Y. Tamura , K. Yamazaki , K. Ueda , K. Hatada

Photoionization from atom-C60 hybrid levels in halogen endufullerene molecules, Cl@C60, Br@C60 and I@C60, are calculated using a linear response density functional method. Both the ordinary electron-configuration where the open shell…

Atomic and Molecular Clusters · Physics 2021-06-08 Dakota Shields , Ruma De , Esam Ali , Mohamed E Madjet , Steven T Manson , Himadri S. Chakraborty

We investigate the effects of the multielectron polarization of the ion described by the induced dipole potential in photoelectron momentum distributions produced in ionization of the CO molecule by a strong laser field. We present results…

Atomic Physics · Physics 2024-04-23 Mahmoud Abu-samha , L. B. Madsen , N. I. Shvetsov-Shilovski

The ionization of two-active-electron systems by intense laser fields is investigated theoretically. In comparison with time-dependent Hartree-Fock and exact two electron simulation, we show that the ionization rate is overestimated in SAE…

Atomic Physics · Physics 2015-06-18 Zengxiu Zhao , Jianmin Yuan

Characterization of the inner-shell decay processes in molecules containing heavy elements is key to understanding x-ray damage of molecules and materials and for medical applications with Auger-electron-emitting radionuclides. The 1s hole…

We study the scattering of infrared light by small dielectric core-shell particles taking a sapphire sphere with a CaO core as an example. The extinction efficiency of such a particle shows two intense series of resonances attached,…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 E. Thiessen , F. X. Bronold , R. L. Heinisch , H. Fehske

We present the angular distribution of electrons knocked out from an atom in a fast charge particle collision at small momentum transfer. It is determined not only by dipole but also by quadrupole transitions, the contribution of which can…

Atomic Physics · Physics 2015-06-03 M. Ya. Amusia , L. V. Chernysheva , E. Z. Liverts

We present ionization probability and line shape calculations for the two-step 3-photon ionization process, $1S \stackrel{2\hbar \omega}{\longrightarrow}2S \stackrel{\hbar \omega}{\longrightarrow}\epsilon P $, of the ground state of…

Atomic Physics · Physics 2016-08-15 V Yakhontov , R. Santra , K. Jungmann

We present and discuss a new computationally inexpensive method to study, within the single active electron approximation, the interaction of a complex system with an intense ultrashort laser pulse. As a first application, we consider the…

We explore excitation and ionization by neutron impact as a novel tool for the investigation of electron-electron correlations in helium. We present single and double ionization spectra calculated in accurate numerical ab-initio simulations…

Atomic Physics · Physics 2013-05-24 M. Liertzer , J. Feist , S. Nagele , J. Burgdörfer

We employ the recently developed multi-photon R-matrix method for molecular above-threshold photoionization to obtain second-order ionization amplitudes that govern the interference in RABITT experiments. This allows us to extract RABITT…

Atomic Physics · Physics 2022-05-03 Jakub Benda , Zdeněk Mašín , Jimena D. Gorfinkiel

The analytical structure and absolute values of the generalized cross-section of the two-photon resonance single ionization of the K-shell of a heavy neon-like ion of an iron atom (Fe$^{16+}$) were theoretically predicted. A pronounced…

Using the recently developed concept of the 2-electron streak camera (see NJP 12, 103024 (2010)), we have studied the energy-sharing between the two ionizing electrons in single-photon double ionization of He(1s2s). We find that the most…

Atomic Physics · Physics 2015-05-28 H. Price , A. Staudte , A. Emmanouilidou

Considering C$_{60}$ as a model system for describing field emission from the extremity of a carbon nanotip, we explore electron emission from this fullerene excited by an intense, near-infrared, few-cycle laser pulse…

Atomic and Molecular Clusters · Physics 2016-03-23 Cong-Zhang Gao , Phuong Mai Dinh , Peter Kluepfel , Chris Meier , Paul-Gerhard Reinhard , Eric Suraud

Theoretical approaches to the photoionization of few-electron atoms are discussed. These include nonequilibrium Greens functions and wave function based approaches. In particular, the Multiconfiguration Time-Dependent Hartree-Fock method is…

Atomic Physics · Physics 2015-05-14 M. Bonitz , D. Hochstuhl , S. Bauch , K. Balzer

Shocks, modelled over a broad range of parameters, are used to construct a new tool to deduce the mechanical energy and physical conditions from observed atomic or molecular emission lines. We compute magnetised, molecular shock models with…

Astrophysics of Galaxies · Physics 2022-03-14 Andrew Lehmann , Benjamin Godard , Gillaume Pineau des Forêts , Alba Vidal-García , Edith Falgarone

We present experimental measurements and theoretical calculations of photoionization time delays from the $3s$ and $3p$ shells in Ar in the photon energy range of 32-42 eV. The experimental measurements are performed by interferometry using…

We study strong-field double ionization in a three-electron atom by applying a simplified, reduced-dimensionality model with three active electrons. The influence of the spin-induced symmetry of the spatial part of the wavefunction on the…

Theoretical study on H$_2^+$ in an intense infrared laser field on the attosecond time-scale reveals that the molecular ion shows multiple bursts of ionization within a half-cycle of the laser field oscillation, in contrast to the widely…

Chemical Physics · Physics 2010-12-10 Norio Takemoto , Andreas Becker