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Using an \textit{ab initio} approach based on the GW approximation which includes strong local \textbf{k}-space correlations, the Metal-Insulator Transition of M$_2$ vanadium dioxide is broken down into its component parts and investigated.…

Strongly Correlated Electrons · Physics 2017-09-15 Jamie M. Booth , Daniel W. Drumm , Phil S. Casey , Suresh K. Bhargava , Jackson S. Smith , Salvy P. Russo

Correlated electron materials (CEMs) host a rich variety of condensed matter phases. Vanadium dioxide (VO2) is a prototypical CEM with a temperature-dependent metal-to-insulator (MIT) transition with a concomitant crystal symmetry change.…

Tungsten oxide and its associated bronzes (compounds of tungsten oxide and an alkali metal) are well known for their interesting optical and electrical characteristics. We have modified the transport properties of thin WO$_3$ films by…

Superconductivity · Physics 2017-07-19 X. Leng , J. Pereiro , J. Strle , G. Dubuis , A. T. Bollinger , A. Gozar , J. Wu , N. Litombe , C. Panagopoulos , D. Pavuna , I. Božović

We present a density-functional theory (DFT) study of the structural, electronic, and chemical bonding behaviour in germanium (Ge)-doped vanadium dioxide (VO$_2$). Our motivation is to explain the reported increase of the metal-insulator…

Materials Science · Physics 2023-02-03 Peter Mlkvik , Claude Ederer , Nicola A. Spaldin

We report modulation of a reversible phase transition in VO2 films by hydrogen doping. A metallic phase and a new insulating phase are successively observed at room temperature as the doping concentration increases. It is suggested that the…

Strongly Correlated Electrons · Physics 2017-09-27 Shi Chen , Zhaowu Wang , Lele Fan , Yuliang Chen , Hui Ren , Heng Ji , Douglas Natelson , Yingying Huang , Jun Jiang , Chongwen Zou

Charge dynamics of (Ti1-xVx)2O3 with x=0-0.06 has been investigated by measurements of charge transport and optical conductivity spectra in a wide temperature range of 2-600K with the focus on the thermally and doping induced…

Strongly Correlated Electrons · Physics 2009-11-13 M. Uchida , J. Fujioka , Y. Onose , Y. Tokura

Electrons in correlated insulators are prevented from conducting by Coulomb repulsion between them. When an insulator-to-metal transition is induced in a correlated insulator by doping or heating, the resulting conducting state can be…

Metal-ion doping can effectively regulate the metal-insulator transition temperature in $\mathrm{VO}_2$. Experiments found that the pentavalent and hexavalent ion doping dramatically reduces the transition temperature while the trivalent…

Materials Science · Physics 2020-01-09 Yin Shi , Long-Qing Chen

We investigate the changes in the infrared response due to charge carriers introduced by electrostatic doping of the correlated insulator vanadium dioxide (VO2) integrated in the architecture of the field effect transistor. Accumulation of…

Strongly Correlated Electrons · Physics 2009-11-13 M. M. Qazilbash , Z. Q. Li , V. Podzorov , M. Brehm , F. Keilmann , B. G. Chae , H. T. Kim , D. N. Basov

Vanadium dioxide, VO2, and its metal-insulator transition at T=340K continues to receive considerable interest. The question whether the physics of the insulating low-temperature phase is dominated by the Mott or the Peierls scenario, i.e.…

Strongly Correlated Electrons · Physics 2008-11-10 Jan M. Tomczak , Silke Biermann

A theory of the metal-insulator transition in vanadium dioxide from the high-temperature rutile to the low- temperature monoclinic phase is proposed on the basis of cluster dynamical mean field theory, in conjunction with the density…

Strongly Correlated Electrons · Physics 2009-11-10 S. Biermann , A. Poteryaev , A. I. Lichtenstein , A. Georges

By means of first principles schemes based on magnetically constrained density functional theory and on the band unfolding technique we study the effect of doping on the conducting behaviour of the Lifshitz magnetic insulator NaOsO3.…

Strongly Correlated Electrons · Physics 2019-05-01 Sabine Dobrovits , Bongjae Kim , Michele Reticcioli , Alessandro Toschi , Sergii Khmelevskyi , Cesare Franchini

The evolution of the electronic structures of strongly correlated insulators with doping has long been a central fundamental question in condensed matter physics; it is also of great practical relevance for applications. We have studied the…

We present a study on the modification of the electronic structure and hole-doping effect for the layered dichalcogenide WSe_2 with a multi-valley band structure, where Ta is doped on the W site along with a partial substitution of Te for…

Materials Science · Physics 2015-02-20 M. Kriener , A. Kikkawa , T. Suzuki , R. Akashi , R. Arita , Y. Tokura , Y. Taguchi

Metal-insulator (MI) transitions in correlated electron systems have long been a central and controversial issue in material science. Vanadium dioxide (VO2) exhibits a first-order MI transition at 340 K. For more than half a century, it has…

Strongly Correlated Electrons · Physics 2020-08-26 Yasuhiro H. Matsuda , Daisuke Nakamura , Akihiko Ikeda , Shojiro Takeyama , Yuji Muraoka , Yuki Suga

In this work we investigate doping and temperature dependences of electronic structure of system with strong electronic correlations and strong electron-phonon interaction modeling cuprates in the frameworks of the three-band p-d-Holstein…

Strongly Correlated Electrons · Physics 2016-12-09 I. A. Makarov , S. G. Ovchinnikov

We present a theoretical investigation of the electronic structure of rutile (metallic) and M$_1$ and M$_2$ monoclinic (insulating) phases of VO$_2$ employing a fully self-consistent combination of density functional theory and embedded…

Strongly Correlated Electrons · Physics 2016-08-03 W. H. Brito , M. C. O. Aguiar , K. Haule , G. Kotliar

We investigate the influence of an unoccupied band on the transport properties of a strongly correlated electron system. For that purpose, additional orbitals are coupled to a Hubbard model via hybridization. The filling is one electron per…

Condensed Matter · Physics 2009-10-28 Stefan Blawid , Hoangh Anh Tuan , Takashi Yanagisawa , Peter Fulde

Modulation of the charge carrier density in a Mott material by remote doping from a highly doped conventional band insulator is proposed to test theoretical predictions of band filling control of the Mott metal-insulator transition without…

Materials Science · Physics 2011-11-11 Junwoo Son , Bharat Jalan , Adam P. Kajdos , Leon Balents , S. James Allen , Susanne Stemmer

The combination of bandstructure theory in the local density approximation with dynamical mean field theory was recently successfully applied to V$_2$O$_3$ -- a material which undergoes the f amous Mott-Hubbard metal-insulator transition…

Strongly Correlated Electrons · Physics 2009-11-10 K. Held , J. W. Allen , V. I. Anisimov , V. Eyert , G. Keller , H. -D. Kim , S. -K. Mo , D. Vollhardt
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