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We describe a method for simulating exciton dynamics in protein-pigment complexes, including effects from charge transfer as well as fluorescence. The method combines the hierarchical equations of motion, which are used to describe quantum…

Chemical Physics · Physics 2022-11-23 Thomas P. Fay , David T. Limmer

We theoretically investigate a photosystem II-based reaction center modeled as a nonequilibrium quantum junction. We specifically focus on the electron-electron interactions that enable cotunneling events to be captured through quantum…

Mesoscale and Nanoscale Physics · Physics 2024-10-16 Debasish Sharma , Manash Jyoti Sarmah , Mriganka Sandilya , Himangshu Prabal Goswami

We analyze a theoretical model for energy and electron transfer in an artificial photosynthetic system. The photosystem consists of a molecular triad (i.e., with a donor, a photosensitive unit, and an acceptor) coupled to four accessory…

Biological Physics · Physics 2015-05-20 Pulak Kumar Ghosh , Anatoly Yu. Smirnov , Franco Nori

We study a model of a light-induced proton pump in artificial reaction centers. The model contains a molecular triad with four electron states (i.e., one donor state, two photosensitive group states, and one acceptor state) as well as a…

Biological Physics · Physics 2015-05-13 Pulak Kumar Ghosh , Anatoly Yu. Smirnov , Franco Nori

Understanding the behavior of charged complex fluids is crucial for a plethora of important industrial, technological, and medical applications. Using coarse-grained molecular dynamics simulations, here we investigate the properties of a…

Soft Condensed Matter · Physics 2022-08-04 Debarshee Bagchi

Quantum information theorems state that it is possible to exploit collective quantum resources to greatly enhance the charging power of quantum batteries (QBs) made of many identical elementary units. We here present and solve a model of a…

Mesoscale and Nanoscale Physics · Physics 2018-03-19 Dario Ferraro , Michele Campisi , Gian Marcello Andolina , Vittorio Pellegrini , Marco Polini

One of the promising approaches to revealing the photosynthetic efficiency of close to one unit is to investigate the quantum regime of excitation energy transfer (EET). The majority of studies, however, have concluded that different…

Applied Physics · Physics 2024-03-12 Lu-Xin Xu , Shun-Cai Zhao , Sheng-Nan Zhu , Lin-Jie Chen

Quantum batteries (QBs), harnessing quantum systems to transfer and store energy, have garnered substantial attention recently, enabling potentials in enhanced charging capacity, increased charging power, and device miniaturization.…

Quantum Physics · Physics 2025-03-31 Hua-Wei Zhao , Yong Xie , Xinyao Huang , Guo-Feng Zhang

Non-equilibrium transport properties and energy conversion performance of a molecular photo-voltaic cell are analyzed using the Lindblad master equation within the open quantum systems approach. The method allows us to calculate the…

Mesoscale and Nanoscale Physics · Physics 2015-04-09 Shigeru Ajisaka , Bojan Zunkovic , Yonatan Dubi

We explore a protocol that efficiently charges multiple open quantum batteries in parallel using a single charger. This protocol shows super-extensive charging through collective coupling of the charger and the battery to the same thermal…

Quantum Physics · Physics 2024-10-28 Josephine Dias , Hui Wang , Kae Nemoto , Franco Nori , William J. Munro

A quantum heat engine (QHE) based on the interaction driving of a many-particle working medium is introduced. The cycle alternates isochoric heating and cooling strokes with both interaction-driven processes that are simultaneously…

Quantum Physics · Physics 2019-10-18 Yang-Yang Chen , Gentaro Watanabe , Yi-Cong Yu , Xi-Wen Guan , Adolfo del Campo

The majority of photoelectrochemical (PEC) water splitting cells cannot drive the overall water splitting reactions without the assistance of an external power source. To provide added power, the cells are usually connected to photovoltaic…

Applied Physics · Physics 2018-10-31 Gideon Segev , Jeffery Beeman , Ian D. Sharp

The quantum well solar cell (QWSC) has been proposed as a route to higher efficiency than that attainable by homojunction devices. Previous studies have established that carriers escape the quantum wells with high efficiency in forward bias…

Mesoscale and Nanoscale Physics · Physics 2010-06-10 James P. Connolly , Jenny Nelson , Keith W. J. Barnham , Ian Ballard , C. Roberts , J. S. Roberts , C. T. Foxon , .

With intensive studies of quantum thermodynamics, quantum batteries (QBs) have been proposed to store and transfer energy via quantum effects. Despite many theoretical models, decoherence remains a severe challenge and practical platforms…

Quantum Physics · Physics 2026-05-21 Jin-Tian Zhang , Shuang-Quan Ma , Jing-Yi-Ran Jin , Tao Liu , Qing Ai

Separating heat from charge in a material is an extremely challenging task since they are transported by the very same carriers, i.e. electrons or holes. In this Letter we show that such separation can reach 100% efficiency in a hybrid…

Mesoscale and Nanoscale Physics · Physics 2025-03-28 Carlo Panu , Fabio Taddei , Marco Polini , Amir Yacoby

Recently, significant progress in the development of III-V/Si dual-junction solar cells has been achieved. This not only boosts the efficiency of Si-based photovoltaic solar cells, but also offers the possibility of highly efficient green…

Enhanced interaction between two two-level emitters (e.g., atoms) by nonreciprocal photonic media can be of benefit to broad areas, from quantum information science to biological detection. Here we provide a detailed analysis on why…

Quantum Physics · Physics 2022-09-14 S. Ali Hassani Gangaraj , Lei Ying , Francesco Monticone , Zongfu Yu

Recombination of photogenerated charge carriers in polymer bulk heterojunction (BHJ) solar cells reduces the short circuit current (Jsc) and the fill factor (FF). Identifying the mechanism of recombination is, therefore, fundamentally…

Materials Science · Physics 2015-05-20 Sarah R. Cowan , Anshuman Roy , Alan J. Heeger

In organic photovoltaic systems, a photogenerated molecular exciton in the donor domain dissociates into a hole and an electron at the donor/acceptor heterojunction, and subsequently separate into free charge carriers that can be extracted…

Mesoscale and Nanoscale Physics · Physics 2018-07-18 Akihito Kato , Akihito Ishizaki

In green plants, chlorophyll-a and chlorophyll-b are the predominant pigments bound to light-harvesting proteins. While the individual characteristics of these chlorophylls are well understood, the advantages of their coexistence remain…

Data Analysis, Statistics and Probability · Physics 2024-07-17 Eunchul Kim , Daekyung Lee , Souichi Sakamoto , Ju-Yeon Jo , Mauricio Vargas , Akihito Ishizaki , Jun Minagawa , Heetae Kim
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