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Related papers: Vibrational Heat Transport in Molecular Junctions

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Understanding and controlling the flow of heat is a major challenge in nanoelectronics. When a junction is driven out of equilibrium by light or the flow of electric charge, the vibrational and electronic degrees of freedom are, in general,…

Mesoscale and Nanoscale Physics · Physics 2011-06-29 Daniel R. Ward , David A. Corley , James M. Tour , Douglas Natelson

A vibrational model of heat transfer in simple liquids with soft pairwise interatomic interactions is discussed. A general expression is derived, which involves an averaging over the liquid collective mode excitation spectrum. The model is…

Soft Condensed Matter · Physics 2021-01-13 S. A. Khrapak

Determining the vibrational structure of a molecule is central to fundamental applications in several areas, from atmospheric science to catalysis, fuel combustion modeling, biochemical imaging, and astrochemistry. However, when significant…

Quantum Physics · Physics 2021-12-22 Nicolas P. D. Sawaya , Francesco Paesani , Daniel P. Tabor

Heat transfer is a fundamental concept in physics, and how to characterize the microscopical physical mechanism of heat transfer is a significant topic. Recently, a new mechanism for heat transfer, phonon heat transfer across a vacuum…

Quantum Physics · Physics 2025-08-05 Yue-Hui Zhou , Jie-Qiao Liao

Atomic and single-molecule junctions represent the ultimate limit to the miniaturization of electrical circuits. They are also ideal platforms to test quantum transport theories that are required to describe charge and energy transfer in…

Mesoscale and Nanoscale Physics · Physics 2013-08-01 Woochul Lee , Kyeongtae Kim , Wonho Jeong , Linda Angela Zotti , Fabian Pauly , Juan Carlos Cuevas , Pramod Reddy

We examine the electronic heat transport phenomena in nanoscale junctions composed of organic molecules coupled to two metallic reservoirs of different temperatures. The electronic heat flux and its dynamical noise properties are calculated…

Mesoscale and Nanoscale Physics · Physics 2016-08-02 Arthur Luniewski , Rita Aghjayan , Kamil Walczak

We study heat transfer between conductors, mediated by the excitation of a monomodal harmonic oscillator. Using a simple model, we show that the onset of rectification in the system is directly related to the nonlinearity of the electron…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Dvira Segal

Understanding heat transport in semiconductors and insulators is of fundamental importance because of its technological impact in electronics and renewable energy harvesting and conversion. Anharmonic Lattice Dynamics provides a powerful…

Materials Science · Physics 2020-10-13 Giuseppe Barbalinardo , Zekun Chen , Nicholas W. Lundgren , Davide Donadio

In molecular devices electronic degrees of freedom are coupled to vibrational modes of the molecule, offering an opportunity to study fundamental aspects of this coupling between at the nanoscale. To this end we consider the nonequilibrium…

Strongly Correlated Electrons · Physics 2014-01-29 Yuval Vinkler-Aviv , Avraham Schiller , Natan Andrei

We apply the hierarchical equations of motion technique to analyzing nonequilibrium heat transport in a spin-boson type model, whereby heat transfer through a central spin is mediated by an intermediate pair of coupled harmonic oscillators.…

Mesoscale and Nanoscale Physics · Physics 2024-07-29 Graeme Pleasance , Francesco Petruccione

In this work we study the energy transport in a one-dimensional system composed of two dissimilar Frenkel-Kontorova lattices connected by a time-modulated coupling and in contact with two heat reservoirs operating at different temperature…

Statistical Mechanics · Physics 2021-03-03 M. Romero-Bastida

We study thermal transport through Pt nanowires that bridge planar contacts as a function of wire length and vibrational frequency of the contacts. When phonons in the contacts have lower average frequencies than those in the wires thermal…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 Ya Zhou , Alejandro Strachan

We theoretically analyzed inelastic effects in the electron transport through molecular junctions originating from electron-vibron interactions. The molecular bridge was simulated by a periodic chain of identical interacting hydrogen-like…

Materials Science · Physics 2010-01-03 Natalya A. Zimbovskaya , Maija M. Kuklja

Here we present theoretical studies of the effect of vibronic coupling on nonlinear transport characteristics (current-voltage and conductance-voltage) in molecular electronic devices. Considered device is composed of molecular quantum dot…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Kamil Walczak

Recent progress in the field of molecular electronics has revealed the fundamental importance of the coupling between the electronic degrees of freedom and specific vibrational modes. Considering the examples of a molecular dimer and a…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

We develop a Born-Oppenheimer type formalism for the description of quantum thermal transport along hybrid nanoscale objects. Our formalism is suitable for treating heat transfer in the off-resonant regime, where e.g., the relevant…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Lian-Ao Wu , Dvira Segal

The realization of molecular-based electronic devices depends to a large extent on the ability to mechanically stabilize the involved molecular bonds, while making use of efficient resonant charge transport through the device. Resonant…

Mesoscale and Nanoscale Physics · Physics 2018-09-11 David Gelbwaser-Klimovsky , Alán Aspuru-Guzik , Michael Thoss , Uri Peskin

We studied the phononic heat transfer through an atomic dielectric wire with both infinite and finite lengths by using a model Hamiltonian approach. At low temperature under ballistic transport, the thermal conductance contributed by each…

Condensed Matter · Physics 2009-10-31 A. Buldum , S. Ciraci , C. Y. Fong

The influence of multiple vibrational modes on current fluctuations in electron transport through single-molecule junctions is investigated. Our analysis is based on a generic model of a molecular junction, which comprises a single…

Mesoscale and Nanoscale Physics · Physics 2014-09-26 C. Schinabeck , R. Härtle , H. B. Weber , M. Thoss

We investigate the interplay of quantum interference effects and electronic-vibrational coupling in electron transport through single-molecule junctions, employing a nonequilibrium Green's function approach. Our findings show that inelastic…

Mesoscale and Nanoscale Physics · Physics 2013-02-18 R. Härtle , M. Butzin , M. Thoss