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The duration of isolated attosecond pulses created via high-order harmonic generation is determined by the number of optical cycles in the driving laser. Achieving shorter attosecond soft X-ray pulses requires minimizing the number of…

Optics · Physics 2025-11-03 Kaito Nishimiya , Rambabu Rajpoot , Eiji J Takahashi

High-order harmonic generation in polyatomic molecules generally involves multiple channels, each associated with a different orbital. Their unambiguous assignment remains a major challenge for high-harmonic spectroscopy. Here we present a…

Second-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length-scales, quantum mechanical effects come into play which could be…

Optics · Physics 2021-05-11 Muhammad Khalid , Cristian Ciracì

In strong field laser physics it is a common practice to use the high-order harmonic cutoff to estimate the laser intensity of the pulse that generates the harmonic radiation. Based on the semiclassical arguments it is possible to find a…

Atomic Physics · Physics 2015-06-11 T. Shaaran , M. F. Ciappina , M. Lewenstein

High-order harmonic generation stands as a unique nonlinear optical up-conversion process, mediated by a laser-driven electron recollision mechanism, which has been shown to conserve energy, momentum, and spin and orbital angular momentum.…

High-order harmonic generation (HHG) is investigated theoretically in the over-the-barrier ionization (OBI) regime revealing the strong signature of interference between two separately ionized and separately propagating free wave packets of…

High harmonic generation in solids is becoming an important method for strong field solid state physics research. The power scale relationship between high harmonics and the driving laser is investigated both experimentally and…

Optics · Physics 2022-08-23 Shuai Wang , Xinkui He , Yueying Liang , Yabei Su , Shaobo Fang , Zhiyi Wei

A theory for laser-driven electron dynamics and high-harmonic generation in bulk solids with two lattice sites per unit cell of arbitrary dimension is formulated. In tight-binding approximation, such solids can be described by $2\times 2$…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Daniel Moos , Hannah Jürß , Dieter Bauer

We study the temporal and spatial dynamics of the large amplitude and frequency modulation that can be induced in an intense, few cycle laser pulse as it propagates through a rapidly ionizing gas. Our calculations include both single atom…

Atomic Physics · Physics 2009-11-11 Mette B. Gaarde , Mitsuko Murakami , Reinhard Kienberger

The cut-off regime of high-order harmonic generation (HHG) by atoms in an intense laser field is studied numerically and analytically. We find that the cut-off regime is characterized by equal dephasing between the successive harmonics. The…

Atomic Physics · Physics 2016-04-27 M. A. Khokhlova , V. V. Strelkov

We present a high harmonic generation theory which generalizes the strong-field approximation to the resonant case, when the harmonic frequency is close to that of the transition from the ground to an autoionizing state of the generating…

Atomic Physics · Physics 2015-06-16 V. V. Strelkov , M. A. Khokhlova , N. Yu. Shubin

We present a numerical method for investigating the non-perturbative quantum mechanical interaction of light with atoms in two dimensions, without a basis expansion. This enables us to investigate intense laser-atom interactions with light…

Quantum Physics · Physics 2009-10-30 M. Protopapas , D. G. Lappas , P. L. Knight

High harmonic generation in benzene is studied using a mixed quantum-classical approach in which the electrons are described using time-dependent density functional theory while the ions move classically. The interaction with both…

Atomic Physics · Physics 2016-03-02 Abigail Wardlow , Daniel Dundas

Over the past decade, ultrafast electron dynamics in the solid state have been extensively studied using various strong light-matter interaction techniques, such as high-harmonic generation. These studies lead to multiple interpretations of…

High harmonic emissions from crystalline solids contain rich information on the dynamics of electrons driven by intense infrared laser fields and have been intensively studied owing to their potential use as a probe of microscopic…

Materials Science · Physics 2023-05-01 K. Uchida , K. Tanaka

We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…

Strongly Correlated Electrons · Physics 2019-05-24 Shintaro Takayoshi , Yuta Murakami , Philipp Werner

We consider the dynamics of electrons in combined strong laser and Coulomb fields. Under a timescale separation condition, we reduce this dynamics to a guiding-center framework. More precisely, we derive a hierarchy of models for the…

Chaotic Dynamics · Physics 2018-11-28 Jonathan Dubois , S. Berman , C. Chandre , T. Uzer

We studied the high-order harmonic generation (HHG) from 2D solid materials in circularly and bichromatic circularly polarized laser fields numerically by simulating the dynamics of single-active-electron processes in 2D periodic…

We investigate the interwoven dynamic evolutions of neutral nitrogen molecules together with nitrogen ions created through transient tunnel ionization in an intense laser field. By treating the molecules as open quantum systems, it is found…

Harmonic generation is a general characteristic of driven nonlinear systems, and serves as an efficient tool for investigating the fundamental principles that govern the ultrafast nonlinear dynamics. In atomic gases, high-harmonic radiation…