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We report the first three-dimensional wavevector analysis of the jellium exchange-correlation (xc) surface energy in the random-phase approximation (RPA). The RPA accurately describes long-range xc effects which are challenging for…

Materials Science · Physics 2009-11-11 J. M. Pitarke , L. Constantin , J. P. Perdew

In non-self-consistent calculations of the total energy within the random-phase approximation (RPA) for electronic correlation, it is necessary to choose a single-particle Hamiltonian whose solutions are used to construct the electronic…

Materials Science · Physics 2016-01-28 Christopher E. Patrick , Kristian S. Thygesen

Self-consistent relativistic random-phase approximation (RPA) in the radial coordinate representation is established by using the finite amplitude method (FAM). Taking the isoscalar giant monopole resonance in spherical nuclei as example,…

Nuclear Theory · Physics 2013-10-16 Haozhao Liang , Takashi Nakatsukasa , Zhongming Niu , Jie Meng

We present an approximation scheme for the calculation of the principal excitation energies and transition moments of finite many-body systems. The scheme is derived from a first order approximation to the self energy of a recently proposed…

Chemical Physics · Physics 2009-10-30 Joachim Brand , Lorenz S. Cederbaum

We develop and implement a formalism which enables calculating the analytical gradients of particle-hole random-phase approximation (RPA) ground-state energy with respect to the atomic positions within the atomic orbital basis set…

Chemical Physics · Physics 2021-09-03 Muhammad N. Tahir , Tong Zhu , Honghui Shang , Jia Li , Volker Blum , Xinguo Ren

We investigate fractional-charge and fractional-spin errors in range-separated density-functional theory. Specifically, we consider the range-separated hybrid (RSH) method which combines long-range Hartree-Fock (HF) exchange with a…

Chemical Physics · Physics 2017-03-08 Bastien Mussard , Julien Toulouse

We present a new method to obtain interaction part of a model Hamiltonian from the result of the first-principles calculation. The effective interaction contained in the model is determined based on the random phase approximation (RPA). In…

Materials Science · Physics 2017-04-26 Hirofumi Sakakibara , Seung Woo Jang , Hiori Kino , Myung Joon Han , Kazuhiko Kuroki , Takao Kotani

The Self-Consistent RPA (SCRPA) equations in the particle-particle channel are solved without any approximation for the picket fence model. The results are in excellent agreement with the exact solutions found with the Richardson method.…

Nuclear Theory · Physics 2009-11-07 Jorge G. Hirsch , Alejandro Mariano , Jorge Dukelsky , Peter Schuck

In this work, we consider the particle-hole random phase approximation (phRPA), an approximation to the correlation energy in electronic structure, and show that the phRPA energy of the H2 molecule correctly dissociates. That is, as the…

Analysis of PDEs · Mathematics 2022-10-11 Mi-Song Dupuy , Kyle Thicke

Range separated hybrid density functionals are very successful in describing a wide range of molecular and solid state properties accurately. Range separated hybrid functionals are designed from spherically averaged or system averaged…

Materials Science · Physics 2017-12-15 Subrata Jana , Prasanjit Samal

This paper is concerned with classes of models of stochastic reaction dynamics with time-scales separation. We demonstrate that the existence of the time-scale separation naturally leads to the application of the averaging principle and…

Computational Physics · Physics 2007-05-23 Sergey Plyasunov

The recent major modification, r$^2$SCAN, of the SCAN (strongly constrained and appropriately normed) meta-GGA exchange-correlation functional is shown to give substantially better spin-crossover electronic energies (high spin minus low…

Chemical Physics · Physics 2021-01-27 Daniel Mejia-Rodriguez , S. B. Trickey

By coupling a doorway state to a see of random background states, we develop the theory of doorway states in the framework of the random-phase approximation (RPA). Because of the symmetry of the RPA equations, that theory is radically…

Nuclear Theory · Physics 2015-06-22 A. De Pace , A. Molinari , H. A. Weidenmueller

The nuclear symmetry energy calculated in the RPA from the pairing plus symmetry force Hamiltonian with equidistant single-nucleon levels is for mass number A=48 approximately proportional to T(T+1.025), where T is the isospin quantum…

Nuclear Theory · Physics 2015-06-26 Kai Neergård

We obtain the RPA summed one-meson exchange potential between nucleons in symmetric nuclear matter at zero temperature, from a model which includes $\rho $, $\sigma $, $\omega $ and $\pi $ mesons. The behavior of rho mesons inside the…

Nuclear Theory · Physics 2007-05-23 L. Mornas , E. Gallego , A. Perez

We propose a staggered mesh method for correlation energy calculations of periodic systems under the random phase approximation (RPA), which generalizes the recently developed staggered mesh method for periodic second order…

Computational Physics · Physics 2023-04-10 Xin Xing , Lin Lin

Self-consistent random phase approximation (RPA) approaches in the relativistic framework are applied to calculate the isospin symmetry-breaking corrections $\delta_c$ for the $0^+\to0^+$ superallowed transitions. It is found that the…

Nuclear Theory · Physics 2009-08-03 Haozhao Liang , Nguyen Van Giai , Jie Meng

Direction of arrival (DOA) estimation in array processing using uniform/sparse linear arrays is concerned in this paper. While sparse methods via approximate parameter discretization have been popular in the past decade, the discretization…

Information Theory · Computer Science 2014-10-24 Zai Yang , Lihua Xie , Cishen Zhang

We performed density functional calculations to estimate the formation energies of intermetallic alloys. We used two semilocal approximations, the generalized gradient approximation (GGA) by Perdew-Burke-Ernzerhof (PBE) and the strongly…

Materials Science · Physics 2020-11-25 Niraj K. Nepal , Santosh Adhikari , Bimal Neupane , Adrienn Ruzsinszky

A systematic analysis of giant quadrupole resonances is performed for several nuclei, from $^{30}$Si to $^{208}$Pb, within the subtracted second random--phase--approximation (SSRPA) model in the framework of the energy--density--functional…

Nuclear Theory · Physics 2018-10-17 Olivier Vasseur , Danilo Gambacurta , Marcella Grasso