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In this paper we consider the essential electronic excited states in parallel chains of semiconducting polymers that are currently being explored for photovoltaic and light-emitting diode applications. In particular, we focus upon various…

Materials Science · Physics 2009-11-11 Eric R. Bittner , John Glenn Santos Ramon , Stoyan Karabunarliev

The electronic excitation of molecules triggers diverse phenomena such as luminescence and photovoltaic effects, which are the bases of various energy-converting devices. Understanding and control of the excitations at the single-molecule…

Chemical Physics · Physics 2017-07-12 Hiroshi Imada , Kuniyuki Miwa , Miyabi Imai-Imada , Shota Kawahara , Kensuke Kimura , Yousoo Kim

Two-dimensional semiconducting systems, such as quantum wells and transition metal dichalcogenides, are the foundations to investigate low dimensional light-matter interactions. To date, the study of elementary photoexcitation, namely the…

Explaining the mechanism of superconductivity in the high-$T_c$ cuprates requires an understanding of what causes electrons to form Cooper pairs. Pairing can be mediated by phonons, the screened Coulomb force, spin or charge fluctuations,…

An exciton, a two-body composite quasiparticle formed of an electron and hole, is a fundamental optical excitation in condensed-matter systems. Since its discovery nearly a century ago, a measurement of the excitonic wavefunction has…

Based on a microscopic many-particle theory we investigate the influence of excitonic correlations on the vectorial polarization state characteristics of the parametric amplification of polaritons in semiconductor microcavities. We study a…

Other Condensed Matter · Physics 2009-11-13 S. Schumacher , N. H. Kwong , R. Binder

Exciton-exciton annihilation is a ubiquitous nonlinear dynamical phenomenon in materials hosting Frenkel excitons, that has been employed to probe exciton diffusion processes in conjugated polymeric materials. In this work, we investigate…

Bose-Fermi systems such as mixtures of electrons with excitons or exciton-polaritons are extensively discussed as candidates to host a variety of intriguing phenomena, including polaron formation, drag effects, supersolidity, and…

Mesoscale and Nanoscale Physics · Physics 2023-08-09 Andrey S. Plyashechnik , Alexey A. Sokolik , Nina S. Voronova , Yurii E. Lozovik

The momentum-space signatures of excitons can be experimentally accessed through time-resolved (pump-probe) photoelectron spectroscopy. In this work, we develop a computational framework for exciton photoemission orbital tomography (exPOT)…

Electron energy loss spectroscopy is consolidating as a powerful tool to explore electronic (as well as vibrational) excitations of matter, including molecules. Performed in a scanning transmission electron microscope, this technique is…

Chemical Physics · Physics 2021-03-05 Ciro A. Guido , Enzo Rotunno , Matteo Zanfrognini , Stefano Corni , Vincenzo Grillo

We present a theory of polarized photoluminescence of triplet excitons in semiconductor nanocrystal ensembles with the random fine structure contributed by the electron-hole exchange and carrier-nuclear hyperfine interactions. The…

Mesoscale and Nanoscale Physics · Physics 2026-03-31 D. S. Smirnov , E. L. Ivchenko

In this paper we consider dynamics of a molecular system subjected to external pumping by a light source. Within a completely quantum mechanical treatment, we derive a general formula, which enables to asses effects of different light…

Biological Physics · Physics 2012-01-30 Tomas Mancal , Leonas Valkunas

Symmetric electron-hole bilayer systems have been studied at zero temperature using the diffusion quantum Monte Carlo method. A flexible trial wave function is used that can describe fluid, excitonic and biexcitonic phases. We calculate…

Strongly Correlated Electrons · Physics 2013-09-10 Ryo Maezono , Pablo López Ríos , Tetsuo Ogawa , Richard J. Needs

An overview on photon echo spectroscopy under resonant excitation of the exciton complexes in semiconductor nanostructures is presented. The use of four-wave-mixing technique with the pulsed excitation and heterodyne detection allowed us to…

Mesoscale and Nanoscale Physics · Physics 2018-08-29 S. V. Poltavtsev , I. A. Yugova , I. A. Akimov D. R. Yakovlev , M. Bayer

We derive exciton-spin interactions from a microscopic correlated model that captures important aspects of the physics of charge-transfer (CT) insulators to address magnetism associated with exciton creation. We present a minimal model…

Strongly Correlated Electrons · Physics 2023-11-16 Tatsuya Kaneko , Yuta Murakami , Denis Golež , Zhiyuan Sun , Andrew J. Millis

We theoretically investigate the Stark shift of the exciton goundstate in two vertically coupled quantum dots as a function of the interdot distance. The coupling is shown to enhance the tuneability of the linear optical properties,…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 F. Troiani , E. Molinari

Control of the band-edge offsets at heterojunctions between organic semiconductors allows efficient operation of either photovoltaic or light-emitting diodes. We investigate systems where the exciton is marginally stable against charge…

Soft Condensed Matter · Physics 2013-09-27 Arne C. Morteani , Paiboon Sreearunothai , Laura M. Herz , Richard H. Friend , Carlos Silva

We develop a theory of polarized photoluminescence of interface excitons localized at lateral heterojunctions between transition metal dichalcogenide monolayers. We show that the circular selection rules governing interband optical…

Mesoscale and Nanoscale Physics · Physics 2026-03-26 M. V. Durnev , D. S. Smirnov

Macroscopic coherence in quantum fluids allows the observation of interference effects in their wavefunctions, and enables applications such as superconducting quantum interference devices based on Josephson tunneling. The Josephson effect…

Inelastic electron tunneling in a scanning tunneling microscope (STM) is used to generate excitons in monolayer tungsten disulfide (WS$_2$). Excitonic electroluminescence is measured both at positive and negative sample bias. Using optical…