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Nuclear magnetic resonance (NMR) is a powerful tool for applications ranging from chemical analysis to quantum information processing. Achieving optical initialization and detection of molecular nuclear spins promises new opportunities -…

Optically addressable electron spin clusters are of interest for quantum computation, simulation and sensing. However, with interaction length scales of a few tens of nanometers in the strong coupling regime, they are unresolved in…

Quantum Physics · Physics 2024-12-30 Matthew Joliffe , Vadim Vorobyov , Jörg Wrachtrup

The Nitrogen-Vacancy (NV) defect in diamond is a unique quantum system that offers precision sensing of nanoscale physical quantities beyond the current state-of-the-art. Here we present a method to controllably encode the interactions in…

Spin systems in solid state materials are promising qubit candidates for quantum information or quantum sensing. A major prerequisite here is the coherence of spin phase oscillations. In this work, we show a control sequence which, by…

Decoupling the interactions in a spin network governed by a pair-interaction Hamiltonian is a well-studied problem. Combinatorial schemes for decoupling and for manipulating the couplings of Hamiltonians have been developed which use…

Quantum Physics · Physics 2023-11-27 Martin Roetteler

A dynamical decoupling scheme for the deterrence of errors in the non-Markovian (usually corresponding to low temperature, short time, and strong coupling) regimes suitable for qubits constructed out of a multilevel structure is studied. We…

Quantum Physics · Physics 2007-05-23 K. Shiokawa , B. L. Hu

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

Atom-like emitters in solids are promising platforms for quantum sensing and information processing, but inhomogeneities in the emitter fine structure complicate quantum control. We present a framework that leverages this diversity to…

Quantum Physics · Physics 2025-09-04 Pratyush Anand , Louis Follet , Odiel Hooybergs , Dirk R. Englund

The hyperpolarisation of nuclear spins within target molecules is a critical and complex challenge in magnetic resonance imaging (MRI) and nuclear magnetic resonance (NMR) spectroscopy. Hyperpolarisation offers enormous gains in signal and…

Long qubit coherence and efficient atom-photon coupling are essential for advanced applications in quantum communication. One technique to maintain coherence is dynamical decoupling, where a periodic sequence of refocusing pulses is…

Quantum Physics · Physics 2021-02-02 Chang Hoong Chow , Boon Long Ng , Christian Kurtsiefer

We study dynamical decoupling in a multi-qubit setting, where it is combined with quantum logic gates. This is illustrated in terms of computation using Heisenberg interactions only, where global decoupling pulses commute with the…

Quantum Physics · Physics 2008-08-14 K. Khodjasteh , D. A. Lidar

Nuclear quadrupolar resonance (NQR) spectroscopy reveals chemical bonding patterns in materials and molecules through the unique coupling between nuclear spins and local fields. However, traditional NQR techniques require macroscopic…

Mesoscale and Nanoscale Physics · Physics 2025-01-14 S. Alex Breitweiser , Mathieu Ouellet , Tzu-Yung Huang , Tim H. Taminiau , Lee C. Bassett

The use of nuclear spins as physical sensing systems is disadvantaged by their low signal responsivity, particularly when compared to sensing techniques based on electron spins. This primarily results from the small nuclear gyromagnetic…

We have developed semiconductor point contact devices in which nuclear spins in a nanoscale region are coherently controlled by all-electrical methods. Different from the standard nuclear-magnetic resonance technique, the longitudinal…

Quantum Physics · Physics 2009-11-13 Y. Hirayama , A. Miranowicz , T. Ota , G. Yusa , K. Muraki , S. K. Ozdemir , N. Imoto

We propose a nuclear-spin-polarization protocol in a general evolution-and-measurement framework. The protocol works in a spin-star configuration, where the central spin is coupled to the surrounding bath (nuclear) spins by flip-flop…

Quantum Physics · Physics 2022-12-07 Zhu-yao Jin , Jia-shun Yan , Jun Jing

Characteristic dips appear in the coherence traces of a probe qubit when dynamical decoupling (DD) is applied in synchrony with the precession of target nuclear spins, forming the basis for nanoscale nuclear magnetic resonance (NMR). The…

The central spin decoherence problem has been researched for over 50 years in the context of both nuclear magnetic resonance and electron spin resonance. Until recently, theoretical models have employed phenomenological stochastic…

Mesoscale and Nanoscale Physics · Physics 2012-08-03 Wayne M. Witzel , Malcolm S. Carroll , Lukasz Cywinski , S. Das Sarma

For a generic dynamical decoupling sequence employing a single-axis control, we study its efficiency in the presence of small errors in direction of the controlling-pulses. In the case that the corresponding ideal dynamical-decoupling…

Quantum Physics · Physics 2013-05-29 Zhihao Xiao , Lewei He , Wen-ge Wang

We report on a nanoscale quantum-sensing protocol which tracks a free precession of a single nuclear spin and is capable of estimating an azimuthal angle---a parameter which standard multipulse protocols cannot determine---of the target…

Quantum Physics · Physics 2018-09-17 Kento Sasaki , Kohei M. Itoh , Eisuke Abe

We present theoretical proposals for two-dimensional nuclear magnetic resonance spectroscopy protocols based on Nitrogen-vacancy (NV) centers in diamond that are strongly coupled to the target nuclei. Continuous microwave and…

Quantum Physics · Physics 2024-10-31 Matthias Kost , Jianming Cai , Martin B. Plenio