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Spectroscopy of magnetization-induced second-harmonic generation (MSHG) is studied in magnetic Co$_{x}$Ag$_{1-x}$ granular films containing Co nanoparticles. A strong resonance of the magnetic contrast of the second-harmonic generation…

Adaptation and Self-Organizing Systems · Physics 2007-05-23 E. M. Kim , T. V. Murzina , A. F. Kravets , M. Inoue , G. Marowsky , O. A. Aktsipetrov

Nonlinear optics of semiconductors is an important field of fundamental and applied research, but surprisingly the role of excitons in the coherent processes leading to harmonics generation has remained essentially unexplored. Here we…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 M. Lafrentz , D. Brunne , A. V. Rodina , V. V. Pavlov , R. V. Pisarev , D. R. Yakovlev , A. Bakin , M. Bayer

An optical Second-Harmonic Generation (SHG) allows to probe various structural and symmetry-related properties of materials, since it is sensitive to the inversion symmetry breaking in the system. Here, we investigate the SHG response from…

Mesoscale and Nanoscale Physics · Physics 2019-05-08 M. Vandelli , M. I. Katsnelson , E. A. Stepanov

Surfaces and interfaces of magnetic nanostructures can reveal rather interesting and unusual properties that differ substantially from those of bulky materials. Here we apply the surface-sensitive method of optical second harmonic…

Mesoscale and Nanoscale Physics · Physics 2018-12-13 T. V. Murzina , K. A. Lazareva , E. E. Shalygina , I. A. Kolmychek , E. A. Karashtin , N. S. Gusev , A. A. Fraerman

A comparative experimental investigation of the dependence of second harmonic generation (SHG) on applied external voltage between the standard nematic liquid crystalline material and an analogue ferromagnetic nematic liquid crystalline…

Soft Condensed Matter · Physics 2019-09-30 Jure Brence , Luka Cmok , Nerea Sebastian , Alenka Mertelj , Darja Lisjak , Irena Drevensek-Olenik

NiO is a good candidate for ultrafast magnetic switching because of its large spin density, antiferromagnetic order, and clearly separated intragap states. In order to detect and monitor the switching dynamics, we develop a systematic…

Other Condensed Matter · Physics 2008-11-26 C. Li , G. Lefkidis , W. Hübner

We report on the experimental and theoretical investigation of magnetic-field-induced second harmonic generation (SHG) and two-photon absorption (TPA) of excited exciton states ($n \geq 3$) of the yellow series in Cu$_2$O. In this…

Mesoscale and Nanoscale Physics · Physics 2020-04-01 A. Farenbruch , J. Mund , D. Fröhlich , D. R. Yakovlev , M. Bayer , M. A. Semina , M. M. Glazov

Using symmetry arguments we show how optical second harmonic generation (SHG) can be used to detect antiferromagnetism at surfaces and in thin films. Based on the group theoretical analysis of the nonlinear electric susceptibility we…

Condensed Matter · Physics 2007-05-23 A. Daehn , W. Huebner , K. H. Bennemann

Second-harmonic generation (SHG) is a well-known nonlinear spectroscopy method to probe electronic structure, specifically, in transition metal dichalcogenide (TMDC) monolayers. This work investigates the nonlinear dynamics of a strongly…

Second harmonic generation (SHG) is a non-linear optical process, where two photons coherently combine into one photon of twice their energy. Efficient SHG occurs for crystals with broken inversion symmetry, such as transition metal…

The efficient optical second-harmonic generation (SHG) of two-dimensional (2D) crystals, coupled with their atomic thickness that circumvents the phase-match problem, has garnered considerable attention. While various 2D heterostructures…

Materials Science · Physics 2023-10-31 Wontaek Kim , Gyouil Jeong , Juseung Oh , Jihun Kim , Kenji Watanabe , Takashi Taniguchi , Sunmin Ryu

Although second harmonic generation (SHG) is a promising and widely used method recently for studying 2D magnetic materials, the quantitative analysis of the full SHG tensor is currently challenging. In this letter, we describe a…

Strongly Correlated Electrons · Physics 2026-02-04 Banasree S. Mou , Stephen M. Winter

A comprehensive study of second harmonic generation on thermally oxidized MoS2 flakes with thickness ranging from monolayer up to seven layers is presented. Observing the fundamental nonlinear behavior for non-treated and oxidized MoS2…

We compute and analyze the dependence of excitonic second- and third-harmonic generation (SHG/THG) as a function of the optical excitation intensity in the presence of static electric fields by solving the semiconductor Bloch equations. Our…

Mesoscale and Nanoscale Physics · Physics 2025-11-10 Ruixin Zuo , Matthias Reichelt , Cong Ngo , Xiaohong Song , Weifeng Yang , Torsten Meier

Nonlinear optical (NLO) responses of noncentrosymmetric nonmagnets have drawn a lot of attention in the past decades because of their significance in materials characterization, green energy and device applications. However, the…

Materials Science · Physics 2024-07-25 Babu Baijnath Prasad , Guan-Fu Liu , Guang-Yu Guo

We report on the optical second harmonic generation (SHG) on the 1S exciton-polariton resonance in bulk ZnSe that is subject to an external magnetic field applied perpendicular to the light wave vector $\mathbf k$ (Voigt geometry). For the…

Mesoscale and Nanoscale Physics · Physics 2025-07-18 J. Mund , D. R. Yakovlev , A. Farenbruch , N. V. Siverin , M. A. Semina , M. M. Glazov , E. L. Ivchenko , M. Bayer

Second harmonic generation (SHG) is a nonlinear optical response arising exclusively from broken inversion symmetry in the electric-dipole limit. Recently, SHG has attracted widespread interest as a versatile and noninvasive tool for…

Recently Second Harmonic Generation (SHG) for the yellow exciton series in cuprous oxide has been demonstrated [J. Mund et al., Phys. Rev. B 98, 085203 (2018)]. Assuming perfect $O_{\mathrm{h}}$ symmetry, SHG is forbidden along certain…

We theoretically consider magnetization dynamics in a ferromagnetic slab induced by the magnetic field of a strong femtosecond laser pulse. The longitudinal geometry, in which the initial magnetization lies in both the plane of incidence…

Mesoscale and Nanoscale Physics · Physics 2025-04-01 Evgeny A. Karashtin , Tatiana V. Murzina

Optical second-harmonic generation (SHG) is a nonlinear parametric process that doubles the frequency of incoming light. Only allowed in non-centrosymmetric materials, it has been widely used in frequency modulation of lasers, surface…

Materials Science · Physics 2021-01-05 Wontaek Kim , Je Yhoung Ahn , Juseung Oh , Ji Hoon Shim , Sunmin Ryu
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